0000000000006404
AUTHOR
O. Klepper
Laser spectroscopy of radioactive lead and thallium isotopes
By collincar fast beam laser spectroscopy hyperfine structure and isotope shift have been measured of neutron deficient radioactive isotopes of lead (190Pb,191Pb,192Pb,193Pb,194Pb,195Pb,196Pb,197Pb) and thallium (188Tl190Tl,191Tl,192Tl,194Tl,196Tl). Therefrom nuclear magnetic dipole moments, electric quadrupole moments, changes of the mean square charge radii and deformation parameters are deduced and compared with predictions from theory.
Precision experiments with time-resolved Schottky mass spectrometry
Abstract A large area on the mass surface of neutron-deficient nuclides (36≤Z≤85) was measured with time-resolved Schottky mass spectrometry at the FRS-ESR facilities. The masses of 114 nuclides were obtained for the first time from which 43 were determined via known decay energies. The improved mass accuracy of 30 keV allowed to study the isospin dependence of nuclear pairing, to precisely locate the one-proton dripline for odd-Z isotopes from Tb to Pa and to make crucial tests of the predictive powers of modern mass models.
Nuclear moments and change in the charge-radii of neutron deficient lead isotopes
The nuclear moments of195Pb and the change in the charge radii of192,194,195,196Pb have been determined from the isotope shift and hyperfine structure of the 723 nm line of neutral lead by collinear laser spectroscopy.
Collinear laser spectroscopy on108g, 108m In using an ion source with bunched beam release
The hyperfine structure and isotope shift of108gIn and108mIn have been investigated by means of collinear fast-beam laser spectroscopy in the resonance line atλ=451 nm. The indium isotopes were prepared at the GSI on-line mass separator following a fusion evaporation reaction. For the first time, a FEBIAD ion source with bunched release of indium was used. Magnetic dipole moments, electric quadrupole moments and isotope shifts were determined. The present results lead us to assign the spinI=2 to the108In (T 1/2=40 min) state. Spins and moments are discussed in the framework of thejj-coupling model.
Mass measurement of cooled neutron-deficient bismuth projectile fragments with time-resolved Schottky mass spectrometry at the FRS-ESR facility
Masses of 582 neutron-deficient nuclides ($30\leq{Z}\leq{85}$) were measured with time-resolved Schottky mass spectrometry at the FRS-ESR facility at GSI, 117 were used for calibration. The masses of 71 nuclides were obtained for the first time. A typical mass accuracy of 30 $\mu$u was achieved. These data have entered the latest atomic mass evaluation. The mass determination of about 140 additional nuclides was possible via known energies ($Q$-values) of $\alpha-$, $\beta-$, or proton decays. The obtained results are compared with the results of other measurements.
Beta decay of $^{61}$Ga
The β decay of 61Ga to its mirror nucleus 61Zn has been measured for the first time by using on-line mass separation and β-delayed gamma-ray spectroscopy. The observed decay strength to the ground state implies superallowed character in accordance with the systematics of the mirror decays in the sd and fp shell. The β feedings observed to four excited states in 61Zn are consistent with earlier spin-parity assignments based on in-beam experiments. The ground-state spin and parity for 61Ga were determined to be 3/2−.
Observation of a dramatic hindrance of the nuclear decay of isomeric states for fully ionized atoms
Abstract The half-lives of isomeric states of fully ionized 144Tb, 149Dy and 151Er have been measured. These nuclides were produced via fragmentation of about 900 MeV/u 209Bi projectiles, separated in flight with the fragment separator (FRS) and stored in the cooler ring (ESR). The decay times of the cooled fragments have been measured with time-resolved Schottky spectrometry. We observed for the first time drastic increases of the half-lives of bare isomers by factors of up to 30 compared to their neutral counterparts. This is due to the exclusion of the strong internal conversion and electron-capture channels in the radioactive decay of these bare nuclei. The experimental results are in g…
Nuclear spins, moments and charge radii of108?111Sn
The hyperfine structure splittings (hfs) and isotope shifts (IS) in the atomic transitions 5s2 5p21S0 → 5s2 5p6s1,3P1 have been measured for the radioactive isotopes108−111Sn and all stable ones. The tin isotopes were prepared as fast atomic beams for collinear laser spectroscopy at the GSI online mass separator following a fusion reaction. Nuclear spins, magnetic dipole, electric quadrupole moments and changes in mean square charge radii have been determined. In109Sn the spinI=5/2 was measured for the nuclear ground state (T1/2=18 min) in contradiction to the literature value. The mean square charge radii show a parabolic behaviour with a maximum at N=66. This is interpreted by collective …
Total absorption spectroscopy of 58Cu decay
The β decay of 58Cu has been studied by means of total absorption γ-ray spectroscopy. The β feeding to the 58Ni states has been measured, and the strength of the 58Cu(1+) →58Ni(0+) Gamow-Teller transition has been determined with improved accuracy.
