Electron capture decay of116Inand nuclear structure of doubleβdecays

Quasiparticle-random-phase-approximation (QRPA) calculations of double $\ensuremath{\beta}$ decays have not been able to reproduce data in the $A=100$ system. We propose the $A=116$ system---because of its smaller deformation---as a simpler system to test QRPA calculations. We present results of two experiments we performed, which determine the electron-capture-decay branch of ${}^{116}\mathrm{In}$ to be $(2.27\ifmmode\pm\else\textpm\fi{}0.63)\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}2}%$, from which we deduce $\mathrm{log}{ft=4.39}_{\ensuremath{-}0.15}^{+0.10}$. We present QRPA calculations and compare their predictions to experimental data. Finally we use these calculations to…

Entry distribution of 220Th: A method to determine the fission barrier of an unstable nucleus

Evolution of collective motion in light polonium nuclei

The {gamma}-ray spectroscopy of even- and odd-mass isotopes of polonium have been studied using arrays of Ge detectors coupled to recoil-mass analyzers, including recoil-decay tagging techniques. The level energies and B(E2) branching ratios can be reproduced by theoretical frameworks which do not explicitly include proton particle-hole excitations across the Z = 82 shell, conclusions in contrast to those deduced from alpha-decay measurements.

Proton radioactivity of117La

A new more precise measurement of the ground-state proton decay of ${}^{117}\mathrm{La}$ is presented $[{E}_{p}=806(5) \mathrm{keV},$ ${t}_{1/2,p}=26(3)$ ms]. ${}^{117}\mathrm{La}$ was produced via the $p4n$ fusion-evaporation channel by bombarding a ${}^{64}\mathrm{Zn}$ target with 310 and 295 MeV ${}^{58}\mathrm{Ni}$ beams. The proton decay rate is consistent with emission from a prolate deformed ${3/2}^{+}$ or ${3/2}^{\ensuremath{-}}$ Nilsson state. No evidence is found for a previously reported proton decay from a high spin isomer in ${}^{117}\mathrm{La}.$ An upper limit for the production cross section for proton decay of ${}^{116}\mathrm{La}$ at a bombarding energy of 325 MeV was esta…

Search for a 2-quasiparticle high-Kisomer inRf256

The energies of 2-quasiparticle (2-qp) states in heavy shell-stabilized nuclei provide information on the single-particle states that are responsible for the stability of superheavy nuclei. We have calculated the energies of 2-qp states in {sup 256}Rf, which suggest that a long-lived, low-energy 8{sup -} isomer should exist. A search was conducted for this isomer through a calorimetric conversion electron signal, sandwiched in time between implantation of a {sup 256}Rf nucleus and its fission decay, all within the same pixel of a double-sided Si strip detector. A 17(5)-{mu}s isomer was identified. However, its low population, {approx}5(2)% that of the ground state instead of the expected {a…

α-decay properties ofPb181

The isotope {sup 181}Pb was produced in {sup 92}Mo bombardments of {sup 90}Zr and, together with other reaction products, was passed through a recoil mass separator and implanted in a double-sided silicon strip detector for {alpha}-particle assay. The half-life and energy of the main {sup 181}Pb {alpha} transition were determined to be 45 (20) ms and 7065 (20) keV, respectively. This {sup 181}Pb {ital E}{sub {alpha}} agrees with one previously measured value [7044 (15) keV], but not with the one [7211 (10) keV] used as input to the 1993 Atomic Mass Evaluation. The 6180-keV {alpha} transition assigned to {sup 181}Tl by Bolshakov {ital et} {ital al}. was observed, but the 6566-keV {alpha} par…

Kπ=8−isomers andKπ=2−octupole vibrations inN=150shell-stabilized isotones

Isomers have been populated in {sup 246}Cm and {sup 252}No with quantum numbers K{sup {pi}}=8{sup -}, which decay through K{sup {pi}}=2{sup -} rotational bands built on octupole vibrational states. For N=150 isotones with (even) atomic number Z=94-102, the K{sup {pi}}=8{sup -} and 2{sup -} states have remarkably stable energies, indicating neutron excitations. An exception is a singular minimum in the 2{sup -} energy at Z=98, due to the additional role of proton configurations. The nearly constant energies, in isotones spanning an 18% increase in Coulomb energy near the Coulomb limit, provide a test for theory. The two-quasiparticle K{sup {pi}}=8{sup -} energies are described with single-pa…

