Beta Decay of 111Tc to 111Ru

The β-decay of the very neutron-rich 111Tc nucleus has been observed. A partial decay scheme of 111Ru is presented, complementing the high-spin levels earlier reported in spontaneous fission work.

Proton dripline studies at ISOLDE: 31Ar and 9C

In this contribution examples of the application of new technologies to disentangle the mechanism of $\beta$-delayed multiparticle emission are given. In particular the mechanism of $\beta$2p-emission from $^{31}$Ar has been resolved and proved to be sequential, a preview of $^{9}$C-decay data is discussed.

First decay scheme of 113Tc and identification of 113Ru m

Very neutron–rich fission products of the mass chain A=113 obtained from the IGISOL on–line mass separator have been investigated by γγ coincidence techniques and γ-spectra multiscaling. Gamma–rays following β–decay of 113Tc have been observed for the first time and a new 0.5 s isomeric state has been found in 113Ru.

Erratum to: “Mass measurements on neutron-deficient Sr and neutron-rich Sn isotopes with the ISOLTRAP mass spectrometer” [Nucl. Phys. A 763 (2005) 45]

The neutron-rich Mg isotopes: first results from MINIBALL at REX-ISOLDE

After the successful commissioning of the Radioactive beam EXperiment (REX) at ISOLDE (CERN) in 2002, first physics experiments were performed in 2003 which focussed on the neutron-rich Mg isotopes in the vicinity of the “island of inversion”. After introducing the REX facility and the modern γ spectrometer MINIBALL first preliminary results will be presented showing the high potential and physics opportunities offered by this new radioactive beam facility.

Status report of the Jyvaskyla ion guide isotope separator on-line facility

The ion guide isotope separator facility IGISOL of the University of Jyvaskyla has been moved to the new K-130 heavy ion cyclotron laboratory. The totally reconstructed facility is described in detail. The primary beams and targets, helium pumping, separator beam line construction and separator beam diagnostics are discussed. The spectroscopy stations are introduced with illustrative examples from the research program, including beta-delayed proton and neutron spectroscopy, gamma-ray spectroscopy with and without arrays, conversion electron spectroscopy, collinear laser spectroscopy and nuclear level lifetime spectroscopy.

Production of refractory elements close to the Z=N line using the ion-guide technique

Production of neutron-deficient isotopes of refractory elements in the A = 80-88 region was studied using the IGISOL technique and the 165 MeV Si-32 + Ni-nat reaction. Radioactive isotopes of Y through Mo could be produced up to the M-T = + 1 line. New information on the decay of the A = 82 and 85 nuclei, including a more detailed decay scheme and more accurate half-life for Y-82, was obtained. (C) 1998 Elsevier Science B.V. All rights reserved.

Mirror decay of 75Sr

The β-decay of 75Sr to its mirror nucleus 75Rb was studied at the ISOLDE PSB facility at CERN by means of β-delayed γ and proton spectroscopy. The decay Q-value and β-delayed γ intensity were measured for the first time. These results, 10.60±0.22 MeV and 4.5+1.9 -0.7%, together with accurate measurements of the β-decay half-life and β-delayed proton branching ratio yielded the Gamow-Teller strength 0.35±0.05 for the mirror transition. Implications of the results on studies of deformation effects and on the path of the rapid proton capture process are discussed.

First observation of β decay ofNb108toMo108

The \ensuremath{\beta}-delayed \ensuremath{\gamma} decay of $^{108}\mathrm{Nb}$ has been studied using the on-line mass-separator technique. The measured \ensuremath{\beta}-decay half-life 0.20\ifmmode\pm\else\textpm\fi{}0.03 s agrees with the previous measurement based on \ensuremath{\beta}-delayed neutron detection. The lifetime of the first ${2}^{+}$ state in $^{108}\mathrm{Mo}$ was measured to be 0.5\ifmmode\pm\else\textpm\fi{}0.3 ns, which is consistent with a deformation \ensuremath{\beta}\ensuremath{\approxeq}0.4. Spin and parity of ${2}^{+}$ are suggested for the ground state of $^{108}\mathrm{Nb}$. \textcopyright{} 1996 The American Physical Society.

Mass Measurement on the rp-Process Waiting Point 72Kr

The mass of one of the three major waiting points in the astrophysical rp process $^{72}$Kr was measured for the first time with the Penning trap mass spectrometer ISOLTRAP. The measurement yielded a relative mass uncertainty of $\deltam/m = 1.2\times 10–7 (\deltam$ = 8 keV). $^{73,74}$Kr, also needed for astrophysical calculations, were measured with more than 1 order of magnitude improved accuracy. We use the ISOLTRAP masses of $^{72–74}$Kr to reanalyze the role of $^{72}$Kr (T$_{1/2}$ = 17.2 s) in the rp process during x-ray bursts and conclude that $^{72}$Kr is a strong waiting point delaying the burst duration with at least 80\% of its $\beta$-decay half-life.

Spectroscopy at the drip line: the case of 31Ar

The beta decay of exotic nuclei is directly connected to many different and highly relevant issues. While along the years a hundred of nuclei have been identified as beta delayed proton (β-p) emitters only eight have been found to be β-2p emitters and the β-3p decay mode although energetically allowed has so far not been observed [1].

