Asymmetric and symmetric fission of excited nuclei of Hg180,190 and Pb184,192,202 formed in the reactions with Ar36 and Ca40,48 ions

Background: Observation of asymmetric fission of $^{180}\mathrm{Hg}$ has led to intensive theoretical and experimental studies of fission of neutron-deficient nuclei in the lead region.Purpose: The study of asymmetric and symmetric fission modes of $^{180,190}\mathrm{Hg}$ and $^{184,192,202}\mathrm{Pb}$ nuclei.Methods: Mass-energy distributions of fission fragments of $^{180,190}\mathrm{Hg}$ and $^{184}\mathrm{Pb}$ formed in the $^{36}\mathrm{Ar}+^{144,154}\mathrm{Sm}$ and $^{40}\mathrm{Ca}+^{144}\mathrm{Sm}$ reactions, respectively, at energies near the Coulomb barrier have been measured using the double-arm time-of-flight spectrometer CORSET and compared with previously measured $^{192,20…

High-Statistics Sub-Barrier Coulomb Excitation of $^{106,108,110}$Sn

International audience; A Coulomb excitation campaign on $^{106,108,110}$Sn at 4.4–4.5 MeV/u was launched at the HIE-ISOLDE facility at CERN. Larger excitation cross sections and γ-ray statistics were achieved compared to previous experiments at ∼2.8 MeV/u. More precise $(B(E2;0_{1}^{ + } \to 2_{1}^{ + }))$ values, lifetimes of states via the Doppler shift attenuation method, and new $(B(E2;0_{1}^{ + } \to 2_{x}^{ + })), (B(E2;2_{1}^{ + } \to 4_{1}^{ + }))$ and $(Q(2_{1}^{ + }))$ values from the new Miniball data will be obtained and applied to test modern nuclear structure theories.

Beta-decay measurements of neutron-rich thallium, lead, and bismuth by means of resonant laser ionisation

Abstract Neutron-rich thallium, lead, and bismuth isotopes were investigated at the ISOLDE facility. After mass separation and resonant laser ionisation of the produced activity, new spectroscopic data were obtained for 215,218 Bi and 215 Pb. An attempt to reach heavy thallium had to be abandoned because of a strong francium component in the beam that gave rise to a neutron background through (α,n) reactions on the aluminium walls of the experimental chamber.

The GREAT spectrometer

Abstract The GREAT spectrometer is designed to measure the decay properties of reaction products transported to the focal plane of a recoil separator. GREAT comprises a system of silicon, germanium and gas detectors optimised for detecting the arrival of the reaction products and correlating with any subsequent radioactive decay involving the emission of protons, α particles, β particles, γ rays, X-rays or conversion electrons. GREAT can either be employed as a sensitive stand-alone device for decay measurements at the focal plane, or used to provide a selective tag for prompt conversion electrons or γ rays measured with arrays of detectors deployed at the target position. A new concept of …

Evidence for prolate structure in light Pb isotopes from in-beamγ-ray spectroscopy ofPb185

For the first time, excited states in {sup 185}Pb have been observed in in-beam {gamma}-ray spectroscopic measurements using the recoil-decay tagging method. The resulting level scheme reveals a strongly coupled yrast band structure that originates from coupling of the i{sub 13/2} quasineutron to a prolate deformed core. The band is also observed to de-excite via the spherical {alpha}-decaying 13/2{sup +}isomeric state.

Laser Spectroscopy of Neutron-Rich Hg207,208 Isotopes: Illuminating the Kink and Odd-Even Staggering in Charge Radii across the N=126 Shell Closure

The mean-square charge radii of $^{207,208}$Hg ($Z=80, N=127,128$) have been studied for the first time and those of $^{202,203,206}$Hg ($N=122,123,126$) remeasured by the application of in-source resonance-ionization laser spectroscopy at ISOLDE (CERN). The characteristic \textit{kink} in the charge radii at the $N=126$ neutron shell closure has been revealed, providing the first information on its behavior below the $Z=82$ proton shell closure. A theoretical analysis has been performed within relativistic Hartree-Bogoliubov and non-relativistic Hartree-Fock-Bogoliubov approaches, considering both the new mercury results and existing lead data. Contrary to previous interpretations, it is d…