Identification of excited states in119Ba

Excited states have been identified in the very neutron-deficient ${}^{119}\mathrm{Ba}$ nucleus. Two bands have been observed, which are likely to be based on ${h}_{11/2}$ and ${(g}_{7/2}{d}_{5/2})$ neutron orbitals. Despite this being the first observation of excited states in ${}^{119}\mathrm{Ba},$ the bands extend to $(75/2)\ensuremath{\Elzxh}$ and $(79/2)\ensuremath{\Elzxh},$ respectively. The bands have been assigned to ${}^{119}\mathrm{Ba}$ using gamma-recoil and gamma--x-ray coincidences. Several quasiparticle alignments have been identified, involving neutron ${(h}_{11/2}{)}^{2}$ and proton ${(h}_{11/2}{)}^{2}$ aligned configurations. Furthermore, the bands show features which are r…

Identification of yrast states in187Pb

gamma-ray spectroscopy of the high-spin states of the neutron-deficient nucleus Pb-187 has been conducted with the Gd-155(Ar-36,4n) reaction. A cascade of three transitions was deduced from gamma-gamma coincidence data gated by detection of recoiling evaporation residues in a gas-filled recoil separator. In an earlier, separate experiment, two of these gamma rays were positively identified with Pb-187 by recoil-gamma coincidence measurements with a high-resolution, recoil mass spectrometer. From comparison with similar sequences in heavier odd-A lead isotopes, the cascade in Pb-187 is associated with the sequence of three E2 transitions from the yrast 25/2(+) level to a low-lying 13/2(+) is…

Proton radioactivity of 117La

A new more precise measurement of the ground-state proton decay of 117La is presented @Ep 5806(5) keV, t1/2,p526(3) ms#. 117La was produced via the p4n fusion-evaporation channel by bombarding a 64Zn target with 310 and 295 MeV 58Ni beams. The proton decay rate is consistent with emission from a prolate deformed 3/21 or 3/22 Nilsson state. No evidence is found for a previously reported proton decay from a high spin isomer in 117La. An upper limit for the production cross section for proton decay of 116La at a bombarding energy of 325 MeV was established. peerReviewed

Structure of the Odd-A, Shell-Stabilized NucleusNo102253

In-beam {gamma}-ray spectroscopic measurements have been made on {sub 102}{sup 253}No. A single rotational band was identified up to a probable spin of 39/2({Dirac_h}/2{pi}), which is assigned to the 7/2{sup +}[624] Nilsson configuration. The bandhead energy and the moment of inertia provide discriminating tests of contemporary models of the heaviest nuclei. Novel methods were required to interpret the sparse data set associated with cross sections of around 50 nb. These methods included comparisons of experimental and simulated spectra, as well as testing for evidence of a rotational band in the {gamma}{gamma} matrix.

Proton Decay of an Intruder State inB185i

The new proton radioactivity ${}^{185m}\mathrm{Bi}$ has been observed, produced via the ${}^{95}\mathrm{Mo}{(}^{92}\mathrm{Mo},pn{)}^{185}\mathrm{Bi}$ reaction. Its decay proceeds from the low-lying ${\frac{1}{2}}^{+}$ intruder state in ${}^{185}\mathrm{Bi}$ to the ${}^{184}\mathrm{Pb}$ ground state with the emission of a proton of energy $1.585\ifmmode\pm\else\textpm\fi{}0.009\mathrm{MeV}$ and a half-life of $44\ifmmode\pm\else\textpm\fi{}16\ensuremath{\mu}\mathrm{s}$. This marks the first observation of proton radioactivity above the $Z\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}82$ closed shell, and it has been used to obtain the admixture of a ${0}^{+}$ intruder state in ${}^{184…

Mass and low-lying levels ofIn106,108from theCd106,108(p,nγ)reactions

106In has been studied via the reaction 106Cd(p,nγ)106In in the energy range Ep=7-9 MeV. Inbeam γ-ray excitation functions, γ-γ coincidence measurements, and β+-delayed γ-ray excitation functions have been used to identify thirteen levels in 106In. From this new level scheme the energy separation of the high-spin ground state and the low-spin isomer has been determined to be 28.6±0.5 keV. The threshold energy of the strongest low-lying γ-ray transition yields a mass excess for 106In of -80601±15 keV. Spins for some states are suggested by comparing the excitation functions to Hauser-Feshbach calculations. In-beam γ-ray excitation functions for the 108Cd(p,nγ)108In reaction give a mass exces…

Half-life measurements for neutron-rich Tc, Ru, Rh, and Pd isotopes. Identification of the new isotopesTc111,Ru113, andRh113

