Implantation-decay station for low-energy proton measurements

Abstract We have built an implantation-decay station for β - delayed proton and α decay studies at the focal plane of the Momentum Achromat Recoil Spectrometer (MARS) at the Cyclotron Institute of Texas A&M University. Energetic secondary beams with a small momentum spread are stopped in a controlled manner into a very thin silicon strip detector. In addition, high-purity germanium detectors are installed for γ ray detection. Here we give a description of the setup and the observed performance down to E p ≈ 200 keV using implanted 23 Al and 31 Cl sources.

Reevaluation of theP30(p,γ)S31astrophysical reaction rate from a study of theT=1/2mirror nuclei,S31andP31

The $^{30}\mathrm{P}$($p,\ensuremath{\gamma}$)$^{31}\mathrm{S}$ reaction rate is expected to be the principal determinant for the endpoint of nucleosynthesis in classical novae. To date, the reaction rate has only been estimated through Hauser-Feschbach calculations and is unmeasured experimentally. This paper aims to remedy this situation. Excited states in $^{31}\mathrm{S}$ and $^{31}\mathrm{P}$ were populated in the $^{12}\mathrm{C}$($^{20}\mathrm{Ne}$,$n$) and $^{12}\mathrm{C}$($^{20}\mathrm{Ne}$,$p$) reactions, respectively, at a beam energy of 32 MeV, and their resulting $\ensuremath{\gamma}$decay was detected with the Gammasphere array. Around half the relevant proton unbound states …

Exploring the 10Li structure by the d(9Li,p)10Li transfer reaction

The 9Li + 2H reaction has been investigated at 11 AMeV incident energy at the ISAC II facility (TRIUMF). In the present paper we focus on the one-neutron transfer channel, which potentially holds spectroscopic information on the unbound nucleus 10Li. The TUDA setup has been used in order to detect and identify the outgoing 9Li at forward angles and the recoil protons at backward angles. This setup allows to study the 10Li emitted in the crucial region at forward angles in the center of mass.

First Measurement of Severalβ-Delayed Neutron Emitting Isotopes BeyondN=126

The β-delayed neutron emission probabilities of neutron rich Hg and Tl nuclei have been measured together with β-decay half-lives for 20 isotopes of Au, Hg, Tl, Pb, and Bi in the mass region N≳126. These are the heaviest species where neutron emission has been observed so far. These measurements provide key information to evaluate the performance of nuclear microscopic and phenomenological models in reproducing the high-energy part of the β-decay strength distribution. This provides important constraints on global theoretical models currently used in r-process nucleosynthesis.

Proton radioactivity of117La

A new more precise measurement of the ground-state proton decay of ${}^{117}\mathrm{La}$ is presented $[{E}_{p}=806(5) \mathrm{keV},$ ${t}_{1/2,p}=26(3)$ ms]. ${}^{117}\mathrm{La}$ was produced via the $p4n$ fusion-evaporation channel by bombarding a ${}^{64}\mathrm{Zn}$ target with 310 and 295 MeV ${}^{58}\mathrm{Ni}$ beams. The proton decay rate is consistent with emission from a prolate deformed ${3/2}^{+}$ or ${3/2}^{\ensuremath{-}}$ Nilsson state. No evidence is found for a previously reported proton decay from a high spin isomer in ${}^{117}\mathrm{La}.$ An upper limit for the production cross section for proton decay of ${}^{116}\mathrm{La}$ at a bombarding energy of 325 MeV was esta…

Approaching the precursor nuclei of the third r-process peak with RIBs

The rapid neutron nucleosynthesis process involves an enormous amount of very exotic neutron-rich nuclei, which represent a theoretical and experimental challenge. Two of the main decay properties that affect the final abundance distribution the most are half-lives and neutron branching ratios. Using fragmentation of a primary $^{238}$U beam at GSI we were able to measure such properties for several neutron-rich nuclei from $^{208}$Hg to $^{218}$Pb. This contribution provides a short update on the status of the data analysis of this experiment, together with a compilation of the latest results published in this mass region, both experimental and theoretical. The impact of the uncertainties …

