0000000000139635

AUTHOR

Klaus Harms

showing 16 related works from this author

Stereoselective Nucleophilic Addition Reactions of Reactive Pseudopeptides

1992

Reaction mechanismAddition reactionNucleophilic additionChemistryOrganic chemistryStereoselectivityGeneral MedicineGeneral ChemistryNucleophilic abstractionCatalysisAngewandte Chemie International Edition in English
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Bis (μ-tetrazolato-NN′) bridged dinuclear nickel(II) Schiff base complexes: Tandem synthesis, structure and self assembly

2015

Abstract Two new bis(μ-tetrazolato-NN′) bridged dinuclear nickel(II) Schiff base complexes [Ni2L12(PTZ)2]·2(CH3)2SO·2.69H2O (1) and 2[Ni2L22(PTZ)2]·3H2O (2) (HL1 and HL2 are Schiff bases, HL1 = 2-((2-(dimethylamino)ethylimino)methyl)phenol, HL2 = 2-((2-(methylamino)ethylimino)methyl)-6-methoxyphenol and HPTZ is 5-pyrazinyltetrazole) have been synthesized via [3+2] cyclo-addition of 2-cyanopyrazine and sodium azide in presence of nickel(II) acetate tetrahydrate and the respective Schiff bases. The structures of the complexes are confirmed by single crystal X-ray diffraction analysis. Both complexes show fluorescence. The change in the denticity of the Schiff base blocking ligand is shown to …

Schiff baseDenticityTetrahydrateLigandStereochemistrySupramolecular chemistrychemistry.chemical_elementschiff base 15-pyrazinyltetrazolateInorganic Chemistrychemistry.chemical_compoundNickelchemistry3-dipolar cycloaddition13-Dipolar cycloadditionPolymer chemistryMaterials ChemistrySodium azidePhysical and Theoretical Chemistrydinuclearta116nickel(II)Polyhedron
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Heterotope Wirtmoleküle zur Einlagerung von zwei verschiedenen Gästen

1991

chemistry.chemical_compoundBenzylaminechemistryGeneral MedicineMedicinal chemistryAngewandte Chemie
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Organotin(IV) complexes with tetraethyl ethylene- and propylene-diphosphonates

1995

The series of organotin halide complexes with tetraethyl ethylene- and propylene-diphosphonates R n SnX 4-n .L [n=0, X=Cl; n=1, R=Me, X=Cl, Br; n=1, R=Ph, X=Cl; n=2 R=Me, Et, Bu, X=Cl, Br; n=2, R=Ph, X=Cl; L=(EtO) 2 P(O)CH 2 CHR'P(O)(OEt) 2 , R'=H, Me] were synthesized and characterized by means of NMR and Mossbauer spectroscopy. The crystal structure of the complex of diphenyltin dichloride with propylenediphosphonate was determined. The complex consists of polymer chains with bridging bidentate ligands and an octahedral tin environment containing two types of phosphoryl fragments. All of the R 2 SnX 2 adducts have trans-R 2 SnX 4 geometries of tin coordination octahedra according to the q…

DenticityCoordination sphereEthyleneChemistryStereochemistryGeneral ChemistryNuclear magnetic resonance spectroscopyQuadrupole splittingCrystal structureMedicinal chemistryAdductInorganic Chemistrychemistry.chemical_compoundMössbauer spectroscopyApplied Organometallic Chemistry
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Phosphoraneiminato complexes of manganese and cobalt with heterocubane structure

1999

The phosphoraneiminato complexes [MnBr(NPEt3)]4 (1) and [M4Br5{NP(NMe2)3}3] with M = Mn (2) and M = Co (3) are prepared by melting reactions from the anhydrous metal dibromides with the silylated phosphaneimines Me3SiNPR3 (R = Et, NMe2) in the presence of potassium fluoride. All complexes are characterized by crystal structure analyses. 1 forms an only slightly distorted Mn4N4 heterocubane skeleton with an approximate Td symmetry and short Mn…Mn distances of average 295.7 pm. In the structures of 2 and 3 one μ3-NPEt3 ligand of 1 is replaced by one bromine atom with μ3-function. This leads to the novel heterocubane type M4N3Br with approximate C3 symmetry. The deformation of the cubic skelet…

