Temperature dependence of Photoluminescence and Amplified Spontaneous Emission in thin films of quasi-2D BA3MA3Pb5Br16 perovskites

Amplified spontaneous emission in thin films of quasi-2D BA3MA3Pb5Br16 lead halide perovskites

Quasi-2D (two-dimensional) hybrid perovskites are emerging as a new class of materials with high photoluminescence yield and improved stability compared to their three-dimensional (3D) counterparts. Nevertheless, despite their outstanding emission properties, few studies have been reported on amplified spontaneous emission (ASE) and a thorough understanding of the photophysics of these layered materials is still lacking. In this work, we investigate the ASE properties of multilayered quasi-2D BA3MA3Pb5Br16 films through the dependence of the photoluminescence on temperature and provide a novel insight into the emission processes of quasi-2D lead bromide perovskites. We demonstrate that the …