On-line yields obtained with the ISOLDE RILIS

The ISOLDE resonance ionization laser ion source (RILIS) allows to ionize efficiently and selectively many metallic elements. In recent yield surveys and on-line experiments with the ISOLDE RILIS we observed 23–34 Mg, 26–34 Al, 98–132 Cd, 149 Tb, 155–177 Yb, 179–200 Tl, 183–215 Pb and 188–218 Bi. The obtained yields are presented together with measured release parameters which allow to extrapolate the release efficiency towards more exotic (short-lived) nuclides of the same elements. 2002 Elsevier Science B.V. All rights reserved.

In-beam spectroscopy using the JYFL gas-filled magnetic recoil separator RITU

The techniques of recoil-gating and recoil-decay tagging have been employed at Jyvaskyla to perform in-beam γ-ray and electron spectroscopy studies of heavy nuclei. The JUROSPHERE γ-ray array and the SACRED electron spectrometer have been placed at the target position of the JYFL gas-filled recoil separator recoil ion transport unit (RITU). The RITU separator has been used to collect the recoils of interest and separate them from beam particles and fission products. At the focal plane a detector system consisting of time-of-flight and implantation detectors has been used for further event identification. The method and some highlights from the results in the lead region close to the proton …

Early onset of deformation in the neutron-deficient polonium isotopes

In-source laser spectroscopy has been performed at CERN-ISOLDE with the RILIS laser ion source on Po-191-204,Po-206,Po-208-211,Po-216,Po-218. New information on the beta decay of Po-199 were extracted in the process, challenging previous results. Large-scale atomic calculations were performed to extract the changes in the mean-square charge radius delta from the isotope shifts. The delta for the even-A isotopes reveal a large deviation from the spherical droplet model for N < 116.

New developments of the in-source spectroscopy method at RILIS/ISOLDE

At the CERN ISOLDE facility, long isotope chains of many elements are produced by proton-induced reactions in target materials such as uranium carbide. The Resonance Ionization Laser Ion Source (RILIS) is an efficient and selective means of ionizing the reaction products to produce an ion beam of a chosen isotope. Coupling the RILIS with modern ion detection techniques enables highly sensitive studies of nuclear properties (spins, electromagnetic moments and charge radii) along an isotope chain, provided that the isotope shifts and hyperfine structure splitting of the atomic transitions can be resolved. At ISOLDE the campaign to measure the systematics of isotopes in the lead region (Pb, Bi…

Measurement of the first ionization potential of astatine by laser ionization spectroscopy

The radioactive element astatine exists only in trace amounts in nature. Its properties can therefore only be explored by study of the minute quantities of artificially produced isotopes or by performing theoretical calculations. One of the most important properties influencing the chemical behaviour is the energy required to remove one electron from the valence shell, referred to as the ionization potential. Here we use laser spectroscopy to probe the optical spectrum of astatine near the ionization threshold. The observed series of Rydberg states enabled the first determination of the ionization potential of the astatine atom, 9.31751(8) eV. New ab initio calculations are performed to sup…

Investigation of the Δn = 0 selection rule in Gamow-Teller transitions: The β-decay of 207Hg

5 pags., 3 figs., 1 tab. -- Open Access funded by Creative Commons Atribution Licence 4.0

In-beam andα-decay spectroscopy of191Poand evidence for triple shape coexistence at low energy in the daughter nucleus187Pb

Prompt gamma rays have been observed for the first time from the neutron-deficient nucleus Po-191 using the recoil-decay tagging technique at the RITU gas-filled separator. In addition improved alp ...