On-line yields obtained with the ISOLDE RILIS

The ISOLDE resonance ionization laser ion source (RILIS) allows to ionize efficiently and selectively many metallic elements. In recent yield surveys and on-line experiments with the ISOLDE RILIS we observed 23–34 Mg, 26–34 Al, 98–132 Cd, 149 Tb, 155–177 Yb, 179–200 Tl, 183–215 Pb and 188–218 Bi. The obtained yields are presented together with measured release parameters which allow to extrapolate the release efficiency towards more exotic (short-lived) nuclides of the same elements. 2002 Elsevier Science B.V. All rights reserved.

Gas-silicon detector telescope for charged particle spectroscopy

Abstract A gas-silicon detector telescope for charged particle spectroscopy has been constructed and tested. The lower detection limits were determined to be 155 keV for protons, 180 keV for deuterons and 350 keV for alpha particles. Typical energy resolution of the telescope measured for beta-delayed protons is 20 keV. Time resolution for the signals of the telescope was measured to be less than 10 ns. Examples of using the detector telescope in detection of beta-delayed proton activities are presented.

On-line laser spectroscopy of refractory radioisotopes at the JYFL IGISOL facility

A major objective of the laser-IGISOL program has been realized with the first ever on-line observation of collinear laser induced fluorescence from an ion of a refractory element. The measurements demonstrate that the IGISOL can be operated in a mode that produces ion beams of good emittance with reasonable extraction efficiency. The technique has been used to study the neutron-deficient Hf isotopes.

A new isomer in 125La

Levels in 125La have been studied via β+/EC decay of on-line mass-separated 125Ce using the HIGISOL technique. A new (390 ± 40) ms isomer is definitely attributed to 125La by conversion electron measurements of the 107 keV E3 isomeric transition.

β-delayed neutron decay of 104Y, 112Tc, 113Tc and 114Tc: test of half-life predictions for neutron-rich isotopes of refractory elements

Abstract Beta-decay gross properties of neutron-rich isotopes 104Y and 112,113,114Tc produced in 25 MeV proton-induced fission of 238U have been measured. Decays of 104Y with a half-life of 180±60 ms and of 114Tc with a half-life of 150±30 ms are reported for the first time. Beta-delayed neutron emission probabilities of 112,113,114Tc are determined as (1.5±0.2)%, (2.1±0.3)% and (1.3±0.4)%, respectively. Comparison of the observed Pn values with a recent theoretical calculation based on deformed quasiparticle random phase approximation (QRPA) shows good overall agreement for Tc isotopes. However, comparison of beta-decay half-lives of neutron-rich isotopes of Y to Rh with the QRPA model and…

Intruder features in the island of inversion: The case of33Mg

The Na-33 beta decay was studied online using mass separation techniques and a first description of the level structure of the neutron-rich isotope Mg-33, with N=21, has been obtained. The experiment involved the measurement of beta-gamma, beta-gamma-gamma, and beta -n-gamma coincidences as well as neutron spectra by time-of-flight technique. The first low energy level scheme for the daughter nucleus Mg-33 is given with five bound states. Spin and parity assignments are proposed according to beta feedings and gamma -ray multipolarities, beta -strength distribution is evaluated, taking into account 1n- and 2n-emission channels and it is compared with the calculated GT strength distribution. …

Beta decay of $^{61}$Ga

The β decay of 61Ga to its mirror nucleus 61Zn has been measured for the first time by using on-line mass separation and β-delayed gamma-ray spectroscopy. The observed decay strength to the ground state implies superallowed character in accordance with the systematics of the mirror decays in the sd and fp shell. The β feedings observed to four excited states in 61Zn are consistent with earlier spin-parity assignments based on in-beam experiments. The ground-state spin and parity for 61Ga were determined to be 3/2−.

Spectroscopy of34,35Sibyβdecay:sd−fpshell gap and single-particle states

Ancient bacterial genomes reveal a formerly unknown diversity ofTreponema pallidumstrains in early modern Europe

SummarySexually transmitted (venereal) syphilis marked European history with a devastating epidemic at the end of the 15thcentury, and is currently re-emerging globally. Together with non-venereal treponemal diseases, like bejel and yaws, found in subtropical and tropical regions, it poses a prevailing health threat worldwide. The origins and spread of treponemal diseases remain unresolved, including syphilis’ potential introduction into Europe from the Americas. Here, we present the first genetic data from archaeological human remains reflecting a previously unknown diversity ofTreponema pallidumin historical Europe. Our study demonstrates that a variety of strains related to both venereal…

The genetic prehistory of the Baltic Sea region

Correction: Nature communications 9 (2018), art. no. 1494 doi:10.1038/s41467-018-03872-y While the series of events that shaped the transition between foraging societies and food producers are well described for Central and Southern Europe, genetic evidence from Northern Europe surrounding the Baltic Sea is still sparse. Here, we report genome-wide DNA data from 38 ancient North Europeans ranging from similar to 9500 to 2200 years before present. Our analysis provides genetic evidence that hunter-gatherers settled Scandinavia via two routes. We reveal that the first Scandinavian farmers derive their ancestry from Anatolia 1000 years earlier than previously demonstrated. The range of Mesolit…

