0000000000007526
AUTHOR
M. Hannawald
Frequency tripling for resonance ionization spectroscopy (RIS) of Cd
To explore the nucleosynthesis of heavy elements in the rapid neutron-capture process, investigations on short- lived, very neutron-rich Cd isotopes are planned that require pure samples. These will be produced at the CERN-ISOLDE on-line mass separator in combination with a chemically se- lective laser ion source. The excitation scheme for resonance ionization of Cd was tested in Mainz with a copper-vapor- pumped dye laser system. Due to the high ionization potential of Cd, frequency tripling was required for the first excita- tion step.1D 228: 8n m/. Laser light with an average power of 2m Wwas obtained after frequency tripling and was suc- cessfully used for RIS test measurements on cadmi…
On-line yields obtained with the ISOLDE RILIS
The ISOLDE resonance ionization laser ion source (RILIS) allows to ionize efficiently and selectively many metallic elements. In recent yield surveys and on-line experiments with the ISOLDE RILIS we observed 23–34 Mg, 26–34 Al, 98–132 Cd, 149 Tb, 155–177 Yb, 179–200 Tl, 183–215 Pb and 188–218 Bi. The obtained yields are presented together with measured release parameters which allow to extrapolate the release efficiency towards more exotic (short-lived) nuclides of the same elements. 2002 Elsevier Science B.V. All rights reserved.
β-delayed neutron decay of 104Y, 112Tc, 113Tc and 114Tc: test of half-life predictions for neutron-rich isotopes of refractory elements
Abstract Beta-decay gross properties of neutron-rich isotopes 104Y and 112,113,114Tc produced in 25 MeV proton-induced fission of 238U have been measured. Decays of 104Y with a half-life of 180±60 ms and of 114Tc with a half-life of 150±30 ms are reported for the first time. Beta-delayed neutron emission probabilities of 112,113,114Tc are determined as (1.5±0.2)%, (2.1±0.3)% and (1.3±0.4)%, respectively. Comparison of the observed Pn values with a recent theoretical calculation based on deformed quasiparticle random phase approximation (QRPA) shows good overall agreement for Tc isotopes. However, comparison of beta-decay half-lives of neutron-rich isotopes of Y to Rh with the QRPA model and…
Selective laser ionization of N≥82 indium isotopes: The new r-process nuclide 135In
Production yields and beta-decay half-lives of very neutron-rich indium isotopes were determined at CERN/ISOLDE using isobaric selectivity of a resonance-ionization laser ion-source. Beta-delayed neutron multiscaling measurements have yielded improved half-lives for 206(6)~ms $^{132}$In, 165(3)~ms $^{133}$In and 141(5)~ms $^{134}$In. With 92(10)~ms $^{135}$In, a new r-process nuclide has been identified which acts as an important `waiting-point' in the In isotopic chain for neutron densities in the range n$_n \simeq 10^{24}$--10$^{26}$ n/cm$^3$, where the r-matter flow has already passed the ${\rm A} \simeq 130$ abundance-peak region.
Nuclear physics far from stability and explosive nucleosynthesis processes
In this paper, we discuss the astrophysically relevant nuclear-physics input for a selected set of explosive nucleosynthesis scenarios leading to rapid protonand neutron-capture processes. Observables (like,e.g., luminosity curves or abundance distributions) witness the interplay between nuclear-structure aspects far from β-stability and the appropriate astrophysical environments, and can give guidance to and constraints on stellar conditions and/or key features of reaction and decay data for radioactive isotopes.
New states in heavy Cd isotopes and evidence for weakening of the N = 82 shell structure
A chemically selective laser ion source has been used in a β-decay study of heavy Ag isotopes into even-even Cd nuclides. Gamma-spectroscopic techniques in time-resolving event-by-event and multiscaling modes have permitted the identification of the first 2+ and 4+ levels in 126Cd78, 128Cd80, and tentatively the 2+ state in 130Cd82. From a comparison of these new states in 48Cd with the E(2+) and E(4+)/E(2+) level systematics of 46Pd and 52Te isotopes and several recent model predictions, possible evidence for a weakening of the spherical N = 82 neutron-shell below double-magic 132Sn is obtained.
Selective laser ionization of very neutron-rich cadmium isotopes: Decay properties of131Cd83and132Cd84
A chemically selective laser ion source has been applied in a decay study of the very neutron-rich isotopes ${}^{131}\mathrm{Cd}$ and ${}^{132}\mathrm{Cd}$ at CERN/ISOLDE. For the ${\ensuremath{\beta}}^{\ensuremath{-}}$ decay of the $N=83$ nuclide ${}^{131}\mathrm{Cd}$ a surprisingly short half-life of $(68\ifmmode\pm\else\textpm\fi{}3)$ ms and a weak delayed-neutron branch of ${P}_{n}=(3.5\ifmmode\pm\else\textpm\fi{}1.0)%$ were observed. For the $N=84$ nuclide ${}^{132}\mathrm{Cd}$ a half-life of $(97\ifmmode\pm\else\textpm\fi{}10)$ ms and a ${P}_{n}$ value of $(60\ifmmode\pm\else\textpm\fi{}15)%$ were obtained. Schematic features of both decay schemes are developed. We find that our new d…
Decay of Neutron-Rich Mn Nuclides and Deformation of Heavy Fe Isotopes
The use of chemically selective laser ionization combined with beta-delayed neutron counting at CERN/ISOLDE has permitted identification and half-life measurements for 623-ms Mn-61 up through 14-ms Mn-69. The measured half-lives are found to be significantly longer near N=40 than the values calculated with a QRPA shell model using ground-state deformations from the FRDM and ETFSI models. Gamma-ray singles and coincidence spectroscopy has been performed for Mn-64 and Mn-66 decays to levels of Fe-64 and Fe-66, revealing a significant drop in the energy of the first 2+ state in these nuclides that suggests an unanticipated increase in collectivity near N=40.
β-decay studies of135–137Snusing selective resonance laser ionization techniques
The decays of the very neutron rich Sn isotopes Sn135-137 were studied at CERN/ISOLDE using isotopic and isobaric selectivity achieved by the use of a resonance ionization laser ion source and mass spectroscopy, respectively. Neutron decay rates, gamma-ray singles, and gamma-gamma coincidence data were collected as a function of time. The half-life (T-1/2) and delayed neutron emission probability (P-n) values of 135 Sn were measured to be 530(20) ms and 21(3)%, respectively. For Sn-136, a T-1/2 of 250(30) ms was determined along with a P-n value of 30(5)%. For Sn-137, a T-1/2 of 190(60) ms and a P-n value of 58(15)% were deduced. Identification of low-energy transitions in Sb-135 was made p…