0000000000011190

AUTHOR

P. Delahaye

Towards high-accuracy mass spectrometry of highly charged short-lived ions at ISOLTRAP

Dedicated to H.-J. Kluge on the occasion of his 65th birthday anniversary - Jürgen Kluge Special Issue; Multiply charged ions of stable xenon isotopes from a plasma ion source have been mass-selected by the on-line mass separator ISOLDE/CERN and delivered to the triple-trap mass spectrometer ISOLTRAP. The doubly charged ions that survived the charge-exchange processes during bunching and ion preparation were transferred to a precision Penning trap for mass determination. Mass values were obtained for the isotopes with mass numbers A=126,129,130,136. They are consistent with previous results except for the case of $^{126}Xe$ where a significant deviation from the literature value was found. …

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Diagnostics of a charge breeder electron cyclotron resonance ion source helium plasma with the injection ofNa231+ions

This work describes the utilization of an injected 23Na1+ ion beam as a diagnostics of the helium plasma of a charge breeder electron cyclotron resonance ion source. The obtained data allows estimating the upper limit for the ion-ion collision mean-free path of the incident sodium ions, the lower limit of ion-ion collision frequencies for all charge states of the sodium ions and the lower limit of the helium plasma density. The ion-ion collision frequencies of high charge state ions are shown to be at least on the order of 1–10 MHz and the plasma density is estimated to be on the order of 1011  cm−3 or higher. The experimental results are compared to simulations of the 23Na1+ capture into t…

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Cadmium mass measurements between the neutron shell closures at N=50 and 82

International audience; The mass values of the neutron-deficient cadmium isotopes 99−109Cd and of the neutronrich isotopes 114,120,122−124,126,128Cd have been measured using ISOLTRAP. The behavior of the separation energies of the cadmium isotopes from N = 50 to 82 is discussed.

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"Safe" Coulomb excitation of 30Mg.

We report on the first radioactive beam experiment performed at the recently commissioned REX-ISOLDE facility at CERN in conjunction with the highly efficient $\gamma$ -spectrometer MINIBALL. Using $^{30}$Mg ions accelerated to an energy of 2.25MeV/u together with a thin $^{nat}$Ni target, Coulomb excitation of the first excited 2+ states of the projectile and target nuclei well below the Coulomb barrier was observed. From the measured relative de-excitation $\gamma$ -ray yields the B(E2; 0$^{+}_{gs} \rightarrow 2^{+}_{1}$) value of $^{30}$Mg was determined to be 241(31)$e^{2}$fm$^{4}$. Our result is lower than values obtained at projectile fragmenttion facilities using the intermediate-ene…

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Charge breeding at GANIL: Improvements, results, and comparison with the other facilities

International audience; The 1+/n+ method, based on an ECRIS charge breeder (CB) originally developed at the LPSC laboratory, is now implemented at GANIL for the production of Radioactive Ion Beams (RIBs). Prior to its installation in the middle of the low energy beam line of the SPIRAL1 facility, the 1+/n+ system CB has been modified based on the experiments performed on the CARIBU Facility at Argone National Laboratory. Later, it has been tested at the 1+/n+ LPSC test bench to validate its operation performances. Charge breeding efficiencies as well as charge breeding times have been measured for noble gases and alkali elements. The commissioning phase started at GANIL in the second half-y…

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The neutron-rich Mg isotopes: first results from MINIBALL at REX-ISOLDE

After the successful commissioning of the Radioactive beam EXperiment (REX) at ISOLDE (CERN) in 2002, first physics experiments were performed in 2003 which focussed on the neutron-rich Mg isotopes in the vicinity of the “island of inversion”. After introducing the REX facility and the modern γ spectrometer MINIBALL first preliminary results will be presented showing the high potential and physics opportunities offered by this new radioactive beam facility.