Decay of the neutron-rich isotope 113Ru to 113Rh

The decay of neutron-rich isotope 113Ru obtained as on-line mass separated product of proton-induced fission has been investigated by γγ coincidence and spectrum multiscaling measurements. Decay schemes for both low- and high-spin isomers of 113Ru have been constructed. The level scheme of 113Rh is considerably extended. Systematics of the lowest-lying rhodium levels is smooth. The picture of shape coexistence established for neutron-rich Rh isotopes near-neutron midshell is confirmed with the observation of a K = 1/2 deformed band, with its 3/2+ state at 600 keV being the lowest-lying level and of probable 7/2+ and 5/2+ band members. A large fraction of β feeding is found to populate high-…

Beta-delayed neutron decay of 33Na

Abstract Beta-delayed neutron decay of 33 Na has been studied using the on-line mass separator ISOLDE. The delayed neutron spectra were measured by time-of-flight technique using fast scintillators. Two main neutron groups at 800(60) and 1020(80) keV were assigned to the 33 Na decay, showing evidence for strong feeding of states at about 4 MeV in 33 Mg. By simultaneous β–γ–n counting the delayed neutron emission probabilities P 1n =47(6)% and P 2n =13(3)% were determined. The half-life value for 33 Na, T 1/2 =8.0(3) ms , was measured by three different techniques, one employing identifying gamma transitions and two employing beta and neutron counting.

A new 400 ms isomer in125Ce→125La

By using the IGISOL technique, adapted for the study of products of heavy ion induced fusion-evaporation reactions, it has been possible to identify a new isomer in the mass chainA=125.

Ancient bacterial genomes reveal a high diversity of Treponema pallidum Strains in early Modern Europe

Syphilis is a globally re-emerging disease, which has marked European history with a devastating epidemic at the end of the 15th century. Together with non-venereal treponemal diseases, like bejel and yaws, which are found today in subtropical and tropical regions, it currently poses a substantial health threat worldwide. The origins and spread of treponemal diseases remain unresolved, including syphilis’ potential introduction into Europe from the Americas. Here, we present the first genetic data from archaeological human remains reflecting a high diversity of Treponema pallidum in early modern Europe. Our study demonstrates that a variety of strains related to both venereal syphilis and y…

“Safe” Coulomb Excitation ofMg30

We report on the first radioactive beam experiment performed at the recently commissioned REX-ISOLDE facility at CERN in conjunction with the highly efficient γ spectrometer MINIBALL. Using Mg-30 ions accelerated to an energy of 2.25 MeV/u together with a thin Ni-nat target, Coulomb excitation of the first excited 2(+) states of the projectile and target nuclei well below the Coulomb barrier was observed. From the measured relative deexcitation γ-ray yields the B(E2;0(gs)(+)R 2(1)(+)) value of Mg-30 was determined to be 241(31)e(2) fm(4). Our result is lower than values obtained at projectile fragmentation facilities using the intermediate-energy Coulomb excitation method, and confirms the …

Isomer and decay studies for the rp process at IGISOL

This article reviews the decay studies of neutron-deficient nuclei within the mass region \ensuremathA=56--100 performed at the Ion-Guide Isotope Separator On-Line (IGISOL) facility in the University of Jyväskylä over last 25 years. Development from He-jet measurements to on-line mass spectrometry, and eventually to atomic mass measurements and post-trap spectroscopy at IGISOL, has yielded studies of around 100 neutron-deficient nuclei over the years. The studies form a solid foundation to astrophysical rp -process path modelling. The focus is on isomers studied either via spectroscopy or via Penning-trap mass measurements. The review is complemented with recent results on the ground and is…

Total absorption spectroscopy of 58Cu decay

The β decay of 58Cu has been studied by means of total absorption γ-ray spectroscopy. The β feeding to the 58Ni states has been measured, and the strength of the 58Cu(1+) →58Ni(0+) Gamow-Teller transition has been determined with improved accuracy.

Beta-Decay Half-Lives and Neutron-Emission Probabilities of Very Neutron-Rich Y to Tc Isotopes

Neutron-rich {sub 39}Y to {sub 43}Tc isotopes have been produced by fission of uranium with a 50MeV H{sub 2}{sup +} beam. Beta-decay half-lives, delayed neutron-emission probabilities, and production yields have been measured and compared with theory. Beta decay of 4 new isotopes is reported, and the {beta}-delayed neutron-emission mode has been discovered for 12 isotopes of the elements niobium and technetium. The results compared to quasiparticle random phase approximation predictions indicate the increasing importance of fast {beta} transitions to high-lying states of nuclei with large neutron excess. {copyright} {ital 1996 The American Physical Society.}

A step further in the A = 33−35, N ≃ 21, island of inversion: the structure of 33Mg

Experimental indications have been found in the seventies for the deformation of neutron-rich A ≃ 32 nuclei [1]. This could be explained by Hartree-Fock calculations, predicting deformed configurations in the ground state of nuclei in the A = 33−35, N ≃ 21 mass region. This exotic region, called the island of inversion [2], knows a renewed interest since it can be now experimentally accessible for detailed studies.