Alpha decay of the new isotopes 188,189Po

New neutron-deficient isotopes 188,189Po have been produced in the complete fusion reaction of 52Cr ions with a 142Nd target at the velocity filter SHIP. The evaporation residues were separated in-flight and subsequently identified on the basis of α-γ and α-conversion electron coincidence measurements and of α-α position and time correlations. In 189Po a ground state to ground state α decay with Eα1= 7540(20) keV, T1/2= 5(1) ms and two fine structure α-decays at Eα2= 7264(15) keV and Eα3= 7316(15) keV have been observed. In 188Po (T1/2= 400+200 −150μs) a ground state to ground state α decay at Eα= 7915(25) keV and a fine structure α decay at Eα= 7350(40) keV have been found. Improved data o…

Shape coexistence in odd-mass Au isotopes: Determination of the excitation energy of the lowest intruder state in ^{179}Au

Abstract Phenomenon of the shape coexistence has been investigated in 17979Au100. This very neutron-deficient isotope, 18 neutrons away from the stable gold isotope 19779Au118, was studied by a combination of α-decay and isomer-decay spectroscopy employing the ritu gas-filled separator and the great focal-plane spectrometer at the University of Jyvaskyla. A new isomer with t 1 / 2 = 328 ( 2 ) ns was observed and states associated with π d 3 / 2 − 1 , π s 1 / 2 − 1 , π f 7 / 2 + 1 and π h 9 / 2 + 1 structures were revealed. The implications of these results on the systematics of π h 9 / 2 + 1 and π f 7 / 2 + 1 intruder structures in the odd-mass gold isotopes are discussed. The minimum of th…

Charge radii, moments, and masses of mercury isotopes across the N=126 shell closure

Combining laser spectroscopy in a Versatile Arc Discharge and Laser Ion Source, with Penning-trap mass spectrometry at the CERN-ISOLDE facility, this work reports on mean-square charge radii of neutron-rich mercury isotopes across the $N = 126$ shell closure, the electromagnetic moments of $^{207}$Hg and more precise mass values of $^{206-208}$Hg. The odd-even staggering (OES) of the mean square charge radii and the kink at $N = 126$ are analyzed within the framework of covariant density functional theory (CDFT), with comparisons between different functionals to investigate the dependence of the results on the underlying single-particle structure. The observed features are defined predomina…

The new element 111

The new element 111 was produced and unambiguously identified in an experiment at SHIP, GSI Darmstadt. Three nuclei of the isotope272111 were observed in irradiations of209Bi targets with64Ni projectiles of 318 MeV and 320 MeV energy. The cross-sections are (1.7 −1.4 +3.3 ) pb and (3.5 −2.3 +4.6 ) pb, respectively. The nuclei decay by a emission into the new and so far the heaviest isotopes of the elements 109 and 107 with mass numbers A=268 and A=264. Theα-decay chains were followed down to the known nuclei260105 and256Lr.

Shape staggering of midshell mercury isotopes from in-source laser spectroscopy compared with density-functional-theory and Monte Carlo shell-model calculations

Neutron-deficient Hg177-185 isotopes were studied using in-source laser resonance-ionization spectroscopy at the CERN-ISOLDE radioactive ion-beam facility in an experiment combining different detection methods tailored to the studied isotopes. These include either α-decay tagging or multireflection time-of-flight gating for isotope identification. The endpoint of the odd-even nuclear shape staggering in mercury was observed directly by measuring for the first time the isotope shifts and hyperfine structures of Hg177-180. Changes in the mean-square charge radii for all mentioned isotopes, magnetic dipole, and electric quadrupole moments of the odd-A isotopes and arguments in favor of I=7/2 s…

Collectivity in the light radon nuclei measured directly via Coulomb excitation

Background: Shape coexistence in heavy nuclei poses a strong challenge to state-of-the-art nuclear models, where several competing shape minima are found close to the ground state. A classic region for investigating this phenomenon is in the region around Z=82 and the neutron midshell at N=104. Purpose: Evidence for shape coexistence has been inferred from α-decay measurements, laser spectroscopy, and in-beam measurements. While the latter allow the pattern of excited states and rotational band structures to be mapped out, a detailed understanding of shape coexistence can only come from measurements of electromagnetic matrix elements. Method: Secondary, radioactive ion beams of Rn202 and Rn…