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Direct determination of the excitation energy of the quasistable isomer 180mTa

180mTa is a naturally abundant quasistable nuclide and the longest-lived nuclear isomer known to date. It is of interest, among others, for the search for dark matter, for the development of a γ laser, and for astrophysics. So far, its excitation energy has not been measured directly but has been based on an evaluation of available nuclear reaction data. We have determined the excitation energy of this isomer with high accuracy using the Penning-trap mass spectrometer JYFLTRAP. The determined mass difference between the ground and isomeric states of 180Ta yields an excitation energy of 76.79(55) keV for 180mTa. This is the first direct measurement of the excitation energy and provides a bet…

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Experimental activities with the LPSC charge breeder in the European context

WEOBMH01; International audience; One of the Work Packages of the "Enhanced Multi-Ionization of short-Lived Isotopes at EURISOL"NuPNET project focuses on the ECR charge breeding.The LPSC charge breeder is used for experimental studiesin order to better understand the fundamental processesinvolved in the 1+ beam capture by a 14 GHz ECRplasma. Some improvements, like symmetrisation of themagnetic field at the injection side and higher pumpingspeed, have been carried out on the PHOENIX chargebreeder. The impact of these modifications on theefficiencies and charge breeding times are presented. Inthe same time, the new LPSC 1+ source developmentsperformed in order to ease the efficiency measurem…

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ISOLTRAP mass measurements of exotic nuclides at

The ISOLTRAP experiment at the ISOLDE facility at CERN is a Penning trap mass spectrometer for on-line mass measurements on short-lived radionuclides. It allows the determination of atomic masses of exotic nuclides with a relative uncertainty of only 10−8. The results provide important information for, e.g., weak interaction studies and nuclear models. Recent ISOLTRAP investigations and applications of high-precision mass measurements are discussed.

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Super-Allowed β Decay of23Mg Studied with a High-Precision Germanium Detector

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An ion cooler-buncher for high-sensitivity collinear laser spectroscopy at ISOLDE

International audience; A gas-filled segmented linear Paul trap has been installed at the focal plane of the high-resolution separator (HRS) at CERN-ISOLDE. As well as providing beams with a reduced transverse emittance, this device is also able to accumulate the ions and release the sample in bunches with a well-defined time structure. This has recently permitted collinear laser spectroscopy with stable and radioactive bunched beams to be demonstrated at ISOLDE. Surface-ionized 39, 44, 46K and 85Rb beams were accelerated to 30keV, mass separated and injected into the trap for subsequent extraction and delivery to the laser setup. The ions were neutralized in a charge exchange cell and exci…

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Isoltrap pins down masses of exotic nuclides

The mass of radionuclides contribute to a variety of fundamental studies including tests of the weak interaction and the Standard Model. The limits of mass measurements of exotic nuclides have been extended considerably by the Penning-trap mass spectrometer ISOLTRAP at the ISOLDE facility at CERN. Recent ISOLTRAP measurements are summarized and current technical improvements are outlined.

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Ionization efficiency studies with charge breeder and conventional electron cyclotron resonance ion source

Radioactive Ion Beams play an increasingly important role in several European research facility programs such as SPES, SPIRAL1 Upgrade, and SPIRAL2, but even more for those such as EURISOL. Although remarkable advances of ECRIS charge breeders (CBs) have been achieved, further studies are needed to gain insight on the physics of the charge breeding process. The fundamental plasma processes of charge breeders are studied in the frame of the European collaboration project, EMILIE, for optimizing the charge breeding. Important information on the charge breeding can be obtained by conducting similar experiments using the gas mixing and 2-frequency heating techniques with a conventional JYFL 14 …

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“Safe” Coulomb Excitation ofMg30

We report on the first radioactive beam experiment performed at the recently commissioned REX-ISOLDE facility at CERN in conjunction with the highly efficient γ spectrometer MINIBALL. Using Mg-30 ions accelerated to an energy of 2.25 MeV/u together with a thin Ni-nat target, Coulomb excitation of the first excited 2(+) states of the projectile and target nuclei well below the Coulomb barrier was observed. From the measured relative deexcitation γ-ray yields the B(E2;0(gs)(+)R 2(1)(+)) value of Mg-30 was determined to be 241(31)e(2) fm(4). Our result is lower than values obtained at projectile fragmentation facilities using the intermediate-energy Coulomb excitation method, and confirms the …

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Precise half-life measurement of the Si-26 ground state

The beta-decay half-life of 26Si was measured with a relative precision of 1.4*10e3. The measurement yields a value of 2.2283(27) s which is in good agreement with previous measurements but has a precision that is better by a factor of 4. In the same experiment, we have also measured the non-analogue branching ratios and could determine the super-allowed one with a precision similar to the previously reported measurements. The experiment was done at the Accelerator Laboratory of the University of Jyvaskyla where we used the IGISOL technique with the JYFLTRAP facility to separate pure samples of 26Si.

