High-Statistics Sub-Barrier Coulomb Excitation of $^{106,108,110}$Sn

International audience; A Coulomb excitation campaign on $^{106,108,110}$Sn at 4.4–4.5 MeV/u was launched at the HIE-ISOLDE facility at CERN. Larger excitation cross sections and γ-ray statistics were achieved compared to previous experiments at ∼2.8 MeV/u. More precise $(B(E2;0_{1}^{ + } \to 2_{1}^{ + }))$ values, lifetimes of states via the Doppler shift attenuation method, and new $(B(E2;0_{1}^{ + } \to 2_{x}^{ + })), (B(E2;2_{1}^{ + } \to 4_{1}^{ + }))$ and $(Q(2_{1}^{ + }))$ values from the new Miniball data will be obtained and applied to test modern nuclear structure theories.

Large Shape Staggering in Neutron-Deficient Bi Isotopes

New collective structures in Au179 and their implications for the triaxial deformation of the Pt178 core

Laser Spectroscopy of Neutron-Rich Hg207,208 Isotopes: Illuminating the Kink and Odd-Even Staggering in Charge Radii across the N=126 Shell Closure

The mean-square charge radii of $^{207,208}$Hg ($Z=80, N=127,128$) have been studied for the first time and those of $^{202,203,206}$Hg ($N=122,123,126$) remeasured by the application of in-source resonance-ionization laser spectroscopy at ISOLDE (CERN). The characteristic \textit{kink} in the charge radii at the $N=126$ neutron shell closure has been revealed, providing the first information on its behavior below the $Z=82$ proton shell closure. A theoretical analysis has been performed within relativistic Hartree-Bogoliubov and non-relativistic Hartree-Fock-Bogoliubov approaches, considering both the new mercury results and existing lead data. Contrary to previous interpretations, it is d…

New ß-decaying state in 214Bi

Laser Spectroscopy of Neutron-Rich $^{207,208}$Hg Isotopes: Illuminating the Kink and Odd-Even Staggering in Charge Radii across the $N=126$ Shell Closure

The mean-square charge radii of $^{207,208}$Hg ($Z=80, N=127,128$) have been studied for the first time and those of $^{202,203,206}$Hg ($N=122,123,126$) remeasured by the application of in-source resonance-ionization laser spectroscopy at ISOLDE (CERN). The characteristic \textit{kink} in the charge radii at the $N=126$ neutron shell closure has been revealed, providing the first information on its behavior below the $Z=82$ proton shell closure. A theoretical analysis has been performed within relativistic Hartree-Bogoliubov and non-relativistic Hartree-Fock-Bogoliubov approaches, considering both the new mercury results and existing lead data. Contrary to previous interpretations, it is d…

Coulomb Excitation of Proton-rich N=80 Isotones at HIE-ISOLDE

Abstract A projectile Coulomb-excitation experiment was performed at the radioactive ion beam facility HIE-ISOLDE at CERN. The radioactive 140Nd and 142Sm ions were post accelerated to the energy of 4.62 MeV/A and impinged on a 1.45 mg/cm2-thin 208Pb target. The γ rays depopulating the Coulomb-excited states were recorded by the HPGe-array MINIBALL. The scattered charged particles were detected by a double-sided silicon strip detector in forward direction. Experimental γ-ray intensities were used for the determination of electromagnetic transition matrix elements. Preliminary results for the reduced transition strength of the B ( M 1 ; 2 3 + → 2 1 + ) = 0.35 ( 19 ) μ N 2 of 140Nd and a firs…

Decay studies of the long-lived states in Tl-186

9 pags., 12 figs., 3 tabs.