α-decay spectroscopy of the new isotopeAt192

Decay properties of the new neutron-deficient nuclide $^{192}\mathrm{At}$ have been studied in the complete fusion reaction $^{144}\mathrm{Sm}$($^{51}\mathrm{V}$,3n)$^{192}\mathrm{At}$ at the velocity filter SHIP. Two isomeric states with half-lives of 88(6) ms and 11.5(6) ms, respectively, and with complex $\ensuremath{\alpha}$-decay schemes were identified in $^{192}\mathrm{At}$. The decay pattern of one of the isomers suggests that it is based on the oblate-deformed $\ensuremath{\pi}2{f}_{7/2}\ensuremath{\bigotimes}\ensuremath{\nu}1{i}_{13/2}$ configuration, which confirms the expected onset of deformation in the At isotopes by approaching the neutron midshell at $N=104$.

Production and decay of269110

In an experiment carried out to identify element 110, we have observed anα-decay chain, that can be unambiguously assigned to269110. In a scries of preexperiments the excitation functions of the fusion reactions50Ti +208Pb→258104* and58Fe +208Pb→266108* were measured with high precision in order to get the optimum projectile energies for the production of these heavy elements. The cross-section maxima of the 1n evaporation channels were observed at excitation energies of 15.6 MeV and 13.4 MeV, respectively. These data result in an optimum excitation energy of 12.3 MeV of the compound nucleus for the production of269110 in the reaction62Ni +208Pb→269110 + 1n. In irradiations at the correspon…

Cross section systematics for the lightest Bi and Po nuclei produced in complete fusion reactions with heavy ions

The production of the very neutron-deficient nuclides $^{184\ensuremath{-}192}\mathrm{Bi}$ and $^{186\ensuremath{-}192}\mathrm{Po}$ in the vicinity of the neutron midshell at N = 104 has been studied by using heavy-ion-induced complete fusion reactions in a series of experiments at the velocity filter SHIP. The cross sections for the xn and pxn evaporation channels of the $^{46}\mathrm{Ti}$+$^{144}\mathrm{Sm}$$\ensuremath{\rightarrow}^{190}\mathrm{Po}{}^{*},$$^{98}\mathrm{Mo}$+$^{92}\mathrm{Mo}$$\ensuremath{\rightarrow}^{190}\mathrm{Po}{}^{*},$$^{50,52}\mathrm{Cr}$+$^{142}\mathrm{Nd}$$\ensuremath{\rightarrow}^{192,194}\mathrm{Po}{}^{*}$, and $^{94,95}\mathrm{Mo}$+$^{93}\mathrm{Nb}$$\ensurem…

High-resolution γ-ray spectroscopy: a versatile tool for nuclear β-decay studies at TRIUMF-ISAC

High-resolution γ-ray spectroscopy is essential to fully exploit the unique, high-quality beams available at the next generation of radioactive ion beam facilities such as the TRIUMF isotope separator and accelerator (ISAC). The 8π spectrometer, which consists of 20 Compton-suppressed HPGe detectors, has recently been reconfigured for a vigorous research programme in weak interaction and nuclear structure physics. With the addition of a variety of ancillary detectors it has become the world's most powerful device dedicated to β-decay studies. This paper provides a brief overview of the apparatus and highlights from recent experiments.

Probing intruder structures in lead nuclei

In-beam γ-ray spectroscopy measurements provide important information on coexisting normal and intruder configurations in lead nuclei. However, in these experiments the yrast states are preferentially populated so that in many cases nothing is known about non-yrast states that are essential for obtaining a fuller understanding. Complementary experiments designed to study fine structure in the a decays of polonium nuclei have led to the discovery of low-spin non-yrast states in the daughter lead nuclei, while higher-spin states can be identified through the γ decays of isomeric states. The α-decay studies have the additional benefit of allowing information on configuration mixing in the polo…

Change in structure between the $I = 1/2$ states in $^{181}$Tl and $^{177,179}$Au