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Coulomb Excitation of Neutron-Rich Zn Isotopes: First Observation of the21+State inZn80

Neutron-rich, radioactive Zn isotopes were investigated at the Radioactive Ion Beam facility REX-ISOLDE (CERN) using low-energy Coulomb excitation. The energy of the 2(1)+ state in 78Zn could be firmly established and for the first time the 2+ --> 0(1)+ transition in 80Zn was observed at 1492(1) keV. B(E2,2(1)+ --> 0(1)+) values were extracted for (74,76,78,80)Zn and compared to large scale shell model calculations. With only two protons outside the Z=28 proton core, 80Zn is the lightest N=50 isotone for which spectroscopic information has been obtained to date. Two sets of advanced shell model calculations reproduce the observed B(E2) systematics. The results for N=50 isotones indicate a g…

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Optimizing charge breeding techniques for ISOL facilities in Europe: conclusions from the EMILIE project

ThuM07; International audience; The present paper summarizes the results obtained from the past few years in the framework ofthe Enhanced Multi-Ionization of short-Lived Isotopes for Eurisol (EMILIE) project. The EMILIEproject aims at improving the charge breeding techniques with both Electron Cyclotron ResonanceIon Sources (ECRIS) and Electron Beam Ion Sources (EBISs) for European Radioactive Ion Beam(RIB) facilities. Within EMILIE, an original technique for debunching the beam from EBIS chargebreeders is being developed, for making an optimal use of the capabilities of CW post-acceleratorsof the future facilities. Such a debunching technique should eventually resolve duty cycle andtime st…

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New exotic beams from the SPIRAL 1 upgrade

Since 2001, the SPIRAL 1 facility has been one of the pioneering facilities in ISOL techniques for reaccelerating radioactive ion beams: the fragmentation of the heavy ion beams of GANIL on graphite targets and subsequent ionization in the Nanogan ECR ion source has permitted to deliver beams of gaseous elements (He, N, O, F, Ne, Ar, Kr) to numerous experiments. Thanks to the CIME cyclotron, energies up to 20 AMeV could be obtained. In 2014, the facility was stopped to undertake a major upgrade, with the aim to extend the production capabilities of SPIRAL 1 to a number of new elements. This upgrade, which is presently under commissioning, consists in the integration of an ECR booster in the…

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Approaching theN=82shell closure with mass measurements of Ag and Cd isotopes

Mass measurements of neutron-rich Cd and Ag isotopes were performed with the Penning trap mass spectrometer ISOLTRAP. The masses of ${}^{112,114\ensuremath{-}124}$Ag and ${}^{114,120,122\ensuremath{-}124,126,128}$Cd, determined with relative uncertainties between $2\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}8}$ and $2\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}7}$, resulted in significant corrections and improvements of the mass surface. In particular, the mass of $^{124}\mathrm{Ag}$ was previously unknown. In addition, other masses that had to be inferred from $Q$ values of nuclear decays and reactions have now been measured directly. The analysis includes various mass…

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Towards high-resolution laser ionization spectroscopy of the heaviest elements in supersonic gas jet expansion

Resonant laser ionization and spectroscopy are widely used techniques at radioactive ion beam facilities to produce pure beams of exotic nuclei and measure the shape, size, spin and electromagnetic multipole moments of these nuclei. However, in such measurements it is difficult to combine a high efficiency with a high spectral resolution. Here we demonstrate the on-line application of atomic laser ionization spectroscopy in a supersonic gas jet, a technique suited for high-precision studies of the ground- and isomeric-state properties of nuclei located at the extremes of stability. The technique is characterized in a measurement on actinium isotopes around the N=126 neutron shell closure. A…

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Injected 1+ ion beam as a diagnostics tool of charge breeder ECR ion source plasmas

International audience; Charge breeder electron cyclotron resonance ion sources (CB-ECRIS) are used as 1+  →n+  charge multiplication devices of post-accelerated radioactive ion beams. The charge breeding process involves thermalization of the injected 1+  ions with the plasma ions in ion–ion collisions, subsequent ionization by electron impact and extraction of the n+  ions. Charge breeding experiments of 85Rb and 133Cs ion beams with the 14.5 GHz PHOENIX CB-ECRIS operating with oxygen gas demonstrate the plasma diagnostics capabilities of the 1+  injection method. Two populations can be distinguished in the m/q-spectrum of the extracted ion beams, the low (1+  and 2+) charge states repres…