Laser-stimulated two-step recombination of highly charged ions and electrons in a storage ring
Two-step resonant laser-stimulated recombination of highly charged ions was performed for the first time. Nd:YAG laser pulses overlapped with an Ar[sup 18+] beam in the electron cooler of the ESR storage ring at GSI induced transitions from the continuum to the [ital n]=81 state of hydrogenlike Ar[sup 17+]. To avoid reionization in the bending magnet before reaching the detector, the [ital n]=81 population was transferred to a state well below the reionization threshold by a Ti:sapphire laser. Tuning of this laser yielded the [ital n]=81 to 36 and 37 transition-line profiles. The two-step method provides access to detailed Rydberg spectroscopy in an electron beam environment.
Study of short-lived tin isotopes with a laser ion source
A chemically selective laser ion source based on resonance ionization of atoms in a hot cavity has been applied for the study of short-lived silver isotopes at CERN/ ISOLDE. Silver atoms were ionized by two resonant excitations and final laser ionization into the continuum. Decay properties of the neutron-rich isotopes121–127Ag were studied with a neutron long-counter and aβ-detector.
First isochronous mass spectrometry at the experimental storage ring ESR
Short-lived exotic nuclei can be produced and separated with the high-energy secondary nuclear beam facility FRS at GSI. These nuclides can be injected and stored in the storage ring ESR. The lower lifetime limit of the presently existing methods for mass measurements on these nuclides at the ESR is about a few seconds. We have developed and investigated an isochronous operational mode of the ESR, that makes mass measurements of nuclides with lifetimes down to a few ls feasible. It has been commissioned in experiments using long-lived nuclides with known masses. A mass resolving power of about 150 000 has been achieved in a "rst pilot experiment. A suitable detector system has been implemen…
Nuclear moments and the change in the mean square charge radius of neutron deficient thallium isotopes
The hyperfine structure, isotope and isomeric shifts in the atomic transition 6p 2 P 3/2−7s 2 S 1/2, λ=535 nm have been measured for theI=7 andI=2 states of190, 192, 194, 196Tl; theI=1/2 andI=9/2 states of191Tl and the I=7 isomer of188Tl. The thallium isotopes were prepared as fast atomic beams at the GSI on-line mass separator following fusion reactions and — in some cases — subsequentβ-decay. The nuclear dipole moments, electric quadrupole moments and the change in the nuclear mean square charge radius are evaluated. Theuu-isotopes show an isomeric shift which changes sign between192Tl and194Tl.