Identification of sub-μs isomeric states in the odd-odd nucleus 178Au

The neutron-deficient gold (Z=79) isotopes in the vicinity of the neutron midshell N=104 provide prolific examples of shape coexistence and isomerism at low excitation energy. They can be probed via a number of different experimental techniques. In this study, two new isomeric states with half-lives of 294(7) and 373(9) ns have been observed in the neutron-deficient odd-odd nuclide 178Au (N=99) in an experiment at the RITU gas-filled separator at JYFL, Jyväskylä. This result was achieved due to the use of a segmented planar germanium detector with a high efficiency at low energies. By applying the recoil-decay tagging technique, they were assigned to decay to two different long-lived α-deca…

Charge radii, moments, and masses of mercury isotopes across the N=126 shell closure

Combining laser spectroscopy in a Versatile Arc Discharge and Laser Ion Source, with Penning-trap mass spectrometry at the CERN-ISOLDE facility, this work reports on mean-square charge radii of neutron-rich mercury isotopes across the $N = 126$ shell closure, the electromagnetic moments of $^{207}$Hg and more precise mass values of $^{206-208}$Hg. The odd-even staggering (OES) of the mean square charge radii and the kink at $N = 126$ are analyzed within the framework of covariant density functional theory (CDFT), with comparisons between different functionals to investigate the dependence of the results on the underlying single-particle structure. The observed features are defined predomina…

Shape staggering of midshell mercury isotopes from in-source laser spectroscopy compared with density-functional-theory and Monte Carlo shell-model calculations

Neutron-deficient Hg177-185 isotopes were studied using in-source laser resonance-ionization spectroscopy at the CERN-ISOLDE radioactive ion-beam facility in an experiment combining different detection methods tailored to the studied isotopes. These include either α-decay tagging or multireflection time-of-flight gating for isotope identification. The endpoint of the odd-even nuclear shape staggering in mercury was observed directly by measuring for the first time the isotope shifts and hyperfine structures of Hg177-180. Changes in the mean-square charge radii for all mentioned isotopes, magnetic dipole, and electric quadrupole moments of the odd-A isotopes and arguments in favor of I=7/2 s…

Restoring the valence-shell stabilization in Nd 140

A projectile Coulomb-excitation experiment was performed at the radioactive-ion beam facility HIE-ISOLDE at CERN to obtain E2 and M1 transition matrix elements of Nd-140 using the multistep Coulomb-excitation code GOSIA. The absolute M1 strengths, B(M1; 2(2)(-) -> 2(1)(+)) = 0.033(8)mu(2)(N), B(M1 ; 2(3)(+) -> 2(1)(+)) = 0.26(-0.10)(+0.11)mu(2)(N), and B(M1; 2(4)+ -> 2(1)(+)) <0.04 mu(2)(N) identify the 2(3)(+) state as the main fragment of the one-quadrupole-phonon proton-neutron mixed-symmetry state of Nd-140. The degree of F-spin mixing in Nd-140 was quantified with the determination of the mixing matrix element VF-mix <7(-7)(-13) keV. Peer reviewed

Identification of a 6.6μs isomeric state in 175Ir

An experiment has been performed to study excited states in the neutron-deficient nucleus 175Ir via the use of the JUROGAM II high-purity germanium detector array and the RITU gas-filled separator at JYFL, Jyväskylä. By using isomer tagging, an isomeric state with a half-life of 6.58(15) μs has been observed in 175Ir for the first time. It has been established that the isomer decays via a 45.2 (E1)–26.1 (M1) keV cascade to new states below the previously reported ground state in 175Ir with Iπ = (5/2−). We now reassign this (5/2−) state to the isomeric state discovered in this study. peerReviewed

Competition between allowed and first-forbidden β decays of At208 and expansion of the Po208 level scheme

The structure of 208Po populated through the EC/β+ decay of 208At is investigated using γ-ray spectroscopy at the ISOLDE Decay Station. The presented level scheme contains 27 new excited states and 43 new transitions, as well as a further 50 previously observed γ rays which have been (re)assigned a position. The level scheme is compared to shell model calculations. Through this analysis approximately half of the β-decay strength of 208At is found to proceed via allowed decay and half via first-forbidden decay. The first-forbidden transitions predominantly populate core excited states at high excitation energies, which is qualitatively understood using shell model considerations. This mass r…

Search for Isovector Valence-Shell Excitations in 140 Nd and 142 Sm via Coulomb excitation reactions of radioactive ion beams

Projectile Coulomb excitation experiments were performed at HIE-ISOLDE at CERN with the radioactive ion beams of 140Nd and 142Sm. Ions with an energy of 4:62 MeV/A were impinging on a 1.45 mg/cm2 thick 208Pb target. The γ-rays depopulating the Coulomb-excited states were recorded by the HPGe-array MINIBALL and scattered particles were detected by a double-sided silicon strip detector. Experimental intensities were used for the determination of electromagnetic transition matrix elements. A preliminary result of the B(M1; 2+3 → 2+1) of 140Nd and an upper limit for the case of 142Sm are revealing the main fragments of the proton-neutron mixed-symmetry 2+1;ms states.

