Search results for "tunne"
showing 10 items of 739 documents
Low-energy excitations from interacting tunneling units in the mean-field approximation
1991
Abstract The low-energy excitation spectrum of dilute concentrations of interacting tunneling quadrupoles randomly distributed in a non-polar medium was studied in the mean-field approximation. In particular the case of six-orientational tunneling quadrupoles (TQs) with a r−3 (elastic) interaction was considered. Because of the random position of the TQs, the internal field in a random variable and for relatively low concentrations has a Lorenzian probability distribution. The low-energy density of states is a constant and the low-energy excitations arise from the large internal fields, i.e. strongly interacting tunneling quadrupoles. The low-energy excitations were compared with those obta…
Pulsed-field studies of the magnetization reversal in molecular nanomagnets
2004
We report experimental studies of crystals of Mn12 molecular magnetic clusters in pulsed magnetic fields with sweep rates up to 4x10^3 T/s. The steps in the magnetization curve are observed at fields that are shifted with respect to the resonant field values. The shift systematically increases as the rate of the field sweep goes up. These data are consistent with the theory of the collective dipolar relaxation in molecular magnets.
Transitions between metastable states in silica clusters
1999
Relaxation phenomena in glasses can be related to jump processes between different minima of the potential energy in the configuration space. These transitions play a key role in the low temperature regime, giving rise to tunneling systems responsible for the anomalous specific heat and thermal conductivity in disordered solids with respect to crystals. By using a recently developed numerical algorithm, we study the potential energy landscape of silica clusters, taking as a starting point the location of first order saddle points. This allows us to find a great number of adjacent minima. We analyze the degree of cooperativity of these transitions and the connection of physical properties wi…
Inelastic neutron scattering study of the rotational excitations in(KBr)1−x(KCN)xin the paraelastic and structural glass state
1984
The coupled rotational-translational excitations in ${(\mathrm{KBr})}_{1\ensuremath{-}x}{(\mathrm{KCN})}_{x}$ were studied by inelastic neutron scattering for concentrations $0.008\ensuremath{\le}x\ensuremath{\le}0.20$. We followed the ${A}_{1g}\ensuremath{-}{T}_{2g}$ tunneling transition and the ${A}_{1g}\ensuremath{-}{E}_{g}$ librational excitation through the transition from the paraelastic to the structural glass state. We found that these two excitations and their coupling to the lattice strains exhibit a very different temperature dependence in the glass state. While the tunneling transition, which triggers reorientations of the ${\mathrm{CN}}^{\ensuremath{-}}$ ions, shows a drastic r…
Spin lattice relaxation rates of tunnelling CD3 groups
1991
The spin lattice relaxation rates of deuterated methyl groups are calculated for threefold and sixfold potentials. It is shown that it should be possible to determine the symmetry of the potential hindering the methyl groups from deuteron spin lattice relaxation experiments. The temperature dependence of the spin lattice relaxation rates is discussed using a simple model. The similarities and the differences between proton NMR and deuteron NMR are pointed out. The main difference is thatEa↔Eb transitions are forbidden by spin selection rules in case of CH3, but not for CD3. Therefore, and due to the fact that the quadrupolar interaction is a single particle interaction, deuteron NMR allows …
Quasiparticle interference of spin momentum locked surface states at step edges on Re(0001)
2020
Quasiparticle interference patterns formed by a surface state on the Re(0001) surface were investigated using scanning tunneling spectroscopy. The energy dispersion is inferred from Fourier-transformed differential conductivity maps for occupied and unoccupied states. The band dispersion for occupied states agrees with earlier published results obtained by angle-resolved photoemission spectroscopy. An analysis of the phase of interference patterns at step edges reveals a drastic change in the effective energy barrier for backscattering above and below the Fermi level. The attenuation of the interference pattern with increasing distance indicates interband scattering is the dominant scatteri…
The Impact of a Finite Waveguide Work Function on Resonant Tunneling
2021
To describe electron transport in a waveguide, we assume that the electron wave functions vanish at the waveguide boundary. This means that, being in the waveguide, an electron can not cross the waveguide boundary because of the infinite potential barrier. In reality, the assumption has never been fulfilled: generally, electrons can penetrate through the waveguide boundary and go some distance away from the waveguide. Therefore, we have to clarify how this phenomenon affects the resonant tunneling.
Spin scattering and spin-polarized hybrid interface states at a metal-organic interface
2011
Spin scattering at the interface formed between metallic Fe and Cu-phthalocyanine molecules is investigated by spin-polarized scanning tunneling spectroscopy and spin-resolved photoemission. The results are interpreted using first-principles electronic structure theory. The combination of experimental and theoretical techniques allows us to shed light on the role of hybrid interface states for the spin scattering. We show that Cu-phthalocyanine acts, via hybrid interface states, as a local spin filter up to room temperature both below and above the Fermi energy, ${E}_{\mathrm{F}}$. At the same time, the molecule behaves as a featureless scattering barrier in a region of about 1 eV around ${…
Manipulation of the spin in single molecule magnets via Landau-Zener transitions
2011
We theoretically investigate the effects of a magnetic pulse on a single-molecule magnet (SMM) initially magnetized by a dc field along the easy axis of magnetization. In the Landau\char21{}Zener (LZ) scheme, it is shown that the final spin state is a function of the shape and duration of the pulse, conditioned by the decoherence time of the SMM. In the case of coherent tunneling, the asymmetric pulses are shown to reverse the direction of the magnetization, while the symmetric pulses can only decrease the value of the initial magnetization. It is also demonstrated that the application of an external variable dc field in the hard plane of magnetization provides the possibility to tune the r…
Spin-lattice relaxation via quantum tunneling in anEr3+-polyoxometalate molecular magnet
2010
We investigate the mechanism of spin-lattice relaxation of Er ions encapsulated in polyoxometalate clusters, which below 4 K can only reverse its spin via quantum tunneling processes. The temperature-independent rate −1 is, at zero field, ten orders of magnitude larger than the rates predicted for direct phonon-induced processes. In addition, we observe that −1 is suppressed by external magnetic bias and hyperfine interactions but enhanced by increasing the concentration of Er ions. The observed relaxation agrees with predictions for pure quantum tunneling, showing that this phenomenon drives the thermalization of electronic spins. A possible link between these two phenomena is discussed, i…