0000000000140249
AUTHOR
M. Itoh
Dissociation mechanisms of cluster ions resolved using ab-initio molecular orbital calculations
We have examined the cluster-size effect on fragments in the collision-induced dissociation (CID) of small boron clusters (B + n , n ≤ 8) by means of ab-initio molecular orbital (MO) calculation, for conditions representative of low-Z cationic clusters in plasma. Single cations B + (leaving B 0 n-1 ) are predominantly fragmented from small clusters B + n (n < 5) by low-energy collisions (<10 eV) with Xe atoms. With increasing the size n, beyond n = 5, B + n-1 (leaving B°) clusters are observed preferentially. This alternating trend in experiment has not been quantitatively explained by previous ab-initio MO calculations. We used a density functional method called B3LYP and basis functions 6…
Pygmy dipole resonance in208Pb
Scattering of protons of several hundred MeV is a promising new spectroscopic tool for the study of electric dipole strength in nuclei. A case study of 208Pb shows that at very forward angles J^pi = 1- states are strongly populated via Coulomb excitation. A separation from nuclear excitation of other modes is achieved by a multipole decomposition analysis of the experimental cross sections based on theoretical angular distributions calculated within the quasiparticle-phonon model. The B(E1) transition strength distribution is extracted for excitation energies up to 9 MeV, i.e., in the region of the so-called pygmy dipole resonance (PDR). The Coulomb-nuclear interference shows sensitivity to…
Complete dipole response in [sup 208]Pb from high-resolution polarized proton scattering at 0°
At the Research Center for Nuclear Physics, Osaka, Japan, the 208Pb(p,p´) reaction was measured at Ep=295 MeV and scattering angles Θlab= 0° - 10°. A high energy resolution of the order of ΔE/E ≈ 8x10^-5 was achieved, corresponding to ΔE=25-30 keV (FWHM). Cross sections were extracted by a multipole decomposition analysis of the angular distributions. Dominant contributions at very forward angles originate from E1 excitation due to Coulomb projectile-target interaction and spin M1 transitions caused by the spin-isospin part of the proton-nucleus interaction. A separation of these contributions was performed with two independent methods, viz. a multipole decomposition of the angular distribu…
Study of M1 and E1 excitations by high-resolution proton inelastic scattering measurement at forward angles
Experimental technique for measuring proton inelastic scattering with high‐resolution at 295 MeV and at forward angles including zero degrees is described. The method is useful for extracting spin part of the M1 strength via nuclear excitation as well as E1 strength via Coulomb excitation. An excitation energy resolution of 20 keV, good scattering angle resolution, and low background condition have been achieved. The experimental technique was applied for several sd and pf shell nuclei.
Nonquenched Isoscalar Spin-M1Excitations insd-Shell Nuclei
Differential cross sections of isoscalar and isovector spin-M1 (0(+)→1(+)) transitions are measured using high-energy-resolution proton inelastic scattering at E(p)=295 MeV on (24)Mg, (28)Si, (32)S, and (36)Ar at 0°-14°. The squared spin-M1 nuclear transition matrix elements are deduced from the measured differential cross sections by applying empirically determined unit cross sections based on the assumption of isospin symmetry. The ratios of the squared nuclear matrix elements accumulated up to E(x)=16 MeV compared to a shell-model prediction are 1.01(9) for isoscalar and 0.61(6) for isovector spin-M1 transitions, respectively. Thus, no quenching is observed for isoscalar spin-M1 transi…