0000000000147218
AUTHOR
R. Horn
Laser resonance ionization for efficient and selective ionization of rare species
Abstract Due to the steady development and refinement of powerful pulsed as well as continuous-wave lasers, resonance ionization has developed into an extremely versatile tool for numerous applications. Apart from suppressing isobaric interferences and contributing to isotopic selectivity already in the ionization process, resonant optical excitation and ionization with laser light ensures high overall efficiency and good temporal and spatial controls of the ions delivered to mass spectrometric applications. In the field of rare isotope research laser resonance ionization has nowadays become one of the key techniques, including similarly the determination of long-lived or stable ultra-trace…
Development and analysis of the Soil Water Infiltration Global database
27 Pags.- 11 Tabls.- 8 Figs. © Author(s) 2018. This work is distributed under the Creative Commons Attribution 4.0 License.
Atomic spectroscopy studies of short-lived isotopes and nuclear isomer separation with the ISOLDE RILIS
The Resonance Ionization Laser Ion Source (RILIS) at the ISOLDE on-line isotope separator is based on the selective excitation of atomic transitions by tunable laser radiation. Ion beams of isotopes of 20 elements have been produced using the RILIS setup. Together with the mass separator and a particle detection system it represents a tool for high-sensitive laser spectroscopy of short-lived isotopes. By applying narrow-bandwidth lasers for the RILIS one can study isotope shifts (IS) and hyperfine structure (HFS) of atomic optical transitions. Such measurements are capable of providing data on nuclear charge radii, spins and magnetic moments of exotic nuclides far from stability. Although t…
Resonance Ionization Laser Ion Source - Off-line tests at TRIUMF
Resonance ionization laser ion sources (RILIS) developed into the most powerful tool for radioactive ion beam production at on-line facilities, as they provide a selective ionization process with inherent suppression of unwanted isobaric contaminations at the ion source. While typical tunable laser systems for these applications are based on dye lasers, we developed an all solid state laser system which consists of three pulsed titanium:sapphire (ti:sa) lasers pumped by a single high repetition rate Nd:YAG laser. Each ti:sa laser provides up to 2.5 W average output power at 12 kHz repetition rate in the wavelength region of 700-950 nm with optional frequency doubling in BBO crystals. This l…
First laser ions at an off-line mass separator of the ISAC facility at TRIUMF
For efficient and in particular for selective production of radioactive ion beams at on-line mass separator facilities the technique of resonance ionization laser ion sources (RILIS) has become the most powerful tool. In facilities like ISOLDE at CERN they nowadays represent the most commonly used type of ion source for rare short-lived isotopes, delivering highest suppression of isobaric contaminations. For a first off-line demonstration preparing the development and installation of such a laser ion source at the new ISAC facility at TRIUMF in Vancouver (Canada), an all solid state laser system developed at the University of Mainz (Germany), was transferred and tested there at an off-line …
Charge-radius change and nuclear moments in the heavy tin isotopes from laser spectroscopy: Charge radius ofSn132
Laser spectroscopy measurements have been carried out on the neutron-rich tin isotopes with the COMPLIS experimental setup. Using the $5{s}^{2}5{p}^{2\phantom{\rule{0.3em}{0ex}}3}{P}_{0}\ensuremath{\rightarrow}5{s}^{2}5p6s\phantom{\rule{0.3em}{0ex}}{}^{3}{P}_{1}$ optical transition, hyperfine spectra of $^{126\ensuremath{-}132}\mathrm{Sn}$ and $^{125,127,129\ensuremath{-}131}\mathrm{Sn}{}^{m}$ were recorded for the first time. The nuclear moments and the mean square charge radius variation ($\ensuremath{\delta}\ensuremath{\langle}{r}_{c}^{2}\ensuremath{\rangle}$) were extracted. From the quadrupole moment values, these nuclei appear to be spherical. The magnetic moments measured are thus co…
Temporal Control of Pulses from a High-Repetition-Rate Tunable Ti:Sapphire Laser by Active Q-switching
We investigated the lasing characteristics of a Ti:sapphire laser pumped by a pulsed high-repetition-rate Nd:YAG laser. The pump laser has a pulsewidth of 450 ns, while the Ti:sapphire laser shows a significantly shorter pulse width of 25 ns for suitably intense pumping. The energy conversion efficiency of the laser is more than 10%. To synchronize different lasers and to avoid multiple spiking during one pump pulse, we use a Brewster-cut Pockels cell in the resonator for Q-switching. The temporal profile and conversion efficiency are determined and compared to theoretical estimates.
The next generation of laser spectroscopy experiments using light muonic atoms
Precision spectroscopy of light muonic atoms provides unique information about the atomic and nuclear structure of these systems and thus represents a way to access fundamental interactions, properties and constants. One application comprises the determination of absolute nuclear charge radii with unprecedented accuracy from measurements of the 2S - 2P Lamb shift. Here, we review recent results of nuclear charge radii extracted from muonic hydrogen and helium spectroscopy and present experiment proposals to access light muonic atoms with Z ≥ 3. In addition, our approaches towards a precise measurement of the Zemach radii in muonic hydrogen (μp) and helium (μ 3He+) are discussed. These resul…
Charge radius change in the heavy tin isotopes until A = 132 from laser spectroscopy
Laser spectroscopy measurements have been carried out on the very neutron-rich tin isotopes with the COMPLIS experimental setup. Using the 5s 25p 23P 0 → 5s 25p6s 3P 1 optical transition, hyperfine spectra of 126-132Sn and 125m, 127m, 129m-131mSn where recorded for the first time. The variation of the mean-square charge radius ( δ〈r 2〉) between these nuclei and nuclear moments of the isomers and the odd isotopes were thus measured. An odd-even staggering which inverts at A = 130 is clearly observed. This indicates a small appearance of a plateau on the δ〈r 2〉 which has to be confirmed by measuring the isotope shift beyond A = 132.
Recent developments in and applications of resonance ionization mass spectrometry
Resonance Ionization Mass Spectrometry (RIMS) has nowadays reached the status of a routine method for sensitive and selective ultratrace determination of long-lived radioactive isotopes in environmental, biomedical and technical samples. It provides high isobaric suppression, high to ultra-high isotopic selectivity and good overall efficiency. Experimental detection limits are as low as 106 atoms per sample and permit the fast and sensitive determination of ultratrace amounts of radiotoxic contaminations. Experimental arrangements for the detection of different radiotoxic isotopes, e.g. 236–244Pu, 89,90Sr and 99Tc in environmental samples are described, and the application of RIMS to the ul…