Ecosystem carbon response of an Arctic peatland to simulated permafrost thaw

Permafrost peatlands are biogeochemical hot spots in the Arctic as they store vast amounts of carbon. Permafrost thaw could release part of these long-term immobile carbon stocks as the greenhouse gases (GHGs) carbon dioxide (CO 2 ) and methane (CH 4 ) to the atmosphere, but how much, at which time-span and as which gaseous carbon species is still highly uncertain. Here we assess the effect of permafrost thaw on GHG dynamics under different moisture and vegetation scenarios in a permafrost peatland. A novel experimental approach using intact plant–soil systems (mesocosms) allowed us to simulate permafrost thaw under near-natural conditions. We monitored GHG flux dynamics via high-resolution…

Studying exotic nuclides close to the N = Z line at the HIGISOL facility

The ion guide [1, 2] for heavy-ion fusion-evaporation reactions (HIGISOL) which was developed by Beraud et al. [3] has been implemented at the IGISOL facility in Jyvaskyla [4]. This system was modified over the past 5 years. Figure 1 shows the present set-up. The HIGISOL takes advantage of the different angular distributions of primary beam and reaction products: the primary beam is stopped in front of the stopping chamber and the reaction products enter the stopping chamber through a thin foil passing the beam stop. This so called “shadow” method removes the plasma effect since the primary beam is not ionising the stopping gas. In order to improve ion optical properties, mainly to reduce t…

Beta-decay half-lives of $^{70}$Kr and $^{74}$Rb

Abstract Beta-decay half-lives of two nuclei close to N = Z line, 70 Kr and 74 Rb, have been measured at the ISOLDE mass-separator facility at CERN. Importance of these half-lives on two ingredients explaining existence and development of the Universe, the astrophysical nucleosynthesis and the Standard Model, are discussed.

Alignment of the ALICE Inner Tracking System with cosmic-ray tracks

ALICE (A Large Ion Collider Experiment) is the LHC (Large Hadron Collider) experiment devoted to investigating the strongly interacting matter created in nucleus-nucleus collisions at the LHC energies. The ALICE ITS, Inner Tracking System, consists of six cylindrical layers of silicon detectors with three different technologies; in the outward direction: two layers of pixel detectors, two layers each of drift, and strip detectors. The number of parameters to be determined in the spatial alignment of the 2198 sensor modules of the ITS is about 13,000. The target alignment precision is well below 10 micron in some cases (pixels). The sources of alignment information include survey measurement…

Investigation of the Li9+H2→Li8+t reaction at REX-ISOLDE

The one-neutron transfer reaction Li-9 + H-2 -> Li-8 + t has been investigated in an inverse kinematics experiment by bombarding a deuterated polypropylene target with a 2.36 MeV/u Li-9 beam from the post-accelerator REX-ISOLDE at CERN. Excitation energies in Li-8 as well as angular distributions of the tritons were obtained and spectroscopic factors deduced. (c) 2006 Elsevier B.V. All rights reserved.

First collinear laser spectroscopy measurements of radioisotopes from an IGISOL ion source

Abstract The standard Doppler-free technique of collinear laser spectroscopy has been successfully applied to radioisotopes from the ion-guide isotope separator (IGISOL) at the University of Jyvaskyla. The laser resonance fluorescence signals for the 140,142,144 Ba radioisotopes show that the ion beam energy spread is less than 6 eV, allowing the laser technique to have both high resolution and a sensitivity comparable with the best obtained at conventional facilities.

Two-pion Bose-Einstein correlations inppcollisions ats=900  GeV

We report on the measurement of two-pion correlation functions from pp collisions at root s = 900 GeV performed by the ALICE experiment at the Large Hadron Collider. Our analysis shows an increase of the Hanbury Brown-Twiss radius with increasing event multiplicity, in line with other measurements done in particle- and nuclear collisions. Conversely, the strong decrease of the radius with increasing transverse momentum, as observed at the Relativistic Heavy Ion Collider and at Tevatron, is not manifest in our data.

Measurement of the IAS resonance strength in 23Mg

Abstract Beta decay of 23 Al to excited states in 23 Mg has been studied using low-energy proton and high-energy gamma-ray detection combined with ion-guide-based on-line mass separation. For the first time, a T =3/2 isobaric analogue state, at 7801(2) keV, was observed to decay by both proton and gamma emission, with a proton branching of 0.17(8)%. The deduced resonance strength ωγ =2.2(10) meV is in agreement with upper limits reported from 22 Na(p, γ ) reaction studies. Shell-model calculations are incorporated.

Author Correction: The genetic prehistory of the Baltic Sea region.

While the series of events that shaped the transition between foraging societies and food producers are well described for Central and Southern Europe, genetic evidence from Northern Europe surrounding the Baltic Sea is still sparse. Here, we report genome-wide DNA data from 38 ancient North Europeans ranging from ~9500 to 2200 years before present. Our analysis provides genetic evidence that hunter-gatherers settled Scandinavia via two routes. We reveal that the first Scandinavian farmers derive their ancestry from Anatolia 1000 years earlier than previously demonstrated. The range of Mesolithic Western hunter-gatherers extended to the east of the Baltic Sea, where these populations persis…

Level structure of 99Nb

The β decay of 97Sr to 97Y has been investigated using ion-guide on-line mass separation and a 10 Ge-detector array to record γ−γ coincidences to a detection limit well below that of former studies. Similarities are found in the β-decay patterns of 99Zr and of its isotone 97Sr and also in the γ-ray decay rates and branchings of the corresponding levels in their respective daughters 99Nb and 97Y. This indicates a persisting influence of the d5/2 neutron shell closure for 99Nb. The level structure of 99Nb and the β-feeding pattern are discussed in the frame of the interacting boson-fermion plus broken pair model and the microscopic quasiparticle phonon model.