The decays of three new neutron-rich nuclides $^{111}\mathrm{Tc}$, $^{113}\mathrm{Ru}$, and $^{113}\mathrm{Rh}$ have been observed at an on-line isotope separator facility. In addition, the beta decays of several other n-rich isotopes with Ag100 have been studied for the first time. The new half-lives reported in this work include: $^{111}\mathrm{Tc}$ [${T}_{1/2}$=0.30(3) s], $^{111}\mathrm{Ru}$ [2.12(7) s], $^{112}\mathrm{Ru}$ [1.75(7) s], $^{113}\mathrm{Ru}$ [0.80(10) s], $^{113}\mathrm{Rh}$ [2.72(22) s], and $^{118}\mathrm{Pd}$ [2.24(17) s]. In general, these results support the microscopic theoretical half-life predictions below Z=50.

New Neutron-Rich Nuclei and Isomers Produced in Symmetric Fisson

The novel method for rapid on-line mass separation, the IGISOL, is described. The method has been shown applicable to mass separation of short-lived proton-induced fission products without any chemical dependence on radionuclide. Recent results on isomeric states with half-lives of the order of milliseconds produced directly in proton-induced fission of 238U and separated with the IGISOL are presented. The future plans for connection of the new K-130 cyclotron of the University of Jyvaskyla with the IGISOL are reviewed.

Competing T = 0 and T = 1 structures in the N = Z nucleus $^{62}_{31}$Ga

Abstract The low-lying levels in the odd-odd N = Z nucleus 62 Ga have been identified for the first time. These data reveal a cascade of stretched-E2 transitions based on a T =0, 1 + bandhead which decays directly to the T =1, 0 + ground state. The observed levels are interpreted in the context of theshell model, using as a basis, the pf 5/2 g 9/2 orbits with a 56 Ni core.

Bridging the nuclear structure gap between stable and super heavy nuclei

International audience; Due to recent advances in detection techniques, excited states in several trans-fermium nuclei were studied in many laboratories worldwide, shedding light on the evolution of nuclear structure between stable nuclei and the predicted island of stability centered around spherical magic numbers. In particular, studies of K-isomers around the Z=100 and N=152 deformed shell closures extended information on the energies of Nilsson orbitals at the Fermi surface. Some of these orbitals originate from spherical states, which are relevant to the magic gaps in super-heavy nuclei. The single-particle energies can be used to test various theoretical predictions and aid in extrapo…

Gamow-Teller decay of118Pd and of neighbouring even isotopes of palladium

Neutron-rich isotopes of palladium were produced via the fission of238U by 20 MeV protons. These isotopes were selected using the ion guide-fed on-line mass-separator facility IGISOL at Jyvaskyla. Their decays were studied byβ-ray,γ-ray and conversion-electron spectroscopy. For114Pd and116Pd, the decay schemes established previously were confirmed; additionally multipolarities were determined for a few transitions. In the case of118Pd, only an approximate half-life was known from a previous radiochemical experiment. In the present study, 15 gamma transitions were observed, most of which were placed in a decay scheme. The half-life and the decay energy were found to beT1/2=1.9±0.1 s andQβ=4.…

Effect of a Triaxial Nuclear Shape on Proton Tunneling: The Decay and Structure of 145Tm

Gamma rays deexciting states in the proton emitter 145Tm were observed using the recoil-decay tagging method. The 145Tm ground-state rotational band was found to exhibit the properties expected for an h{11/2} proton decoupled band. In addition, coincidences between protons feeding the 2{+} state in 144Er and the 2{+}-->0{+} gamma-ray transition were detected, the first measurement of this kind, leading to a more precise value for the 2{+} excitation energy of 329(1) keV. Calculations with the particle-rotor model and the core quasiparticle coupling model indicate that the properties of the pi{11/2} band and the proton-decay rates in 145Tm are consistent with the presence of triaxiality with…

Recoil Decay Tagging Study Of Transitional Proton Emitters 145,146,147Tm

International audience; Gamma rays from the transitional proton emitting nuclei 145,146,147Tm have been observed using the recoil-decay tagging technique. The ground state band of 147Tm was confirmed and extended and the unfavoured signature sequence was observed. A ground state rotational band with properties of a decoupled h11/2 band was observed in 145Tm. In addition coincidences between the proton fine structure line and the 2+-->0+ gamma-ray transition in 144Er were detected at the focal plane of the FMA. This is the first time that coincidences between proton radioactive decays and gamma rays have been seen. The particle decay of 146Tm has been measured with improved statistics and a …