Hyperfine anomaly in gold and magnetic moments of $I^{\pi}$ $= 11/2^{−}$ gold isomers

Physical review / C 101(3), 034308 (2020). doi:10.1103/PhysRevC.101.034308

Dealing with contaminants in Coulomb excitation of radioactive beams

Abstract Data analysis of the Coulomb excitation experiment of the exotic 206Hg nucleus, recently performed at CERN’s HIE-ISOLDE facility, needs to account for the contribution to target excitation due to the strongly-present beam contaminant 130Xe. In this paper, the contamination subtraction procedure is presented.

First ß-decay spectroscopy of 135In and new ß-decay branches of 134In

Change in structure between the $I = 1/2$ states in $^{181}$Tl and $^{177,179}$Au

Abstract The first accurate measurements of the α-decay branching ratio and half-life of the I π = 1 / 2 + ground state in 181Tl have been made, along with the first determination of the magnetic moments and I = 1 / 2 spin assignments of the ground states in 177,179Au. The results are discussed within the complementary systematics of the reduced α-decay widths and nuclear g factors of low-lying, I π = 1 / 2 + states in the neutron-deficient lead region. The findings shed light on the unexpected hindrance of the 1 / 2 + → 1 / 2 + , 181Tl → g 177 Aug α decay, which is explained by a mixing of π 3 s 1 / 2 and π 2 d 3 / 2 configurations in 177Aug, whilst 181Tlg remains a near-pure π 3 s 1 / 2 .…

Quadrupole deformation of Xe-130 measured in a Coulomb-excitation experiment

Physical review / C 102(5), 054304 (2020). doi:10.1103/PhysRevC.102.054304

First β -decay spectroscopy of In 135 and new β -decay branches of In 134

α -decay branching ratio of Pt180

Shape coexistence in Au 187 studied by laser spectroscopy

Hyperfine-structure parameters and isotope shift of the 9/2$^−$ isomeric state in $^{187}$Au relative to $^{197}$Au for the 267.6-nm atomic transition have been measured for the first time using the in-source resonance-ionization spectroscopy technique. The magnetic dipole moment and change in the mean-square charge radius for this 9/2$^−$ isomer have been deduced. The observed large isomer shift relative to the 1/2$^+$ ground state in $^{187}$Au confirms the occurrence of the shape coexistence in $^{187}$Au proposed earlier from the analysis of the nuclear spectroscopic data and particle plus triaxial rotor calculations. The analysis of the magnetic moment supports the previously proposed …

Identification of a 6.6μs isomeric state in Ir175

Detailed spectroscopy of doubly magic $^{132}$Sn

The structure of the doubly magic $^{132}_{50}$Sn$_{82}$ has been investigated at the ISOLDE facility at CERN, populated both by the $\beta^-$decay of $^{132}$In and $\beta^-$-delayed neutron emission of $^{133}$In. The level scheme of $^{132}$Sn is greatly expanded with the addition of 68 $\gamma$-transitions and 17 levels observed for the first time in the $\beta$ decay. The information on the excited structure is completed by new $\gamma$-transitions and states populated in the $\beta$-n decay of $^{133}$In. Improved delayed neutron emission probabilities are obtained both for $^{132}$In and $^{133}$In. Level lifetimes are measured via the Advanced Time-Delayed $\beta\gamma\gamma$(t) fas…

Population of lead isotopes in binary reactions using a Rb 94 radioactive beam

8 pags., 9 figs.