Investigation of multiparticle final states in12C photoreactions

The ${}^{12}\mathrm{C}(\ensuremath{\gamma},pn)$, ${}^{12}\mathrm{C}(\ensuremath{\gamma},pp)$, ${}^{12}\mathrm{C}(\ensuremath{\gamma},ppp)$, ${}^{12}\mathrm{C}(\ensuremath{\gamma},pp{\ensuremath{\pi}}^{\ifmmode\pm\else\textpm\fi{}})$, ${}^{12}\mathrm{C}(\ensuremath{\gamma},p{\ensuremath{\pi}}^{\ifmmode\pm\else\textpm\fi{}})$ reactions have been studied using tagged photons of energy ${E}_{\ensuremath{\gamma}}=250$--600 MeV. A model which includes all major absorption mechanisms and final state interactions gives results that agree well with the shapes of missing energy spectra, but for some channels the predicted cross sections are too large.

Commissioning of the BRIKEN beta-delayed neutron detector for the study of exotic neutron-rich nuclei

Beta-delayed neutron emission (Beta-n) is a form of radioactive decay in which an electron, an anti-neutrino and one or more neutrons are emitted. This process arises if the energy window of the decay Q_Beta is greater than the neutron separation energy S n of the daughter. The probability in each decay of emitting neutrons is called the Pn value. This form of decay plays a key role in the synthesis of chemical elements in the Universe via the rapid neutron capture process, or r-process. The r-process proceeds far from the valley of nuclear stability, and leads to very neutron-rich nuclei that then decay to the line of stability. Most of these nuclei are ßn emitters. The initial abundance d…

Evidence for a Smooth Onset of Deformation in the Neutron-Rich Kr Isotopes

The neutron-rich nuclei Kr94,96 were studied via projectile Coulomb excitation at the REX-ISOLDE facility at CERN. Level energies of the first excited 2 + states and their absolute E2 transition strengths to the ground state are determined and discussed in the context of the E(21+) and B(E2;21+→01+) systematics of the krypton chain. Contrary to previously published results no sudden onset of deformation is observed. This experimental result is supported by a new proton-neutron interacting boson model calculation based on the constrained Hartree-Fock-Bogoliubov approach using the microscopic Gogny-D1M energy density functional. © 2012 American Physical Society.

Sub-Barrier Coulomb Excitation ofSn110and Its Implications for theSn100Shell Closure

The first excited 2(+) state of the unstable isotope Sn-110 has been studied in safe Coulomb excitation at 2.82 MeV/u using the MINIBALL array at the REX-ISOLDE post accelerator at CERN. This is the first measurement of the reduced transition probability of this state using this method for a neutron deficient Sn isotope. The strength of the approach lies in the excellent peak-to-background ratio that is achieved. The extracted reduced transition probability, B(E2 : 0(+) -> 2(+)) 0.220 +/- 0.022e(2) b(2), strengthens the observation of the evolution of the B(E2) values of neutron deficient Sn isotopes that was observed recently in intermediate-energy Coulomb excitation of Sn-108. It implies …

Coulomb Excitation of Neutron-Rich Zn Isotopes: First Observation of the21+State inZn80

Neutron-rich, radioactive Zn isotopes were investigated at the Radioactive Ion Beam facility REX-ISOLDE (CERN) using low-energy Coulomb excitation. The energy of the 2(1)+ state in 78Zn could be firmly established and for the first time the 2+ --> 0(1)+ transition in 80Zn was observed at 1492(1) keV. B(E2,2(1)+ --> 0(1)+) values were extracted for (74,76,78,80)Zn and compared to large scale shell model calculations. With only two protons outside the Z=28 proton core, 80Zn is the lightest N=50 isotone for which spectroscopic information has been obtained to date. Two sets of advanced shell model calculations reproduce the observed B(E2) systematics. The results for N=50 isotones indicate a g…

Collectivity in the light radon nuclei measured directly via Coulomb excitation

Background: Shape coexistence in heavy nuclei poses a strong challenge to state-of-the-art nuclear models, where several competing shape minima are found close to the ground state. A classic region for investigating this phenomenon is in the region around Z=82 and the neutron midshell at N=104. Purpose: Evidence for shape coexistence has been inferred from α-decay measurements, laser spectroscopy, and in-beam measurements. While the latter allow the pattern of excited states and rotational band structures to be mapped out, a detailed understanding of shape coexistence can only come from measurements of electromagnetic matrix elements. Method: Secondary, radioactive ion beams of Rn202 and Rn…