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Trap-assisted spectroscopy with REXTRAP

International audience; As one of the fashionable techniques for nuclear spectroscopy experiments, the beam manipulation in gas-filled Penning traps permits the accurate measurement of some of the ground state properties of exotic nuclides. It was recently applied using REXTRAP for the measurement of the half-life of 38Ca, one of the 0+ → 0+ β-decaying nuclide of interest for the determination of the Ft value for super-allowed transitions, and the test of the unitarity of the CKM matrix. The experimental setup and the original method of beam purification adopted for this measurement is presented.

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Off-line commissioning of the ISOLDE cooler

International audience; Among the multiple progresses in radioactive ion beam (RIB) manipulation for physics experiments, the beam cooling and bunching in gas-filled RF traps has become a widely used technique. It is particularly well adapted to precision experiments, such as Penning trap mass spectrometry or collinear laser spectroscopy. At ISOLDE, an rf quadrupole cooler and ion buncher (RFQCB) has been designed and developed to deliver radioactive beams of improved quality among most of the on-line experiments. The results of the first off-line tests have shown that high transmission efficiencies could be achieved with different RIBs of alkali metals, as it was expected. During the later…

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Diagnostics of a charge breeder electron cyclotron resonance ion source helium plasma with the injection of 23 Na 1+ ions

This work describes the utilization of an injected 23Na1þ ion beam as a diagnostics of the helium plasma of a charge breeder electron cyclotron resonance ion source. The obtained data allows estimating the upper limit for the ion-ion collision mean-free path of the incident sodium ions, the lower limit of ion-ion collision frequencies for all charge states of the sodium ions and the lower limit of the helium plasma density. The ion-ion collision frequencies of high charge state ions are shown to be at least on the order of 1–10 MHz and the plasma density is estimated to be on the order of 1011 cm−3 or higher. The experimental results are compared to simulations of the 23Na1þ capture into th…

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The Miniball spectrometer

The Miniball germanium detector array has been operational at the REX (Radioactive ion beam EXperiment) post accelerator at the Isotope Separator On-Line facility ISOLDE at CERN since 2001. During the last decade, a series of successful Coulomb excitation and transfer reaction studies have been performed with this array, utilizing the unique and high-quality radioactive ion beams which are available at ISOLDE. In this article, an overview is given of the technical details of the full Miniball setup, including a description of the γ-ray and particle detectors, beam monitoring devices and methods to deal with beam contamination. The specific timing properties of the REX-ISOLDE facility are hi…

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Developments towards in-gas-jet laser spectroscopy studies of actinium isotopes at LISOL

To study exotic nuclides at the borders of stability with laser ionization and spectroscopy techniques, highest efficiencies in combination with a high spectral resolution are required. These usually opposing requirements are reconciled by applying the in-gas-laser ionization and spectroscopy (IGLIS) technique in the supersonic gas jet produced by a de Laval nozzle installed at the exit of the stopping gas cell. Carrying out laser ionization in the low-temperature and low density supersonic gas jet eliminates pressure broadening, which will significantly improve the spectral resolution. This article presents the required modifications at the Leuven Isotope Separator On-Line (LISOL) facility…

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Coulomb Excitation ofCu68,70: First Use of Postaccelerated Isomeric Beams

We report on the first low-energy Coulomb excitation measurements with radioactive Ipi=6- beams of odd-odd nuclei 68,70Cu. The beams were produced at ISOLDE, CERN and were post-accelerated by REX-ISOLDE to 2.83 MeV/nucleon. gamma rays were detected with the MINIBALL spectrometer. The 6- beam was used to study the multiplet of states (3-, 4-, 5-, 6-) arising from the pi2p3/2nu1g9/2 configuration. The 4- state of the multiplet was populated via Coulomb excitation and the B(E2;6--->4-) value was determined in both nuclei. The results obtained illustrate the fragile stability of the Z=28 shell and N=40 subshell closures. A comparison with large-scale shell-model calculations using the 56Ni core…

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Towards high-precision mass measurements on 74Rb for a test of the CVC hypothesis and the unitarity of the CKM matrix

At the highest possible precisions, atomic-mass measurements can be used to perform fundamental studies. Examples for such studies are a check of the conserved-vector-current (CVC) hypothesis and the unitarity of the Cabibbo-Kobayashi-Maskawa (CKM) matrix, both postulates of the Standard Model. The comparative half-lives Ft of superallowed β decays constitute the nuclear-physics access to these tests. The Q value of the β decay of 74 Rb, one of the three experimentally accessible parameters that enter into the Ft values, has been measured with the ISOLTRAP experiment at ISOLDE/CERN. The ultimate mass precision requirement and the way to achieve it are outlined.

