0000000000010669
AUTHOR
H. Stolzenberg
High-accuracy mass determination of unstable cesium and barium isotopes
Direct mass measurements of short-lived Cs and Ba isotopes have been performed with the tandem Penning trap mass spectrometer ISOLTRAP installed at the on-line isotope separator ISOLDE at CERN. Typically, a mass resolving power of 600 000 and an accuracy of $\delta \mbox{m} \approx 13$ keV have been obtained. The masses of $^{123,124,126}$Ba and $^{122m}$Cs were measured for the first time. A least-squares adjustment has been performed and the experimental masses are compared with theoretical ones, particularly in the frame of a macroscopic-microscopic model.
The Inchworm as a precision translator in a high magnetic field and UHV environment
Abstract A new set-up has been designed and tested for on-line, high-precision mass measurements of short-lived radioactive isotopes via a determination of the ion cyclotron resonance. Ions delivered by the on-line isotope separator ISOLDE at CERN/Geneva are stored in a Penning trap installed in a superconducting solenoid. Due to severe space limitations in the bore of the solenoid, it is impossible to use conventional mechanical feedthroughs for the necessary manipulations inside the uhv chamber. Instead, a number of Inchworms, a high-precision positioning device based on the piezo-electric effect are employed. This publication reports on the first application of this device in a uhv envir…
Ramsey technique applied in a Penning trap mass spectrometer
Abstract The Ramsey method has been applied in an experiment aiming for accurate mass determination of unstable isotopes. The ion motion in a Penning trap has been excited with time-separated oscillatory fields and Ramsey fringes were observed in the case of dipole and quadrupole excitation. The experimental resonances are in good agreement with theory. Further applications of the technique are discussed.
Mass measurements of very high accuracy by time-of-flight ion cyclotron resonance of ions injected into a penning trap
Abstract The possibility of absolute mass measurements using time-of-flight detection of ion cyclotron resonance on ions injected into a Penning trap has been demonstrated. Resolving powers of 2 million have been achieved, with accuracies of about 0.5 ppm. Absolute accuracy is obtained by direct observation of the sum frequency of the cyclotron and the magnetron motions through the use of an azimuthal quadrupole r.f. field to transform initial magnetron motion into cyclotron motion. Imperfections of the Penning trap leading to systematic errors are discussed. The system has been designed specifically to measure the masses of radionuclides produced at the on-line isotope separator ISOLDE. Wi…
First absolute mass measurements of short-lived isotopes
Absolute mass measurements of short-lived isotopes have been performed at the on-line mass separator ISOLDE at CERN by determining the cyclotron frequencies of ions confined in a Penning trap. The cyclotron frequencies for77,78,85,86,88Rb and88Sr ions could be determined with a resolving power of 3×105 and an accuracy of better than 10−6, which corresponds to 100 keV for massA=100. The shortest-lived isotope under investigation was77Rb with a half-life of 3.7 min. The resonances obtained for the isobars88Rb and88Sr were clearly resolved.
Highly-charged ions in a penning trap: mass measurements, etc.
The use of a Penning trap will start a new generation of precision experiments on highly charged ions. The long storage time of the ions in combination with a controlled confinement in a very small volume will enable accuracies in mass determination better than δm/m = 10-8.
Penning-trap mass measurements of neutron-deficient Rb and Sr isotopes
Abstract The Penning-trap mass spectrometer ISOLTRAP installed at the on-line mass separator ISOLDE 2 at CERN has been used for mass determination of 75–87 Rb and 78–83,87 Sr. Ions are captured in a Penning trap and their cyclotron frequency ω c = ( q m )B in the trapping field B is measured. Ratios of these frequencies lead to the determination of the atomic mass of these isotopes. A resolving power of typically m Δm = 10 6 and an accuracy of δm ≈10 keV is obtained. The mass of 78 Sr is measured for the first time and, in most cases, the mass values of the other isotopes are significantly improved. The experimental masses are compared with theoretical predictions.
High-Accuracy Mass Determination of Unstable Rb, Sr, Cs, Ba, Fr and Ra Isotopes with a Penning Trap Mass Spectrometer
The majority of masses of radioactive isotopes has been measured by determination of Q-values in nuclear reactions or in nuclear decay. For a long time the use of direct mass determination has been limited to stable isotopes or isotopes close to stability. This changed in the 70’s with magnetic spectrometers put on-line to isotope separators. The Orsay group (Audi et al., 1986) succeeded in measuring the masses in long isotope chains of alkali elements. They impressively demonstrated the possibilities embedded in direct mass determination of isotopes far from stability. The persisting demand for more precise masses of short-lived isotopes (or exotic particles) has prompted during recent yea…
Mass Determination of Francium and Radium Isotopes by a Penning Trap Mass Spectrometer
Abstract A tandem Penning trap mass spectrometer is used for mass measurement of radioactive isotopes produced at the on-line isotope separator ISOLDE/CERN. The mass is determined directly and with high accuracy by measuring the cyclotron frequency of the stored ions. Measurements were performed on 209 210 211 212 221 222Fr and 226 230Ra. A resolving power of 5 × 105 was used and an accuracy of 1·8 × 10−7 has been achieved.
Accurate mass determination of short-lived isotopes by a tandem Penning-trap mass spectrometer
A mass spectrometer consisting of two Penning traps has been set up for short-lived isotopes at the on-line mass separator ISOLDE at CERN. The ion beam is collected and cooled in the first trap. After delivery to the second trap, high-accuracy direct mass measurements are made by determining the cyclotron frequency of the stored ions. Measurements have been performed for $^{118}--^{137}$Cs. A resolving power of over ${10}^{6}$ and an accuracy of 1.4\ifmmode\times\else\texttimes\fi{}${10}^{\mathrm{\ensuremath{-}}7}$ have been achieved, corresponding to about 20 keV.
Resolution of nuclear ground and isomeric states by a Penning trap mass spectrometer.
Ground and isomeric states of a nucleus have been resolved for the first time by mass spectrometry. Measurements on $^{78}\mathrm{Rb}^{\mathit{m},}$g and $^{84}\mathrm{Rb}^{\mathit{m},}$g were performed using a tandem Penning trap mass spectrometer on-line with the isotope separator ISOLDE/CERN. The effects of ion-ion interaction were investigated for two ion species differing in mass and stored simultaneously in the trap.