Abstract The first accurate measurements of the α-decay branching ratio and half-life of the I π = 1 / 2 + ground state in 181Tl have been made, along with the first determination of the magnetic moments and I = 1 / 2 spin assignments of the ground states in 177,179Au. The results are discussed within the complementary systematics of the reduced α-decay widths and nuclear g factors of low-lying, I π = 1 / 2 + states in the neutron-deficient lead region. The findings shed light on the unexpected hindrance of the 1 / 2 + → 1 / 2 + , 181Tl → g 177 Aug α decay, which is explained by a mixing of π 3 s 1 / 2 and π 2 d 3 / 2 configurations in 177Aug, whilst 181Tlg remains a near-pure π 3 s 1 / 2 .…

β decay of67Co

The \ensuremath{\beta}-decay properties of ${}^{67}\mathrm{Co}$ produced in proton-induced fission of ${}^{238}\mathrm{U}$ were measured by the detection of \ensuremath{\beta}-delayed \ensuremath{\gamma} rays emitted from an isotopically pure mass-separated source obtained by laser ionization. The measured half-life of 0.425(20) s is more accurate than previous values. New \ensuremath{\gamma} transitions were observed, and corresponding branching ratios and $\mathrm{log}\mathrm{ft}$ values were deduced. The ${}^{67}\mathrm{Co}$ decay scheme is discussed in terms of the single-particle shell model.

β−decay of the neutron-rich isotope215Pb

This Brief Report reports on the first observation of the β--delayed γ decay of 215Pb, feeding states in 215Bi. The 215Pb beam was produced using resonant laser ionization and mass separated at the ISOLDE-CERN on-line mass separator. This ensured clean identification of the γ rays as belonging to the decay of 215Pb or its β-decay daughters. A half-life of 147(12) s was measured for the 215Pb β decay and a level scheme for the daughter nucleus 215Bi is proposed, resulting in an extended systematics of the excited states of the neutron-rich Bi isotopes.

Identification of low-lying proton-based intruder states in189–193Pb

Low-lying proton-based intruder states have been observed in the odd-mass isotopes Pb-189,Pb-191,Pb-193 in experiments at the RITU gas-filled recoil separator. The identification has been performed ...

α -decay branching ratio of Pt180

First Accurate Normalization of the β -delayed α Decay of N16 and Implications for the C12(α,γ)O16 Astrophysical Reaction Rate

The C-12(alpha,gamma)O-16 reaction plays a central role in astrophysics, but its cross section at energies relevant for astrophysical applications is only poorly constrained by laboratory data. The reduced a width, gamma(11), of the bound 1(-) level in O-16 is particularly important to determine the cross section. The magnitude of gamma(11) is determined via sub-Coulomb a-transfer reactions or the beta-delayed a decay of N-16, but the latter approach is presently hampered by the lack of sufficiently precise data on the beta-decay branching ratios. Here we report improved branching ratios for the bound 1(-) level [b(beta,11) = (5.02 +/- 0.10) x 10(-2)] and for beta-delayed alpha emission [b(…

Shapes ofPb192,190ground states fromβ-decay studies using the total-absorption technique

The beta decay of Pb-192,Pb-190 has been studied using the total absorption technique at the ISOLDE (CERN) facility. The beta-decay strength deduced from the measurements, combined with QRPA theoretical calculations, allow us to infer that the ground states of the Pb-192,Pb-190 isotopes are spherical. These results represent the first application of the shape determination method using the total absorption technique for heavy nuclei and in a region where there is considerable interest in nuclear shapes and shape effects.

Study of exotic decay of Cs isotope close to the proton drip line

6 pags., 6 figs. -- 27th International Nuclear Physics Conference (INPC2019) 29 July - 2 August 2019, Glasgow, UK

Hindered (Δl=0) Alpha Decay and Shape Staggering in191Po

Two $\ensuremath{\alpha}$-decaying isomeric states were observed in ${}^{191}\mathrm{Po}$ with ${E}_{\ensuremath{\alpha}}\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}7334(10)\mathrm{keV}$ and $\mathrm{T}{}_{1/2}\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}22(1)\mathrm{ms}$ for ${}^{191g}\mathrm{Po}$ and $\mathrm{E}{}_{\ensuremath{\alpha}}\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}7378(10)\mathrm{keV}$ and $\mathrm{T}{}_{1/2}\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}98(8)\mathrm{ms}$ for ${}^{191m}\mathrm{Po}$. Evidence was found for fine-structure decay to excited levels in the ${}^{187}\mathrm{Pb}$ daughter nucleus. The tentative interpretation of these new lev…