The decay of 0.57 s114Cs
Fusion reactions between58Ni projectiles and58Ni target nuclei were used to produce114Cs activity, which was studied by on-line mass separation and decay spectroscopy. The obtained half-life of 0.57±0.02 s and the probability ratio of 44±3 between betadelayed proton and beta-delayed alpha emission represent data with improved precision. The absolute branching ratios for both particle decay modes were determined to be (7 ±2)×10−2 and (1.6±0.6)×10−3, respectively. These branching ratios and the shapes of particle spectra are discussed with reference to the statistical model calculations. Groundstate alpha decay of114Cs was observed with an alpha energy of 3,226±30 keV and a branching ratio of…
Simultaneous Measurement ofβ−Decay to Bound and Continuum Electron States
We report the first measurement of a ratio {lambda}{sub {beta}{sub b}}/{lambda}{sub {beta}{sub c}} of bound-state ({lambda}{sub {beta}{sub b}}) and continuum-state ({lambda}{sub {beta}{sub c}}) {beta}{sup -}-decay rates for the case of bare {sup 207}Tl{sup 81+} ions. These ions were produced at the GSI fragment separator FRS by projectile fragmentation of a {sup 208}Pb beam. After in-flight separation with the B{rho}-{delta}E-B{rho} method, they were injected into the experimental storage-ring ESR at an energy of 400.5A MeV, stored, and electron cooled. The number of both the {sup 207}Tl{sup 81+} ions and their bound-state {beta}{sup -}-decay daughters, hydrogenlike {sup 207}Pb{sup 81+} ion…
Measurement of isotope shift and hyperfine splitting of190, 191, 193, 197Pb isotopes by collinear laser spectroscopy
We report here on the measurement of isotope shift and hyperfine splitting of190, 191, 193, 197Pb for the 723 nm atomic optical transition. Detailed analysis of the optical data has been done by combining them with the available muonic and electronicx-ray isotope shift data. The magnetic dipole moments and the electric quadrupole moments of the odd isotopes have been extracted from the hyperfine coupling constants of the atomic states involved in the optical transition used.
Nuclear moments and charge radii of107?111in determined by laser spectroscopy
Collinear fast beam laser spectroscopy has been used to measure the hyperfine structure and isotope shift in the atomic 5s 2 5p 2 P 3/2-5s 2 6s 2 S 1/2 transition (λ=451 nm) of107–111In. Secondary beams of neutron deficient indium isotopes were prepared at the GSI on-line mass separator following fusion evaporation reactions. Magnetic dipole moments and electric quadrupole moments have been determined. The isotope shifts are discussed in terms of the change of the mean square nuclear charge radii and compared with the droplet model predictions and the deformation values calculated from the quadrupole moments.
Dissociation of 8He into 6He + n + X at 240 MeV/u
4 pages, 3 figures, 2 tables.
New results with stored exotic nuclei at relativistic energies
Recently, much progress has been made with stored exotic nuclei at relativistic velocities ( v c = 0.7 ) . Fragments of 208Pb and 209Bi projectiles and fission products from 238U ions were produced, separated in flight with the fragment separator FRS, and injected into the storage-cooler ring ESR for precision measurements. 114 new masses of neutron-deficient isotopes in the lead region have been measured with time-resolved Schottky Mass Spectrometry (SMS). A new isospin dependence of the pairing energy was observed due to the improved mass accuracy of typically 1.5×10-7 (30 keV). New masses of short-lived neutron-rich fission fragments have been obtained with Isochronous Mass Spectrometry …
Study of Basic Nuclear Properties of Highly-Charged, Unstable Nuclei at the SIS-FRS-ESR Complex
Recent progress in experiments with exotic nuclear beams at the SIS-FRS-ESR facility is summarized. New results on gross properties of exotic nuclei like binding energy, half-lives, and decay modes are presented. A brief outlook to future experiments is given.
Mass mapping of a new area of neutron-deficient suburanium nuclides
Abstract The masses of 64 short-lived neutron-deficient nuclides covering the element range from tungsten to uranium have been obtained for the first time. They have been evaluated by combining directly measured masses from Schottky mass spectrometry with linked experimental Q-values in α-decay chains. Based on these new mass data we have determined the one-proton and two-proton drip-lines as well as the size of the “littoral shallow” of the sea of instability. No evidence of a Thomas–Ehrman shift has been found in the region of the investigated heavy nuclides. A peculiar behavior of two-proton separation energies has been observed in the lead region. The predictive power of various mass mo…
Study of the Unstable NucleusL10iin Stripping Reactions of the Radioactive ProjectilesB11eandL11i
Reactions of the halo systems Be-11 and Li-11 (at 460 and 280 MeV/nucleon) with a carbon target demonstrate that (n + Li-9) has an (unbound) l = 0 ground state very close to the threshold. The neutron halo of Li-11 has appreciable (1s(1/2))(2) and (0p(1/2))(2) components.