β-decay half-life of70Kr: A bridge nuclide for therpprocess beyondA=70

The -decay half-life of 70 Kr has been measured for the first time at the ISOLDE PSB Facility at CERN. Mass separated 70 Kr ions were produced by 1 GeV proton induced spallation reactions in a Nb foil. The measured half-life is 57(21) ms. This value is consistent with the half-life calculated assuming a pure Fermi decay, but is clearly lower than the value used in a recent rp-process reaction flow calculation. The result shows that the reaction flow via two-proton-capture of 68 Se is 2.5 times faster than previously calculated assuming an astrophysical temperature of 1.5 GK and a density of 10 6 g/cm 3 .

Accurate masses of neutron-deficient nuclides close to

Abstract Mass measurements with the Penning-trap mass spectrometer ISOLTRAP at ISOLDE/CERN are extended to nonsurface ionizable species using newly developed ion-beam bunching devices. Masses of 179–197Hg, 196,198Pb, 197Bi, 198Po and 203At were determined with an accuracy of 1×10 −7 corresponding to δm≈20  keV. Applying a resolving power of up to 3.7×10 6 ground and isomeric states of 185,187,191,193,197Hg were separated. First experimental values for the isomeric excitation energy of 187,191Hg are obtained. A least-squares adjustment has been performed and theoretical approaches are discussed to model the observed fine structure in the binding energy.

The Genetic History of Northern Europe

Recent ancient DNA studies have revealed that the genetic history of modern Europeans was shaped by a series of migration and admixture events between deeply diverged groups. While these events are well described in Central and Southern Europe, genetic evidence from Northern Europe surrounding the Baltic Sea is still sparse. Here we report genome-wide DNA data from 24 ancient North Europeans ranging from ~7,500 to 200 calBCE spanning the transition from a hunter-gatherer to an agricultural lifestyle, as well as the adoption of bronze metallurgy. We show that Scandinavia was settled after the retreat of the glacial ice sheets from a southern and a northern route, and that the first Scandinav…

The β2p decay mechanism of Ar

We have measured the beta-decay of Ar-31 with a high granularity setup sensitive to multiparticle decay branches. Two-proton emission is observed from the isobaric analog state in Cl-31 to the four lowest states in P-29 and furthermore from a large number of states fed in Gamow-Teller transitions. The mechanism of two-proton emission is studied via energy and angular correlations between the two protons. In all cases the mechanism is found to be sequential yielding information about states in S-30 up to 8 MeV excitation energy. Improved data on the beta-delayed one-proton branches together with the two-proton data provide precise information about the beta-strength distribution up to 15 MeV…

Midrapidity Antiproton-to-Proton Ratio inppCollisons ats=0.9and 7 TeV Measured by the ALICE Experiment

The ratio of the yields of antiprotons to protons in pp collisions has been measured by the ALICE experiment at root s = 0.9 and 7 TeV during the initial running periods of the Large Hadron Collider. The measurement covers the transverse momentum interval 0.45 < p(t) < 1.05 GeV/c and rapidity vertical bar y vertical bar < 0.5. The ratio is measured to be R-vertical bar y vertical bar<0.5 = 0.957 +/- 0.006(stat) +/- 0.0014(syst) at 0.9 Tev and R-vertical bar y vertical bar<0.5 = 0.991 +/- 0.005 +/- 0.014(syst) at 7 TeV and it is independent of both rapidity and transverse momentum. The results are consistent with the conventional model of baryon-number transport and set stringent limits on a…

Status of REX-ISOLDE

REX-ISOLDE [1] is a post-accelerator situated at the ISOLDE radioactive ion beam facility placed at CERN, Geneva. It’s main aim is to increase the energy of light (A < 50) radioactive ions from 60 keV to 0.8–2.2MeV/u. REX—ISOLDE uses a new concept of post-acceleration of radioactive ion beams by using charge breeding of the ions in a high charge state ion source and the efficient acceleration of the highly charged ions in a short LINAC using modern ion accelerator structures. In a first step the radioactive ions are captured in a large gas-filled Penning trap. The task is to accumulate, cool and bunch the beam and prepare it for the injection into an electron beam ion source (EBIS). Cooling…

Determination of the spin of 31Ar

Abstract The beta-delayed proton emission from the lightest Ar-isotopes has been recorded with a high-granularity, large solid-angle Si-detector set-up. Proton energy shifts due to beta-recoil have been measured. We demonstrate how this allows the spin of 31 Ar to be determined as 5/2. The method can be applied at decay rates as low as 1 s −1 .

New interpretation of shape coexistence in99Zr

Levels in ${}^{99}\mathrm{Zr}$ populated by $\ensuremath{\beta}$ decay of on-line mass separated ${}^{99}$Y have been studied by $\ensuremath{\gamma}$-ray spectroscopic methods, including $\ensuremath{\gamma}$-$\ensuremath{\gamma}$ coincidences recorded with an array of ten Ge detectors and level-lifetime measurements. The formerly reported strongly collective character of the 53-keV transition turns out to be questionable. This implies a revision of the experimental evidence for shape coexistence in ${}^{99}\mathrm{Zr}.$ Transition rates and $\ensuremath{\gamma}$-ray branching ratios make a new level at 679 keV with ${t}_{1/2}=9$ ns another candidate for a deformed state.