Mirror energy differences in theA=31mirror nuclei,S31andP31, and their significance in electromagnetic spin-orbit splitting

Excited states in $^{31}\mathrm{S}$ and $^{31}\mathrm{P}$ were populated in the $^{12}\mathrm{C}$($^{20}\mathrm{Ne}$,n) and $^{12}\mathrm{C}$($^{20}\mathrm{Ne}$,p) reactions, respectively, at a beam energy of 32 MeV. High spin states of positive and negative parity have been observed in $^{31}\mathrm{S}$ for the first time, and the yrast scheme of $^{31}\mathrm{P}$ has been extended. Large mirror energy differences between the first $9/{2}^{\ensuremath{-}}$ and $13/{2}^{\ensuremath{-}}$ states were observed, but only small differences for the first $7/{2}^{\ensuremath{-}}$ and $11/{2}^{\ensuremath{-}}$ levels. The significance of these observations is discussed in relation to the electromag…

Experimental study ofβ-delayed proton decay ofAl23for nucleosynthesis in novae

The $\ensuremath{\beta}$-delayed $\ensuremath{\gamma}$ and proton decay of $^{23}\mathrm{Al}$ has been studied with an alternative detector setup at the focal plane of the momentum achromat recoil separator MARS at Texas A University. We could detect protons down to an energy of 200 keV and determine the corresponding branching ratios. Contrary to results of previous $\ensuremath{\beta}$-decay studies, no strong proton intensity from the decay of the isobaric analog state (IAS) of the $^{23}\mathrm{Al}$ ground state at ${E}_{x}=7803$ keV in $^{23}\mathrm{Mg}$ was observed. Instead we assign the observed low-energy group ${E}_{p,\mathrm{c}.\mathrm{m}.}=206$ keV to the decay from a state that…

Proton photoproduction from 12C

Abstract The 12 C(γ,p) differential cross-section in the Δ-resonance region has been measured using tagged photons. Data are presented for 20 MeV wide photon energy bins at 200, 300, 400 and 500 MeV and for proton angles from 52° to 128°. The present 12 C(γ,p) measurements are compared with previous experiments carried out at Frascati, Tokyo and Bonn. Comparisons are also made with theoretical calculations developed at Gent and Valencia which provide an interpretation of the photon reaction mechanism in terms of the major contributing processes. Coincidence data with correlated neutrons, protons and pions are also presented.

Determination of the B(E3, 0+ → 3−)-excitation strength in octupole-correlated nuclei near A ≈224 by the means of Coulomb excitation at REX-ISOLDE

The IS475 collaboration conducted Coulomb-excitation experiments with postaccelerated radioactive 220Rn and 224Ra beams at the REX-ISOLDE facility. The beam particles (Ebeam ≈ 2.83 MeV/u) were Coulomb excited using 60Ni, 114Cd, and 120Sn scattering targets. De-excitation γ-rays were detected employing the Miniball array and scattered particles were detected in a silicon detector. Exploiting the Coulomb-excitation code GOSIA for each nucleus several matrix elements could be obtained from the measured γ-ray yields. The extracted 3−||Ê3||0+ matrix element allows for the conclusion that, while 220Rn represents an octupole vibrational system, 224Ra has already substantial octupole correlations i…

Candidate superdeformed band in 28Si

Proton Decay of an Intruder State inB185i

The new proton radioactivity ${}^{185m}\mathrm{Bi}$ has been observed, produced via the ${}^{95}\mathrm{Mo}{(}^{92}\mathrm{Mo},pn{)}^{185}\mathrm{Bi}$ reaction. Its decay proceeds from the low-lying ${\frac{1}{2}}^{+}$ intruder state in ${}^{185}\mathrm{Bi}$ to the ${}^{184}\mathrm{Pb}$ ground state with the emission of a proton of energy $1.585\ifmmode\pm\else\textpm\fi{}0.009\mathrm{MeV}$ and a half-life of $44\ifmmode\pm\else\textpm\fi{}16\ensuremath{\mu}\mathrm{s}$. This marks the first observation of proton radioactivity above the $Z\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}82$ closed shell, and it has been used to obtain the admixture of a ${0}^{+}$ intruder state in ${}^{184…

