0000000000129643
AUTHOR
Stephan Oberstedt
Actinide and lanthanide thin-layer developments using a drop-on-demand printing system
Actinide and lanthanide thin layers with specific requirements regarding thickness, homogeneity, chemical purity, mechanical stability, and backing properties are applied in a multitude of physics and chemistry experiments. A novel target preparation method, the so-called “Drop-on-Demand” (DoD) technique, based on a commercial nanoliter (nL) dispenser is applied since a few years in the Nuclear Chemistry unit at Johannes Gutenberg University Mainz. The wetting behaviour of the nL droplets on the substrate’s surface is a key parameter determining the spatial distribution of the deposited material after evaporation. By switching from aqueous to organic solvents as well as by substrate surface…
Mass and charge distributions in the very asymmetric mass region of the neutron induced fission of
Abstract The mass-separator Lohengrin was used to measure the yields of the light fission products with A=74−85 and their nuclear charge and kinetic energy distributions from the odd- Z compound nucleus 239 Np ∗ formed by double capture of thermal neutrons. The mass yield distribution reveals an influence of the fragment shell with N=50 affecting also the nuclear charge and kinetic energy distributions. An odd–even effect for protons is found in the very asymmetric mass division, increasing from 4% to 35% with increasing fission asymmetry. This is in contrast to findings in normal asymmetric fission (region of high fission yields) where no odd–even effect for protons was observed. An odd–ev…
Mass and charge distributions in the very asymmetric thermal neutron induced fission of the odd-Z nucleus 242mAm
Yields of light fission products (A = 68, 70-84, 87, 88, 94, 96, 98, 102 and 106-108), their kinetic energies and nuclear charge distributions (A = 71-84, 87 and 88) in the thermal neutron induced fission of the odd-Z nucleus Am-242m(Z = 95) were measured using the mass-separator Lohengrin at the Institute Laue-Langevin in Grenoble (France). The mass yield curve shows a fine structure at A = 70, probably due to shell and/or odd-even effects affecting also the nuclear charge distribution. The analysis of isotopic chain yields gives evidence for a very low excitation energy of the lightest fission fragments observed. A preferential formation of fragments with even Z is found for this odd-Z co…