$\beta$ - decay of the M$_{T}$=-1 nucleus $^{58}$Zn studied by selective laser ionization

$\beta$ - decay of $^{58}$Zn has been studied for the first time. A new laser ion-source concept has been used to produce mass-separated sources for $\beta$ and $\gamma$ - spectroscopy. The half-life of $^{58}$Zn was determined to be 86(18) ms. Comparisons are made with previous data from charge-exchange reactions. Our Gamow-Teller strength to the 1$^{+}$ state at 1051 keV excitation in $^{58}$Cu agrees well with the value extracted from a recent ($^{3}$He, t) study. Extensive shell-model calculations are presented.

Coulomb Excitation ofCu68,70: First Use of Postaccelerated Isomeric Beams

We report on the first low-energy Coulomb excitation measurements with radioactive Ipi=6- beams of odd-odd nuclei 68,70Cu. The beams were produced at ISOLDE, CERN and were post-accelerated by REX-ISOLDE to 2.83 MeV/nucleon. gamma rays were detected with the MINIBALL spectrometer. The 6- beam was used to study the multiplet of states (3-, 4-, 5-, 6-) arising from the pi2p3/2nu1g9/2 configuration. The 4- state of the multiplet was populated via Coulomb excitation and the B(E2;6--->4-) value was determined in both nuclei. The results obtained illustrate the fragile stability of the Z=28 shell and N=40 subshell closures. A comparison with large-scale shell-model calculations using the 56Ni core…

High-resolution studies of beta-delayed proton emitters at IGISOL facility

Beta-decays of23Al and41Ti have been studied by applying ion guide techniques, gamma detection and a gas-Si telescope for charged-particle detection. The experimental beta-decay strength of41Ti was found to be quenched by a factor ofq2 = 0.64 compared to our shell model calculations below 8 MeV excitation energy in41Sc. This result is in line with the generally accepted value ofq = 0.77. The isobaric analogue state of the41Ti ground state was measured to contain 10(8)% isospin impurity. This relatively high value could be well reproduced by the shell model calculation in thesdfp space. Gamma-decay of theT = 3/2 isobaric analogue state in23Mg was observed together with its decay by proton em…

Independent yields of neutron-rich nuclei in charged-particle induced fission

Abstract Yields of fission products have been studied at the recently upgraded IGISOL facility in Jyvaskyla using 50 MeV H2+ beam (Ep = 25 MeV) and thin natTh and natU targets. The independent yields of fission products in the mass regions A = 99−112 (elements Y, Nb and Tc) and A = 127−134 (elements Sn, Sb and Te) have been obtained. Comparisons of the experimental isotopic distributions with theoretical ones are presented. Enhancement of the production rate of the doubly magic 132Sn is observed in the experimental yield curve.

Spectroscopy with β2p and β-ν recoil shifts

9 pages, 4 figures.-- Printed version published Apr 22, 2002.

Beta-decay strength and isospin mixing studies in the sd and fp-shells

We have studied beta decays of MT<0 nuclei in sd and fp shells. The decay of 41Ti shows a large, 10(8) %, isospin mixing of IAS and the Gamow-Teller strength is observed to be quenched by a factor of q2=0.64. These results can be reproduced qualitatively in our shell model calculations. We have observed for the first time proton and gamma decay of the isobaric analogue state in 23Mg. Our results on the isospin mixing of the isobaric analogue state agrees well with the shell model calculations. The obtained proton branch of the IAS is used to extract the transition strength for the reaction 22Na(p,γ)23Mg.

Decays of theY97isomers to the single neutron nucleusZr97

The decays of the 9/2(+) and of the three-quasiparticle high spin isomer in Y-97 have been investigated following on-line mass separation with the ion-guide technique. Spins and parities for several of the lowest-lying levels in the daughter nucleus Zr-97 are revised and configurations are proposed. In particular, the 2264 keV level is identified as the h(11/2) single-neutron level. The population of a cascade on top of the h(11/2) level provides evidence for Gamow-Teller beta decay of the high-spin Y-97 isomer. Levels and transition rates are qualitatively well reproduced by regarding Zr-97 as a single-neutron nucleus with respect to the doubly closed Zr-96 core.

Stones, Bones, and Hillfort: Radiocarbon Dating of Ķivutkalns Bronze-Working Center

The Bronze Age site of ķivutkalns with its massive amount of archaeological artifacts and human remains is considered the largest bronze-working center in Latvia. The site is a unique combination of cemetery and hillfort believed to be built on top of each other. This work presents new radiocarbon dates on human and animal bone collagen that somewhat challenge this interpretation. Based on analyses using a Bayesian modeling framework, the present data suggest overlapping calendar year distributions for the contexts within the 1st millennium BC. The carbon and nitrogen isotopic ratios indicate mainly terrestrial dietary habits of studied individuals and nuclear family remains buried in one o…

Accelerated radioactive beams from REX-ISOLDE

In 2001 the linear accelerator of the Radioactive beam EXperiment (REX-ISOLDE) delivered for the first time accelerated radioactive ion beams, at a beam energy of 2 MeV/u. REX-ISOLDE uses the method of charge-state breeding, in order to enhance the charge state of the ions before injection into the LINAC. Radioactive singly-charged ions from the on-line mass separator ISOLDE are first accumulated in a Penning trap, then charge bred to an A/q < 4.5 in an electron beam ion source (EBIS) and finally accelerated in a LINAC from 5 keV/u to energies between 0.8 and 2.2 MeV/u. Dedicated measurements with REXTRAP, the transfer line and the EBIS have been carried out in conjunction with the first co…