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In-gas laser ionization and spectroscopy of actinium isotopes near the N=126 closed shell

The in-gas laser ionization and spectroscopy (IGLIS) techniquewas applied on the $^{212–215}$Ac isotopes, produced at the Leuven Isotope Separator On-Line (LISOL) facility by using the in-gas-cell and the in-gas-jet methods. The first application under on-line conditions of the in-gas-jet laser spectroscopy method showed a superior performance in terms of selectivity, spectral resolution, and efficiency in comparison with the in-gas-cell method. Following the analysis of both experiments, the magnetic-dipole moments for the $^{212–215}$Ac isotopes, electric-quadrupole moments and nuclear spins for the $^{214,215}$Ac isotopes are presented and discussed. A good agreement is obtained with lar…

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Direct determination of the excitation energy of the quasistable isomer Ta180m

International audience; Ta180m is a naturally abundant quasistable nuclide and the longest-lived nuclear isomer known to date. It is of interest, among others, for the search for dark matter, for the development of a γ laser, and for astrophysics. So far, its excitation energy has not been measured directly but has been based on an evaluation of available nuclear reaction data. We have determined the excitation energy of this isomer with high accuracy using the Penning-trap mass spectrometer JYFLTRAP. The determined mass difference between the ground and isomeric states of Ta180 yields an excitation energy of 76.79(55) keV for Ta180m. This is the first direct measurement of the excitation e…

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Restoration of theN=82Shell Gap from Direct Mass Measurements ofSn132,134

A high-precision direct Penning trap mass measurement has revealed a 0.5-MeV deviation of the binding energy of (134)Sn from the currently accepted value. The corrected mass assignment of this neutron-rich nuclide restores the neutron-shell gap at N=82, previously considered to be a case of "shell quenching." In fact, the new shell gap value for the short-lived (132)Sn is larger than that of the doubly magic (48)Ca which is stable. The N=82 shell gap has considerable impact on fission recycling during the r process. More generally, the new finding has important consequences for microscopic mean-field theories which systematically deviate from the measured binding energies of closed-shell nu…

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Mass spectrometry of atomic ions produced by in-trap decay of short-lived nuclides

The triple-trap mass spectrometer ISOLTRAP at ISOLDE/CERN has demonstrated the feasibility of mass spectrometry of in-trap-decay product ions. This novel technique gives access to radionuclides, which are not produced directly at ISOL-type radioactive ion beam facilities. As a proof of principle, the in-trap decay of $^{37}K^+$ has been investigated in a Penning trap filled with helium buffer gas. The half-life of the mother nuclide was confirmed and the recoiling $^{37}Ar^+$ daughter ion was contained within the trap. The ions of either the mother or the daughter nuclide were transferred to a precision Penning trap, where their mass was determined.

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The MORA project

The MORA (Matter's Origin from the RadioActivity of trapped and oriented ions) project aims at measuring with unprecedented precision the D correlation in the nuclear beta decay of trapped and oriented ions. The D correlation offers the possibility to search for new CP-violating interactions, complementary to searches done at the LHC and with Electric Dipole Moments. Technically, MORA uses an innovative in-trap orientation method which combines the high trapping efficiency of a transparent Paul trap with laser orientation techniques. The trapping, detection, and laser setups are under development, for first tests at the Accelerator laboratory, JYFL, in the coming years.