Compton imaging with AGATA and SmartPET for DESPEC

DESPEC (DEcay SPECtroscopy) is a spectrometer, currently under construction, which is to be used at the FAIR (Facility for Antiproton and Ion Research) facility at GSI Darmstadt, Germany, as part of the NuSTAR (Nuclear STructure, Astrophysics and Reactions) project. Its goal is to analyse the decay of exotic nuclei produced via the Super-FRS (SUPERconducting FRagment Separator). The optimal configuration of certain elements of the spectrometer, namely a HPGe (High Purity Germanium) tracking array, is still under consideration. Work currently being carried out at the University of Liverpool using a segmented, coaxial HPGe detector (AGATA B009) and a pixelated, planar HPGe detector (SmartPET …

10Li low-lying resonances populated by one-neutron transfer

The 9Li + 2H → 10Li + 1H one-neutron transfer reaction has been performed at 100 MeV incident energy at TRIUMF using a 9Li beam delivered by the ISAC-II facility. A setup based on double-sided silicon strip detectors has been used in order to detect and identify the outgoing 9Li produced by the 10Li breakup at forward angles and the recoil protons emitted at backward angles. The 10Li low-lying resonances, whose energies, widths and configurations are still unclear, have been populated with significant statistics.

The Miniball spectrometer

The Miniball germanium detector array has been operational at the REX (Radioactive ion beam EXperiment) post accelerator at the Isotope Separator On-Line facility ISOLDE at CERN since 2001. During the last decade, a series of successful Coulomb excitation and transfer reaction studies have been performed with this array, utilizing the unique and high-quality radioactive ion beams which are available at ISOLDE. In this article, an overview is given of the technical details of the full Miniball setup, including a description of the γ-ray and particle detectors, beam monitoring devices and methods to deal with beam contamination. The specific timing properties of the REX-ISOLDE facility are hi…

β -decay half-lives and β -delayed neutron emission probabilities for several isotopes of Au, Hg, Tl, Pb, and Bi, beyond N=126

Background: Previous measurements of Beta-delayed neutron emitters comprise around 230 nuclei, spanning from the 8He up to 150La. Apart from 210Tl, with a minuscule branching ratio of 0.07%, no other neutron emitter is measured yet beyond A = 150. Therefore new data are needed, particularly in the heavy mass region around N=126, in order to guide theoretical models and to understand the formation of the third r-process peak at A 195. Purpose: To measure both, Beta-decay half-lives and neutron branching ratios of several neutron-rich Au, Hg, Tl, Pb and Bi isotopes beyond N = 126. Method: Ions of interest are produced by fragmentation of a 238U beam, selected and identifed via the GSI-FRS fra…

12C(γ,π+n) and 12C(γ,π+p) reactions across the Δ resonance region

Abstract Differential cross-sections from (γ,π+n) and (γ,π+p) experiments on 12C are presented together with a microscopic model calculation. The comparison of experimental data with theory confirms that quasifree pion production is the dominant process for the (γ,π+n) reaction. The comparison of (γ,π+p) with (γ,π+n) data shows the importance of final state interactions. first time to experimentally study the strength and the possible mechanisms involved in the final state interaction.

Studies of pear-shaped nuclei using accelerated radioactive beams

There is strong circumstantial evidence that certain heavy, unstable atomic nuclei are ‘octupole deformed’, that is, distorted into a pear shape. This contrasts with the more prevalent rugby-ball shape of nuclei with reflection-symmetric, quadrupole deformations. The elusive octupole deformed nuclei are of importance for nuclear structure theory, and also in searches for physics beyond the standard model; any measurable electric-dipole moment (a signature of the latter) is expected to be amplified in such nuclei. Here we determine electric octupole transition strengths (a direct measure of octupole correlations) for short-lived isotopes of radon and radium. Coulomb excitation experiments we…

