0000000000132874
AUTHOR
Karl-heinz Hellmuth
The effect of microscale pore structure on matrix diffusion—a site-specific study on tonalite
Abstract The matrix diffusion of non-sorbing tracers was studied in rocks from the Syyry area, Central Finland (SY1). The effect of alteration and weathering on rock matrix porosity and on the available pore space, which affects diffusivity, are discussed. The main rock type in the crystalline bedrock of Syyry is a slightly foliated, gray tonalite with mica gneiss inclusions as well as minor, more mafic inclusions. The total porosity and the spatial porosity distribution and microstructure of the rocks were investigated using infiltration of carbon- 14-methylmethacrylate, electron microscopy and Hg-porosimetry. The laboratory-scale diffusion experiments were performed using (1) the out-leac…
Transport of recoil atoms in a stream of liquid-air-cooled pure helium
Abstract Pure commercial helium cooled down to the temperature of liquid air (80 K) has been used for rapid transportation of recoil atoms over distances as long as 10 m. Transport efficiencies of several tens of per cent have been obtained for recoil atoms resulting from alpha decay or from decay by fission. The angle of divergence of the beam of recoil atoms at the exit of the transport capillary is measured to be (11±2)° for particles of mass number A = 211. Experimental results are discussed in terms of thermal diffusion. The elimination of carrier vapors will probably simplify the use of the helium-jet technique in on-line mass separators.
Ein schnelles on-line trennsystem unter anwendung von helium-jet- und zentrifugentechnik
Abstract A centrifuge for continuous liquid-liquid phase separation is described. It is designed for rapid solvent extraction of short-lived radioactive isotopes (half-lives in the order of seconds). The centrifuge is characterized by simple construction and operation principle, easy handling, low cost, and a minimum hold-up time of less than five seconds (phase purity 99.0–99.9%). The on-line connection to a helium-jet transport system is described. Problems concerning the transfer of activities into a liquid phase from the helium-jet at atmospheric pressure are discussed.