Identification of sub- μs isomeric states in the odd-odd nucleus Au178

The neutron-deficient gold (Z=79) isotopes in the vicinity of the neutron midshell N=104 provide prolific examples of shape coexistence and isomerism at low excitation energy. They can be probed via a number of different experimental techniques. In this study, two new isomeric states with half-lives of 294(7) and 373(9) ns have been observed in the neutron-deficient odd-odd nuclide Au178 (N=99) in an experiment at the RITU gas-filled separator at JYFL, Jyvaskyla. This result was achieved due to the use of a segmented planar germanium detector with a high efficiency at low energies. By applying the recoil-decay tagging technique, they were assigned to decay to two different long-lived α-deca…

β decay of In133 : γ emission from neutron-unbound states in Sn133

Excited states in Sn-133 were investigated through the beta decay of In-133 at the ISOLDE facility. The ISOLDE Resonance Ionization Laser Ion Source (RILIS) provided isomer-selective ionization for In-133, allowing us to study separately, and in detail, the beta-decay branch of In-133 J(pi)= (9/2(+)) ground state and its J(pi) = (1/2(-)) isomer.Thanks to the large spin difference of the two beta-decaying states of In-133, it is possible to investigate separately the lower and higher spin states in the daughter, Sn-133, and thus to probe independently different single-particle and single-hole levels. We report here new gamma transitions observed in the decay of In-133, including those assign…

Charge radii and electromagnetic moments of At195–211

Hyperfine-structure parameters and isotope shifts of At195-211 have been measured for the first time at CERN-ISOLDE, using the in-source resonance-ionization spectroscopy method. The hyperfine structures of isotopes were recorded using a triad of experimental techniques for monitoring the photo-ion current. The Multi-Reflection Time-of-Flight Mass Spectrometer, in connection with a high-resolution electron multiplier, was used as an ion-counting setup for isotopes that either were affected by strong isobaric contamination or possessed a long half-life; the ISOLDE Faraday cups were used for cases with high-intensity beams; and the Windmill decay station was used for short-lived, predominantl…

Large shape staggering in neutron-deficient Bi isotopes

The changes in the mean-square charge radius (relative to 209Bi), magnetic dipole, and electric quadrupole moments of 187,188,189,191Bi were measured using the in-source resonance-ionization spectroscopy technique at ISOLDE (CERN). A large staggering in radii was found in 187,188,189Big, manifested by a sharp radius increase for the ground state of 188Bi relative to the neighboring 187,189Big. A large isomer shift was also observed for 188Bim. Both effects happen at the same neutron number, N=105, where the shape staggering and a similar isomer shift were observed in the mercury isotopes. Experimental results are reproduced by mean-field calculations where the ground or isomeric states were…

In-source laser spectroscopy of dysprosium isotopes at the ISOLDE-RILIS

A number of radiogenically produced dysprosium isotopes have been studied by in-source laser spectroscopy at ISOLDE using the Resonance Ionization Laser Ion Source (RILIS). Isotope shifts were measured relative to $^{152}$Dy in the 4 f$^{ 10}$6s$^{2}$ $^5$I$_8$ (gs) $\rightarrow$ 4 f$^{ 10}$6s6p (8,1)$^8_o$ (418.8 nm$_{vac}$) resonance transition. The electronic factor, F, and mass shift factor, M, were extracted and used for determining the changes in mean-squared charge radii for $^{145m}$Dy and $^{147m}$Dy for the first time. A number of radiogenically produced dysprosium isotopes have been studied by in-source laser spectroscopy at ISOLDE using the Resonance Ionization Laser Ion Source (…

Characterization of the shape-staggering effect in mercury nuclei

In rare cases, the removal of a single proton (Z) or neutron (N) from an atomic nucleus leads to a dramatic shape change. These instances are crucial for understanding the components of the nuclear interactions that drive deformation. The mercury isotopes (Z = 80) are a striking example1,2: their close neighbours, the lead isotopes (Z = 82), are spherical and steadily shrink with decreasing N. The even-mass (A = N + Z) mercury isotopes follow this trend. The odd-mass mercury isotopes 181,183,185Hg, however, exhibit noticeably larger charge radii. Due to the experimental difficulties of probing extremely neutron-deficient systems, and the computational complexity of modelling such heavy nucl…