Accelerated radioactive beams from REX-ISOLDE

In 2001 the linear accelerator of the Radioactive beam EXperiment (REX-ISOLDE) delivered for the first time accelerated radioactive ion beams, at a beam energy of 2 MeV/u. REX-ISOLDE uses the method of charge-state breeding, in order to enhance the charge state of the ions before injection into the LINAC. Radioactive singly-charged ions from the on-line mass separator ISOLDE are first accumulated in a Penning trap, then charge bred to an A/q < 4.5 in an electron beam ion source (EBIS) and finally accelerated in a LINAC from 5 keV/u to energies between 0.8 and 2.2 MeV/u. Dedicated measurements with REXTRAP, the transfer line and the EBIS have been carried out in conjunction with the first co…

Nuclear pion photoproduction in theΔresonance region

A measurement of the /sup 12/C( gamma , pi /sup +/n)/sup 11/B reaction in quasifree pi -production kinematic regimes has been performed using tagged photons in conjunction with large solid angle pi and n detectors. The aim of the experiment was to investigate predicted modifications to the Delta excitation of nucleons and their subsequent propagation and decay, brought about by the nuclear medium. Differential cross sections are presented for photon energies spanning the Delta (1232) excitation region. The measurements are consistent with distorted wave impulse approximation calculations in which the amplitude for proton Delta excitation, followed by Delta propagation and decay to pi /sup +…

Superallowed Gamow-Teller decay of the doubly magic nucleus $^{100}$Sn

Expérience au GSI; The shell structure of atomic nuclei is associated with 'magic numbers' and originates in the nearly independent motion of neutrons and protons in a mean potential generated by all nucleons. During b1-decay, a proton transforms into a neutron in a previously not fully occupied orbital, emitting a positron-neutrino pair with either parallel or antiparallel spins, in a Gamow-Teller or Fermi transition, respectively. The transition probability, or strength, of a Gamow-Teller transition depends sensitively on the underlying shell structure and is usually distributed among many states in the neighbouring nucleus. Here we report measurements of the half-life and decay energy fo…

β-delayed neutron emission measurements around the third r-process abundance peak

This contribution summarizes an experiment performed at GSI (Germany) in the neutron-rich region beyond N=126. The aim of this measurement is to provide the nuclear physics input of relevance for r-process model calculations, aiming at a better understanding of the third r-process abundance peak. Many exotic nuclei were measured around 211Hg and 215Tl. Final ion identification diagrams are given in this contribution. For most of them, we expect to derive halflives and and β-delayed neutron emission probabilities. The detectors used in this experiment were the Silicon IMplantation and Beta Absorber (SIMBA) detector, based on an array of highly segmented silicon detectors, and the BEta deLayE…

Do nuclei go pear-shaped? Coulomb excitation of 220Rn and 224Ra at REX-ISOLDE (CERN)

Artículo escrito por muchos autores, sólo se referencian el primero, los autores que firman como Universidad Autónoma de Madrid y el grupo de colaboración en el caso de que aparezca en el artículo

Studies of astrophysically interesting nucleus23Al

We have studied the β-delayed proton decay of 23Al with a novel detector setup at the focal plane of the MARS separator at the Texas A&M University to resolve existing controversies about the proton branching of the IAS in 23Mg and to determine the absolute proton branchings by combining our results to the latest βγ-decay data. We have made also a high precision mass measurement of the ground state of 23Al to establish more accurate proton separation energy of 23Al. Here the description of the used techniques along with preliminary results of the experiments are given.

β-decay and β-delayed Neutron Emission Measurements at GSI-FRS Beyond N=126, for r-process Nucleosynthesis

New measurements of very exotic nuclei in the neutron-rich region beyond N=126 have been performed at the GSI facility with the fragment separator (FRS). The aim of the experiment is to determine half-lives and β-delayed neutron emission branching ratios of isotopes of Hg, Tl and Pb in this region. This contribution summarizes final counting statistics for identification and for implantation, as well as the present status of the data analysis of the half-lives. In summary, isotopes of Pt, Au, Hg, Tl, Pb, Bi, Po, At, Rn and Fr were clearly identified and several of them (208-211Hg, 211-215Tl, 214-218Pb) were implanted with enough statistics to determine their half-lives. About half of them a…

Coulomb excitation of Na-29,Na-30: Mapping the borders of the island of inversion

Seidlitz, M., et all ; 10 pags. ; 9 figs. ; 1 tab. ; PACS number(s): 21.60.Cs, 23.20.Js, 25.70.De, 29.38.Gj