High-resolution study of the beta decay of 41Ti

Abstract An improved high-resolution study of the beta decay of 41 Ti, produced in the 40 Ca( 3 He, 2n) reaction at 40 MeV, has been performed at the Ion Guide Isotope Separator On-Line (IGISOL) facility. The beta-delayed radiation was detected by a low-energy charged-particle detector and a large Ge detector for gamma rays. The experimental beta-decay strength and its distribution, extracted from delayed-proton data, are compared with results of shell-model calculations in the sdfp space. The lowest J π = 3 2 + , T = 3 2 state in 41 Sc, the isobaric analogue state of the 41 Ti ground state, is estimated to contain 10% isospin impurity.

Improved ion guide for heavy-ion fusion-evaporation reactions

The ion guide for heavy-ion-induced reactions developed originally for the SARA facility in Grenoble has been implemented at the Jyvaskyla IGISOL facility. For the Cd-116(Ar-40, 6n)Dy-150 reaction an efficiency of 0.5% relative to the number of reaction products entering the stopping chamber was obtained. This is 3.5 times higher than previously obtained at SARA and corresponds to a yield of about 100 ions/(p mu C mb). Mass-separated yields for the Ar-36 + Mo-92 and Ar-36 + Mo-94 reactions were measured. (C) 1998 Elsevier Science B.V. All rights reserved.

First observation of nonyrast levels inZr103and level systematics ofN= 63 Sr, Zr, and Mo isotones

The {beta} decay of the very-neutron-rich nucleus {sup 103}Y has been studied at the isotope separator IGISOL, allowing for the first time the observation of nonyrast levels in its daughter {sub 40}{sup 103}Zr{sub 63}. The level structure is similar to that of its isotones {sup 101}Sr and {sup 105}Mo, suggesting a large ground-state deformation of {beta}{approx_equal} 0.4. Level systematics allows for new level assignments in both {sup 103}Zr and {sup 105}Mo. {copyright} {ital 1996 The American Physical Society.}

Accurate mass measurements on neutron-deficient krypton isotopes

soumis à Nuclear Physics A; The masses of $^{72-78,80,82,86}$Kr were measured directly with the ISOLTRAP Penning trap mass spectrometer at ISOLDE/CERN. For all these nuclides, the measurements yielded mass uncertainties below 10 keV. The ISOLTRAP mass values for $^{72-75}$Kr outweighed previous results obtained by means of other techniques, and thus completely determine the new values in the Atomic-Mass Evaluation. Besides the interest of these masses for nuclear astrophysics, nuclear structure studies, and Standard Model tests, these results constitute a valuable and accurate input to improve mass models. In this paper, we present the mass measurements and discuss the mass evaluation for t…

Isomeric state of 80Y and its role in the rp-process

The HIGISOL facility has been used to investigate carefully the isomeric transition 228.5 keV in 80Y. We have measured the electron internal conversion coefficient for this transition αK = 0.50 ± 0.07 which gives the value for half-life of “bare” isomeric state T 1/2 = 6.8 ± 0.5 s. The isomeric state should play an important role in the rp-process calculations.

Two-proton decay of the isobaric analogue state of Ar-31

8 pages, 1 table, 4 figures.-- Journal issue title: "Nucleus-Nucleus Collisions".

First measurement of radioisotopes by collinear laser spectroscopy at an ion-guide separator

The first successful application of an ion-guide separator (IGISOL) for collinear laser spectroscopy of radioisotopes has achieved an efficiency comparable with the best obtained with catcher-ionizer facilities. The ion beam energy spread was determined to be less than 6 eV, allowing laser fluorescence resonance signals for the Ba-140,Ba-142,Ba-144 radioisotopes to be detected with high resolution and sensitivity. Applications of this technique to measuring nuclear properties of refractory elements and short lived isomers promises to be particularly advantageous.

First Precision Mass Measurements of Refractory Fission Fragments

Atomic masses of 95-100Sr, 98-105Zr, and [corrected] 102-110Mo and have been measured with a precision of 10 keV employing a Penning trap setup at the IGISOL facility. Masses of 104,105Zr and 109,110Mo are measured for the first time. Our improved results indicate significant deviations from the previously published values deduced from beta end point measurements. The most neutron-rich studied isotopes are found to be significantly less bound (1 MeV) compared to the 2003 atomic mass evaluation. A strong correlation between nuclear deformation and the binding energy is observed in the two-neutron separation energy in all studied isotope chains.