Competition between Allowed and First-Forbidden β Decay: The Case of Hg208→Tl208

The β decay of ^{208}Hg into the one-proton hole, one neutron-particle _{81}^{208}Tl_{127} nucleus was investigated at CERN-ISOLDE. Shell-model calculations describe well the level scheme deduced, validating the proton-neutron interactions used, with implications for the whole of the N>126, Z<82 quadrant of neutron-rich nuclei. While both negative and positive parity states with spin 0 and 1 are expected within the Q_{β} window, only three negative parity states are populated directly in the β decay. The data provide a unique test of the competition between allowed Gamow-Teller and Fermi, and first-forbidden β decays, essential for the understanding of the nucleosynthesis of heavy nuclei in…

Spectroscopy of very neutron-deficient 187,189Bi isotopes

Shape coexistence is well known to occur in nuclei, in particular near closed shells [1], where particle-hole excitations across the shell gap can create deformed intruder states. In the neutron-deficient lead isotopes (Z = 82), deformed structures appear at low excitation energy. The isotope 188Pb [2] shows for example a triple shape coexistence with oblate and prolate excited 0+ states that compete with the spherical ground state. The study of the odd-proton single-particle excitations in Bi isotopes allows to obtain information on the orbitals involved in the different shapes observed in this mass region.

Fine structure in theαdecay ofPo188,192

The alpha decay of Po-188,Po-192 has been reexamined in order to probe the 0(+) states in the daughter nuclei Pb-184,Pb-188 that can be associated with coexisting spherical, oblate, and/or prolate ...

Identification of a 6.6μs isomeric state in Ir175

Conversion electron and beta decay spectroscopy at SHIP

Abstract Novel methods for internal conversion electron and β -decay spectroscopy at the focal plane of a recoil separator are discussed. As an example the experimental data collected at the focal plane of the velocity filter SHIP (GSI, Darmstadt) are presented and compared with the results of the GEANT Monte Carlo simulations. It is shown that the simultaneous detection of conversion electrons, γ -rays and X-rays is possible, which significantly broadens the range of applications of this and similar systems.

Shape-changing particle decays ofBi185and structure of the lightest odd-mass Bi isotopes

Proton and alpha decay of the proton-rich nuclide Bi-185 has been restudied in more detail in the complete fusion reaction Nb-93(Mo-95, 3n)Bi-185 at the velocity filter SHIP. The observed decay pat ...

Isomeric states in proton-unbound 187, 189Bi isotopes

Prompt and delayed gamma-ray spectroscopy of very neutron-deficient bismuth isotopes 187, 189Bi has been performed using the Recoil Decay Tagging (RTD) method. The isomeric i 13/2 states have been identified and their lifetimes have been measured. The systematics of these long-lived M2 isomers has been extended to the proton-unbound isotopes. The general behaviour of single-proton states is discussed within the systematics and interpreted within the shell-model framework.

De-excitation of the strongly coupled band in Au177 and implications for core intruder configurations in the light Hg isotopes

Excited states in the proton-unbound nuclide $^{177}$Au were populated in the $^92}$Mo($^{88}$Sr, p2n) reaction and identified using the Jurogam-II and GREAT spectrometers in conjunction with the RITU gas-filled separator at the University of Jyvaskyla Accelerator Laboratory. A strongly coupled band and its decay path to the 11/2−α-decaying isomer have been identified using recoil-decay tagging. Comparisons with cranked Hartree-Fock-Bogoliubov (HFB) calculations based on Skyrme energy functionals suggest that the band has a prolate deformation and is based upon coupling the odd 1h11/2 proton hole to the excited 02+ configuration in the $^{178}$Hg core. Although these configurations might be…

