Search results for "ultrafast"

Transient absorption and luminescence of LiNbO3 and KNbO3

2001

Abstract The results of time-resolved optical absorption spectra in congruent and stoichiometric LiNbO3 as well as KNbO3 crystals are reported. The role of different polaron types in transient absoiption and luminescence spectra and decay kinetics are discussed.

Luminescence and Transient Optical Absorption in CdWO<sub>4</sub>

1997

Ultrafast spectroscopic investigation on fluorescent carbon nanodots: the role of passivation.

2019

Disentangling the respective roles of the surface and core structures in the photocycle of carbon nanodots is a critical open problem in carbon nanoscience. While the need of passivating carbon dot surfaces to obtain efficiently emitting nanoparticles is very well-known in the literature, it is unclear if passivation introduces entirely new surface emitting states, or if it stabilizes existing states making them fluorescent. In this multi-technique femtosecond spectroscopy study, the relaxation dynamics of non-luminescent (non-passivated) carbon dots are directly compared with their luminescent (passivated) counterparts. Non-passivated dots are found to host emissive states, albeit very sho…

Photodynamics at the CdSe Quantum Dot–Perylene Diimide Interface: Unraveling the Excitation Energy and Electron Transfer Pathways

2021

Excitation energy and charge transfer processes in perylene diimide dye–CdSe quantum dot complexes have been studied by femtosecond transient absorption spectroscopy. After excitation of the quantu...

Relaxation of electronic excitations in LiNbO3crystals

2001

Transient absorption both in stoichiometric and Mg doped congruent LiNbO was observed after pulsed electron beam excitation. The luminescence spectra and decay kinetics in these materials show different excitonic relaxation possibilities. The dependence on sample stoichiometry is also discussed.

Tuning the Ultrafast Response of Fano Resonances in Halide Perovskite Nanoparticles

2020

International audience; The full control of the fundamental photophysics of nanosystems at frequencies as high as few THz is key for tunable and ultrafast nanophotonic devices and metamaterials. Here we combine geometrical and ultrafast control of the optical properties of halide perovskite nanoparticles, which constitute a prominent platform for nanophotonics. The pulsed photoinjection of free carriers across the semiconducting gap leads to a subpicosecond modification of the far-field electromagnetic properties that is fully controlled by the geometry of the system. When the nanoparticle size is tuned so as to achieve the overlap between the narrowband excitons and the geometry-controlled…

Luminescence and Transient Absorption of CdWO4Crystals

1999

Passively mode-locked erbium-doped double-clad fiber laser operating at the 322nd harmonic

2009

International audience; We report passive mode locking of a soliton erbium-doped double-clad fiber laser operating at the 322nd harmonic of the fundamental cavity frequency. Repetition rates up to 3 GHz have been obtained with pulses of 1 ps duration and 18 pJ of energy. The supermode suppression at the 322nd harmonic is better than 25 dB. In addition, the transition dynamics from a bunched state of pulses to stable harmonic mode locking is presented, revealing a very long time scale.

Ab Initio Simulation of Attosecond Transient Absorption Spectroscopy in Two-Dimensional Materials

2018

We extend the first-principles analysis of attosecond transient absorption spectroscopy to two-dimensional materials. As an example of two-dimensional materials, we apply the analysis to monolayer hexagonal boron nitride (h-BN) and compute its transient optical properties under intense few-cycle infrared laser pulses. Nonadiabatic features are observed in the computed transient absorption spectra. To elucidate the microscopic origin of these features, we analyze the electronic structure of h-BN with density functional theory and investigate the dynamics of specific energy bands with a simple two-band model. Finally, we find that laser-induced intraband transitions play a significant role in…

Affordable, ultra-broadband coherent detection of terahertz pulses via CMOS-compatible solid-state devices

2017

We demonstrate the first fully solid-state technique for the coherent detection of ultra-broadband THz pulses (0.1-10 THz), relying on the electric-field-induced second-harmonic generation attained in integrated CMOS-compatible devices.