Study of the neutron-rich nuclei with $N$ = 21, $^{35}$Si and $^{33}$Mg, by beta decay of $^{35}$Al and $^{33}$Na

Abstract The first information on the level structure of the N =21 nuclei, 35 Si and 33 Mg, has been obtained by the beta decay study of 35 Al and 33 Na, produced by fragmentation of an UC target with 1.4 GeV protons at CERN/ISOLDE. The experimental technique involved β – γ , β – γ – γ , and β –n– γ coincidences, neutron spectra being obtained by time of flight measurements. Gamma detection was made either using large Ge counters or small BaF 2 scintillators (for lifetime measurements). In the case of the 35 Al decay, ( T 1/2 =41.6(2.2) ms), a simple structure has been found for the level scheme of 35 Si ( Z =14, N =21) which has been interpreted with the level sequence : 7/2 − , 3/2 − and …

Beta-decay of 56Cu

Beta-decay studies of proton-rich isotopes near the doubly closed-shell nucleus 56Ni are of interest as (i) nuclei with a few nucleons outside a doubly-magic core are expected to represent comparatively simple configurations and thus be useful for testing nuclear shell-model predictions, and (ii) the large decay-energy window guarantees that a sizeable fraction of the strength of the allowed β-decay can be reached by the experiment. Moreover, nuclear structure properties of proton-rich N ~ Z isotopes are of astrophysical interest, e.g., concerning the EC cooling of supernovae and the astrophysical rp-process.

Beta decay of very neutron-rich110Mo studied at the new IGISOL facility

The decay of the new activity110Mo (t1/2=0.30(4).s) has been observed at the new IGISOL separator. Multiscaled singles,β-γ-t and γ-y-t coincidences were recorded. The decay scheme suggests Iπ=2+ for the ground state of the daughter nucleus110Tc. Three 1+ levels are fed with logft values below 5, indicating no drastic change among Mo and Ru decays at the middle of the neutron shell. This experiment confirms the expectation that the new IGISOL facility will allow the identification of one or two new more neutron-rich isotopes per element in this region.

Mass measurements on unstable Sn and Sr isotopes with the ISOLTRAP mass spectrometer

Direct mass measurements have been performed on the isotopes 76,77,80,81Sr and 129,130,131,132Sn by means of the Penning trap mass spectrometer ISOLTRAP at ISOLDE/CERN. In the case of 76Sr the mass was measured for the first time and an accuracy of about 30 keV was reached (Fig. 1). The masses of the tin isotopes are known for a long time from Q β measurements.

Ground-state spin of 59Mn

Beta decay of $^{59}$Mn has been studied at PSB-ISOLDE, CERN. The intense and pure Mn beam was produced using the Resonance Ionization Laser Ion Source (RILIS). Based on the measured $\beta$-decay rates the ground-state spin and parity are proposed to be $J^{\pi}$ = 5/2$^{-}$. This result is consistent with the systematic trend of the odd-A Mn nuclei and extends the systematics one step further towards the neutron drip line.

Optimization of krypton yields for rp-process studies at ISOLDE(CERN)

The production of neutron-deficient krypton isotopes having astrophysical importance has been studied at the ISOLDE PBS facility at CERN. To investigate several effects on the yield a Monte Carlo code has been extensively applied.

Superasymmetric fission at intermediate energy and production of neutron-rich nuclei with A &lt; 80

Abstract The yields of neutron-rich Ni, Cu, Zn, Ga and Ge-isotopes were measured in 25 MeV proton induced fission of 238 U using the ion guide-based isotope separator technique. The results indicate enhancement for superasymmetric mass division at intermediate excitation energy of the fissioning nucleus and show the potential of this reaction for the production of neutron-rich exotic nuclei around Z = 28.

Non-analog β decay of 74Rb

The magnitude of the Coulomb mixing parameter δ 1 has been experimentally deduced, for the first time, for the β decay of 74 Rb. The estimated magnitude is derived from the feeding of the non-analog first excited 0 + state in 74 Kr. The inferred upper limit of 0.07% is small compared to theoretical predictions. The half-life was measured to be 64.90(9) ms.  2001 Published by Elsevier Science B.V.

A thirty second isomer in Hf

An isomer has been detected in Hf-171 with a half-life of T-1/2 = 29.5(9) s. The state was populated in the Yb-170(alpha,3n)Hf-171m reaction at a beam energy of E-alpha = 50 MeV in an on-line ion guide isotope separator. The isomeric Hf-17lm(+) beam was extracted from the ion guide, mass-analysed and implanted in the surface of a microchannel-plate. The half-life of the collected activity was measured from the decay of the microchannel-plate count rate. We associate the isomer with the first excited slate in Hf-171 with spin 1/2(-) at an excitation energy of 22(2) keV.

Isomeric state of $^{80}$Y and its role in the astrophysical rp-process

5 pages, 7 figures.-- PACS nrs: 21.10.Tg; 23.20.Nx; 27.50.+e.

Mass Measurement on therp-Process Waiting PointKr72

With the aim of improving nucleosynthesis calculations, we performed for the first time, a direct high-precision mass measurement on the waiting point in the astrophysical rp-process 72Kr. We used the ISOLTRAP Penning trap mass spectrometer located at ISOLDE/CERN. The measurement yielded a relative mass uncertainty of δm/m = 1.2×10-7. In addition, the masses of 73Kr and 74Kr were measured directly with relative mass uncertainties of 1.0×10-7 and 3×10-8, respectively. We analyzed the role of 72Kr in the rp-process during X-ray bursts using the ISOLTRAP and previous mass values of 72-74Kr.

Low energy reactions with radioactive ions at REX-ISOLDE-the 9Li + 2H case

19 pages, 12 figures, 2 tables.-- PACS nrs.: 25.60.-t; 25.45.-z; 27.20.+n.-- et al. ISOLDE Collaborattion and REX-ISOLDE Collaboration.