Electromagnetic properties of low-lying states in neutron-deficient Hg isotopes: Coulomb excitation of Hg-182, Hg-184, Hg-186 and Hg-188

The neutron-deficient mercury isotopes serve as a classical example of shape coexistence, whereby at low energy near-degenerate nuclear states characterized by different shapes appear. The electromagnetic structure of even-mass 182-188 Hg isotopes was studied using safe-energy Coulomb excitation of neutron-deficient mercury beams delivered by the REX-ISOLDE facility at CERN. The population of $ 0^{+}_{1,2}$01,2+, $ 2^{+}_{1,2}$21,2+and $ 4^{+}_{1}$41+states was observed in all nuclei under study. Reduced E2 matrix elements coupling populated yrast and non-yrast states were extracted, including their relative signs. These are a sensitive probe of shape coexistence and may be used to validate…

Identification of sub- μs isomeric states in the odd-odd nucleus Au178

The neutron-deficient gold (Z=79) isotopes in the vicinity of the neutron midshell N=104 provide prolific examples of shape coexistence and isomerism at low excitation energy. They can be probed via a number of different experimental techniques. In this study, two new isomeric states with half-lives of 294(7) and 373(9) ns have been observed in the neutron-deficient odd-odd nuclide Au178 (N=99) in an experiment at the RITU gas-filled separator at JYFL, Jyvaskyla. This result was achieved due to the use of a segmented planar germanium detector with a high efficiency at low energies. By applying the recoil-decay tagging technique, they were assigned to decay to two different long-lived α-deca…

First observation of the β-decay of neutron-rich 215Pb and 218Bi by the pulsed-release technique and resonant laser ionisation

The neutron-rich Tl, Pb and Bi isotopes are of exceptional interest to trace the evolution of single-particle levels away from the doubly magic 208Pb towards the neutron-rich side of the nuclear chart. While 208Pb is well understood in terms of the shell model, experimental data on the heavier isotopes is very scarce and it is far from clear to what extent the shell model is upheld [1]. Furthermore, large branchings ratios for β-delayed neutron emission are expected in this mass region, adding astrophysical interest to the subject [2].

In-beam γ-ray spectroscopy of 190Po: First observation of a low-lying prolate band in Po isotopes

Gamma rays from excited states of 190Po have been observed using the Jurosphere Ge-detector array coupled to the RITU gas-filled separator. They were associated with a collective band which from spin 4 onwards resembles the prolate rotational bands known in the isotones 188Pb and 186Hg. This indicates that in 190Po the prolate configuration becomes yrast above I = 2. The experimental results are interpreted in a two-band mixing calculation and are in agreement with α-decay data and potential energy surface calculations.

Charge radii and electromagnetic moments of At195–211

Hyperfine-structure parameters and isotope shifts of At195-211 have been measured for the first time at CERN-ISOLDE, using the in-source resonance-ionization spectroscopy method. The hyperfine structures of isotopes were recorded using a triad of experimental techniques for monitoring the photo-ion current. The Multi-Reflection Time-of-Flight Mass Spectrometer, in connection with a high-resolution electron multiplier, was used as an ion-counting setup for isotopes that either were affected by strong isobaric contamination or possessed a long half-life; the ISOLDE Faraday cups were used for cases with high-intensity beams; and the Windmill decay station was used for short-lived, predominantl…

Large shape staggering in neutron-deficient Bi isotopes

The changes in the mean-square charge radius (relative to 209Bi), magnetic dipole, and electric quadrupole moments of 187,188,189,191Bi were measured using the in-source resonance-ionization spectroscopy technique at ISOLDE (CERN). A large staggering in radii was found in 187,188,189Big, manifested by a sharp radius increase for the ground state of 188Bi relative to the neighboring 187,189Big. A large isomer shift was also observed for 188Bim. Both effects happen at the same neutron number, N=105, where the shape staggering and a similar isomer shift were observed in the mercury isotopes. Experimental results are reproduced by mean-field calculations where the ground or isomeric states were…

New microsecond isomers in 189, 190Bi

New microsecond isomers in the neutron-deficient isotopes 189g, 190Bi have been identified after in-flight separation by the velocity filter SHIP. The evaporation residues were identified on the basis of delayed recoil-γ/X-ray, recoil-γ/X-ray-α and excitation function measurements. The systematics of the [ π1i 13/2]13/2+ excited states in the odd-mass Bi nuclei is discussed.