Ligandchemistry.chemical_elementBromine atomCrystal structureManganeseMagnetic susceptibilityPotassium fluorideInorganic ChemistryMetalchemistry.chemical_compoundCrystallographychemistryvisual_artPolymer chemistryvisual_art.visual_art_mediumCobalt
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ChemInform Abstract: Stereoselective Nucleophilic Addition Reactions of Reactive Pseudopeptides.

2010

Addition reactionNucleophilic additionChemistryStereoselectivityGeneral MedicineCombinatorial chemistryChemInform
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Kronenether mit einem Lewis-sauren Zentrum, eine neue Klasse heterotoper Wirtmoleküle

1991

chemistry.chemical_compoundchemistryStereochemistryGeneral MedicineNuclear magnetic resonance spectroscopyLewis acids and basesCyclophaneAngewandte Chemie
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A ferromagnetic tetranuclear nickel(II) Schiff-base complex with an asymmetric Ni4O4 cubane core

2014

Abstract The ferromagnetic tetranuclear nickel(II) complex [Ni4(L)4(CH3OH)2]·2MeOH·8H2O (1) has been synthesized by reacting nickel nitrate hexahydrate with the Schiff base ligand H2L (H2L = N-(2-hydroxyphenyl)-3-methoxy-salicylideneamine). Complex 1 was characterized by analytical, thermogravimetric, optical and magnetic techniques. The solid state structure of 1 was established by single crystal X-ray diffraction analysis. Crystal structure determination shows the formation of a distorted Ni4O4 cubane moiety encapsulated by four Schiff base ligands. Compound 1 crystallizes in the triclinic space group P 1 ¯ with a = 12.7624(9) A, b = 15.0477(9) A, c = 16.8589(10) A, α = 94.732(2)°, β = 94…

Schiff baseChemistryLigandchemistry.chemical_elementCrystal structureTriclinic crystal systemInorganic Chemistrychemistry.chemical_compoundCrystallographyNickelCubaneMaterials ChemistryMoietyPhysical and Theoretical ChemistrySingle crystalPolyhedron
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Co-crystallization of Keggin type polyoxometalates [HL]3[PW12O40] and [Ln(DMF)8][PW12O40] (Ln=La, Dy, Yb) (L=N-(2-hydroxyphenyl)-3-methoxy-salicylide…

2016

Abstract Four new Keggin type polyoxometalate clusters [HL]3[PW12O40]·5MeOH (1) and [Ln(DMF)8][PW12O40] {Ln = La (2), Dy (3), Yb (4)} (L = N-(2-hydroxyphenyl)-3-methoxy-salicylideneamine) have been synthesized. Co-crystallization of complex 1 with each of the three complexes 2–4 takes place when the Schiff base ligand is treated with hydrated phosphotungstic acid, H3[PW12O40]·xH2O, hydrated lanthanide nitrate, Ln(NO3)3·6H2O in the presence of Ni(NO3)2·6H2O. The Schiff base ligand is protonated in complex 1 and thus it is neutralizing the charge of the polyoxotungstate anion, [PW12O40]3−. A dimethylformamide (DMF) coordinated trivalent lanthanide ion balances the negative charge of the polyo…

LanthanideSchiff base010405 organic chemistryLigandInorganic chemistryProtonationCrystal structure010402 general chemistry01 natural sciences0104 chemical sciencesInorganic Chemistrychemistry.chemical_compoundCrystallographychemistryPolyoxometalateMaterials ChemistryDimethylformamidePhosphotungstic acidPhysical and Theoretical ChemistryPolyhedron
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CCDC 968535: Experimental Crystal Structure Determination

2014

Related Article: Hari Nayek, Sudeshna Saha, Souvik Pal, Carlos Gomez Garcia, Klaus Harms|2014|Polyhedron|74|1|doi:10.1016/j.poly.2014.02.036