Beta decay of the new isotope101Sn
The very neutron-deficient isotope 101Sn was produced in a 50Cr(58Ni, 2p5n) reaction and its decay properties were determined for the first time. By using chemically selective ion sources of an on-line mass separator, the energy spectrum and the half-life (3 ± 1 s) of beta-delayed protons of 101Sn were measured. These results are compared to theoretical predictions.
Laser spectroscopy of neutron deficient lead and thallium isotopes: Systematics of nuclear radii in the Z = 82 region
Publisher Summary The high sensitivity achievable in laser spectroscopic methods allows the extraction of nuclear quantities even of artificially produced short-lived nuclides far off from nuclear stability. By analyzing the hyperfine structure and the isotope shift magnetic dipole moments, the electric quadrupole moments and the change of the nuclear charge radius can be studied. This chapter describes an experiment that was carried out at the GSI on-line mass separator using collinear fast atomic-beam laser spectroscopy. Radioactive lead and thallium isotopes were produced by bombarding natural tungsten targets with oxygen beams. For the lighter thallium isotopes, a tantalum target was us…
Optical spectroscopy using mass-separated beams: Nuclear properties of unstable indium and tin isotopes
Abstract Collinear fast-beam laser-spectroscopy has been used to measure the hyperfine structure and isotope shift of several indium and tin isotopes. The related experimental techniques are described, including the preparation of mass-separated beams of neutron-deficient indium and tin isotopes at the GSI on-line mass separator following fusion-evaporation reactions. The deviation of the observed dependence of the charge radii upon the neutron number from the expected behaviour is briefly discussed.
Beta-decay of 56Cu
Beta-decay studies of proton-rich isotopes near the doubly closed-shell nucleus 56Ni are of interest as (i) nuclei with a few nucleons outside a doubly-magic core are expected to represent comparatively simple configurations and thus be useful for testing nuclear shell-model predictions, and (ii) the large decay-energy window guarantees that a sizeable fraction of the strength of the allowed β-decay can be reached by the experiment. Moreover, nuclear structure properties of proton-rich N ~ Z isotopes are of astrophysical interest, e.g., concerning the EC cooling of supernovae and the astrophysical rp-process.
Experiments with stored exotic nuclei at relativistic energies
Abstract A review and recent progress are presented from experiments on masses and lifetimes of bare and few-electron exotic nuclei at GSI. Relativistic rare isotopes produced via projectile fragmentation and fission were separated in flight by the fragment separator FRS and injected into the storage ring ESR. This worldwide unique experimental method gives access to all fragments with half-lives down to the microsecond range. The great research potential is demonstrated by the discovery of new isotopes along with simultaneous mass and lifetime measurements. Single particle decay measurements and the continuous recording of both stored mother and daughter nuclei open up a new era for nuclea…
Intense beams of mass-separated, neutron-deficient indium, tin, thallium and lead isotopes
A discharge ion source of the FEBIAD-type that delivers intense beams of neutron-deficient isotopes of indium, tin, thallium and lead produced in heavy-ion-induced fusion reactions is described. After mass separation the isotopically pure beams with intensities of up to 3 × 107 ions/s were available for gamma and laser spectroscopy. This corresponds to an overall separation efficiency of about 30%.
Nuclear moments and charge radii of105, 106In
With high resolution collinear fast beam laser spectroscopy in the 451 nm-line of Indium nuclear moments and the change in the mean square radii of the nuclear charge distribution of105,106 In have been determined.
Longitudinal and transverse momentum distributions of 9Li fragments from break-up of 11Li
7 pages, 3 figures, 1 table.
Schottky mass measurements of stored and cooled neutron-deficient projectile fragments in the element range of 57≤Z≤84
Abstract A novel method for direct, high precision mass measurements of relativistic exotic nuclei has been successfully applied in the storage ring ESR at GSI. The nuclei of interest were produced by projectile fragmentation of 930 MeV / u bismuth ions, separated in-flight by the fragment separator FRS, stored and cooled in the ESR. The mass values have been deduced from the revolution frequencies of the coasting cooled ions. We have measured 104 new mass values with a precision of about 100 keV and a resolving power of 3.5×10 5 for the neutron-deficient isotopes of the elements 57≤Z≤84 . This paper presents the experimental method, the mass evaluation and a table of the experimental mass …