Structure of191Pb from α- and β-decay spectroscopy

International audience; Complementary studies of 191 Pb have been made in the β decay of 191 Bi at LISOL (CRC) and in the α decay of 195 Po at ISOLDE (CERN). Fine structures in the α decay of the low-spin and high-spin isomers of 195 Po have been fully resolved. Identification of the parent state is made possible via isomer selection based on narrowband laser frequency scanning. The α-particle and γ-ray energies have been determined with greater precision. New α-particle and γ-ray energies are identified. Branching ratios in the decay of 195 Po and 191 Pb have been examined. Structure of 191 Pb from α- and β-decay spectroscopy 2 PACS numbers: 23.20.Nx Internal conversion, 23.60.+e α decay, …

In-source laser spectroscopy of dysprosium isotopes at the ISOLDE-RILIS

A number of radiogenically produced dysprosium isotopes have been studied by in-source laser spectroscopy at ISOLDE using the Resonance Ionization Laser Ion Source (RILIS). Isotope shifts were measured relative to $^{152}$Dy in the 4 f$^{ 10}$6s$^{2}$ $^5$I$_8$ (gs) $\rightarrow$ 4 f$^{ 10}$6s6p (8,1)$^8_o$ (418.8 nm$_{vac}$) resonance transition. The electronic factor, F, and mass shift factor, M, were extracted and used for determining the changes in mean-squared charge radii for $^{145m}$Dy and $^{147m}$Dy for the first time. A number of radiogenically produced dysprosium isotopes have been studied by in-source laser spectroscopy at ISOLDE using the Resonance Ionization Laser Ion Source (…

Excitation energy dependence of fragment-mass distributions from fission of 180,190 Hg formed in fusion reactions of 36 Ar + 144,154 Sm

Physics letters / B 748, 89 - 94 (2015). doi:10.1016/j.physletb.2015.06.068

Population of a low-spin positive-parity band from high-spin intruder states in 177Au: The two-state mixing effect

The extremely neutron-deficient isotopes 177,179Au were studied by means of in-beam ?-ray spectroscopy. Specific tagging techniques, ?-decay tagging in 177Au and isomer tagging in 179Au, were used for these studies. Feeding of positive-parity, nearly spherical states, which are associated with 2d3/2 and 3s1/2 proton-hole configurations, from the 1i13/2 proton-intruder configuration was observed in 177Au. Such a decay path has no precedent in odd-Au isotopes and it is explained by the effect of mixing of wave functions of the initial state. © 2020

Characterization of the shape-staggering effect in mercury nuclei

In rare cases, the removal of a single proton (Z) or neutron (N) from an atomic nucleus leads to a dramatic shape change. These instances are crucial for understanding the components of the nuclear interactions that drive deformation. The mercury isotopes (Z = 80) are a striking example1,2: their close neighbours, the lead isotopes (Z = 82), are spherical and steadily shrink with decreasing N. The even-mass (A = N + Z) mercury isotopes follow this trend. The odd-mass mercury isotopes 181,183,185Hg, however, exhibit noticeably larger charge radii. Due to the experimental difficulties of probing extremely neutron-deficient systems, and the computational complexity of modelling such heavy nucl…

A new pulsed release method for element selective production of neutron rich isotopes near 208Pb

Abstract A new method to reduce the isobaric contamination problem for the production of neutron rich Bi, Pb and Tl nuclei at on-line mass separators, based on the pulsed release of these radioactive species, is presented. The results of a feasibility study are reported.

Study of a-cluster states of 22Mg from resonance scattering of a post-accelerated 18Ne radioactive ion beam

An experiment aimed at the study of the α-cluster structure of 22Mg was performed at the Louvain la Neuve RIB facility. Preliminary results from a first feasibility run will be presented.