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High-accuracy mass measurements of neutron-rich Kr isotopes

The atomic masses of the neutron-rich krypton isotopes {sup 84,86-95}Kr have been determined with the tandem Penning trap mass spectrometer ISOLTRAP with uncertainties ranging from 20 to 220 ppb. The masses of the short-lived isotopes {sup 94}Kr and {sup 95}Kr were measured for the first time. The masses of the radioactive nuclides {sup 89}Kr and {sup 91}Kr disagree by 4 and 6 standard deviations, respectively, from the present Atomic-Mass Evaluation database. The resulting modification of the mass surface with respect to the two-neutron separation energies as well as implications for mass models and stellar nucleosynthesis are discussed.

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Extending the applicability of an open-ring trap to perform experiments with a single laser-cooled ion.

An open-ring ion trap, also referred to as transparent trap was initially built up to perform $\beta$-$\nu$ correlation experiments with radioactive ions. This trap geometry is also well suited to perform experiments with laser-cooled ions, serving for the development of a new type of Penning trap, in the framework of the project TRAPSENSOR at the University of Granada. The goal of this project is to use a single $^{40}$Ca$^+$ ion as detector for single-ion mass spectrometry. Within this project and without any modification to the initial electrode configuration, it was possible to perform Doppler cooling on $^{40}$Ca$^+$ ions, starting from large clouds and reaching single ion sensitivity.…

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ISOLTRAP Mass Measurements for Weak-Interaction Studies

International audience; The conserved-vector-current (CVC) hypothesis of the weak interaction and the unitarity of the Cabibbo-Kobayashi-Maskawa (CKM) matrix are two fundamental postulates of the Standard Model. While existing data on CVC supports vector current conservation, the unitarity test of the CKM matrix currently fails by more than two standard deviations. High-precision mass measurements performed with the ISOLTRAP experiment at ISOLDE/CERN provide crucial input for these fundamental studies by greatly improving our knowledge of the decay energy of super-allowed beta decays. Recent results of mass measurements on the beta emitters 18Ne, 22Mg, 34Ar, and 74Rb as pertaining to weak-i…

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Cooling of radioactive ions with the Penning trap REXTRAP

Abstract Cooling of radioactive ion beams in a Penning trap is an essential component of the post-accelerator REX-ISOLDE at CERN. Prior to their charge-breeding and acceleration, ions from the on-line mass separator ISOLDE are accumulated, cooled and bunched with REXTRAP. This beam preparation provides short ion pulses with low emittance, key ingredient for a high efficiency of REX-ISOLDE. Two different cooling techniques have been investigated with REXTRAP. Both rely on the use of a buffer gas as the coolant but differ in the way the transversal compression of the stored ion cloud is achieved. Sideband cooling with a light buffer gas as coolant is the standard technique used at REXTRAP so …

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Prospects for advanced electron cyclotron resonance and electron beam ion source charge breeding methods for EURISOL

International audience; As the most ambitious concept of isotope separation on line (ISOL) facility, EURISOL aims at producing unprecedented intensities of post-accelerated radioactive isotopes. Charge breeding, which transforms the charge state of radioactive beams from 1+ to an n+ charge state prior to postacceleration, is a key technology which has to overcome the following challenges: high charge states for high energies, efficiency, rapidity and purity. On the roadmap to EURISOL, a dedicated R&D is being undertaken to push forward the frontiers of the present state-of-the-art techniques which use either electron cyclotron resonance or electron beam ion sources. We describe here the gui…

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High-accuracy mass measurements on neutron deficient neon isotopes

International audience; The atomic masses of the short-lived nuclides 17Ne and 19Ne have been measured with the triple-trap mass spectrometer ISOLTRAP at ISOLDE/CERN. The obtained mass excess for both nuclides deviates significantly from the literature value, in the case of 17Ne about 40 keV. The mass value of 17Ne can be applied for a test of the isobaric multiplet mass equation with respect to an isospin T = 3/2 quartet. In addition, both masses can contribute to the data analysis of collinear laser-spectroscopy experiments where mean-square nuclear-charge radii are determined.

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Mass measurements of $^{56-57}$Cr and the question of shell reincarnation at N = 32

Binding energies determined with high accuracy provide smooth derivatives of the mass surface for analysis of shell and pairing effects. Measurements with the Penning trap mass spectrometer ISOLTRAP at CERN-ISOLDE were made for $^{56-57}$Cr for which an accuracy of 4 $\times 10^{-8}$ was achieved. Analysis of the mass surface for the supposed new N = 32 shell closure rather indicates a sub-shell closure, but of a different nature than known cases such as $^{94}$Sr.

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