Space GroupCrystallographyCrystal SystemCrystal StructureCell ParametersExperimental 3D Coordinatestetrakis(mu~3~-2-((2-oxyphenyl)carbonoimidoyl)-6-methoxyphenolato)-bis(methanol)-tetra-nickel methanol solvate octahydrate
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CCDC 1021604: Experimental Crystal Structure Determination

2014

Related Article: Mithun Das, Klaus Harms, Biswa Nath Ghosh, Kari Rissanen, Shouvik Chattopadhyay|2015|Polyhedron|87|286|doi:10.1016/j.poly.2014.11.012

bis(mu2-5-(pyrazin-2-yl)-1H-tetrazol-1-yl)-bis(2-(((2-(dimethylamino)ethyl)imino)methyl)phenolato)-di-nickel dimethyl sulfoxide solvate hydrateSpace GroupCrystallographyCrystal SystemCrystal StructureCell ParametersExperimental 3D Coordinates
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CCDC 1419401: Experimental Crystal Structure Determination

2015

Related Article: Sudeshna Saha, Partha P. Jana, Carlos J. Gómez-García, Klaus Harms, Hari Pada Nayek|2016|Polyhedron|104|58|doi:10.1016/j.poly.2015.11.035

Space GroupCrystallographyoctakis(NN-dimethylformamide)-lanthanum (mu-phosphato)-tetracosakis(mu-oxo)-dodecaoxo-dodeca-tungstenCrystal SystemCrystal StructureCell ParametersExperimental 3D Coordinates
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CCDC 1021611: Experimental Crystal Structure Determination

2014

Related Article: Mithun Das, Klaus Harms, Biswa Nath Ghosh, Kari Rissanen, Shouvik Chattopadhyay|2015|Polyhedron|87|286|doi:10.1016/j.poly.2014.11.012

bis(mu2-5-(pyrazin-2-yl)-1H-tetrazol-1-yl)-bis(2-methoxy-6-(((2-(methylamino)ethyl)imino)methyl)phenolato)-di-nickel unknown solvate sesquihydrateSpace GroupCrystallographyCrystal SystemCrystal StructureCell ParametersExperimental 3D Coordinates
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CCDC 1419400: Experimental Crystal Structure Determination

2015

Related Article: Sudeshna Saha, Partha P. Jana, Carlos J. Gómez-García, Klaus Harms, Hari Pada Nayek|2016|Polyhedron|104|58|doi:10.1016/j.poly.2015.11.035

Space GroupCrystallographyCrystal Systemtris((2-hydroxy-3-methoxyphenyl)-N-(2-hydroxyphenyl)methaniminium) (mu-phosphato)-tetracosakis(mu-oxo)-dodecaoxo-dodeca-tungsten methanol solvateCrystal StructureCell ParametersExperimental 3D Coordinates
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CCDC 1419402: Experimental Crystal Structure Determination

2015

Related Article: Sudeshna Saha, Partha P. Jana, Carlos J. Gómez-García, Klaus Harms, Hari Pada Nayek|2016|Polyhedron|104|58|doi:10.1016/j.poly.2015.11.035

Space GroupCrystallographyCrystal Systemoctakis(NN-dimethylformamide)-dysprosium (mu12-phosphato)-tetracosakis(mu2-oxido)-dodecaoxo-dodeca-tungstenCrystal StructureCell ParametersExperimental 3D Coordinates
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CCDC 1419403: Experimental Crystal Structure Determination

2015

Related Article: Sudeshna Saha, Partha P. Jana, Carlos J. Gómez-García, Klaus Harms, Hari Pada Nayek|2016|Polyhedron|104|58|doi:10.1016/j.poly.2015.11.035

Space GroupCrystallographyoctakis(NN-dimethylformamide)-ytterbium (mu12-phosphato)-tetracosakis(mu2-oxido)-dodecaoxo-dodeca-tungstenCrystal SystemCrystal StructureCell ParametersExperimental 3D Coordinates
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