0000000000147791

AUTHOR

G. Pitari

showing 3 related works from this author

A machine learning examination of hydroxyl radical differences among model simulations for CCMI-1

2020

The hydroxyl radical (OH) plays critical roles within the troposphere, such as determining the lifetime of methane (CH4), yet is challenging to model due to its fast cycling and dependence on a multitude of sources and sinks. As a result, the reasons for variations in OH and the resulting methane lifetime (τCH4), both between models and in time, are difficult to diagnose. We apply a neural network (NN) approach to address this issue within a group of models that participated in the Chemistry-Climate Model Initiative (CCMI). Analysis of the historical specified dynamics simulations performed for CCMI indicates that the primary drivers of τCH4 differences among 10 models are the flux of UV li…

Atmospheric ScienceAtmospheric chemistry010504 meteorology & atmospheric sciencesneural networkAnalytical chemistry010501 environmental sciences01 natural sciencesTropospherelcsh:Chemistrychemistry.chemical_compoundMESSyErdsystem-ModellierungMixing ratioTropospheric ozoneIsopreneNOx0105 earth and related environmental sciencesEMAChydroxyl radicalPhotodissociationlcsh:QC1-999Atmospheric chemistry neural networkmachine learningchemistrylcsh:QD1-99913. Climate actionCCMI[SDE]Environmental SciencesHydroxyl radicalWater vaporlcsh:Physicsmethane lifetime
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Evaluation of observed and modelled aerosol lifetimes using radioactive tracers of opportunity and an ensemble of 19 global models

2016

Aerosols have important impacts on air quality and climate, but the processes affecting their removal from the atmosphere are not fully understood and are poorly constrained by observations. This makes modelled aerosol lifetimes uncertain. In this study, we make use of an observational constraint on aerosol lifetimes provided by radionuclide measurements and investigate the causes of differences within a set of global models. During the Fukushima Dai-Ichi nuclear power plant accident of March 2011, the radioactive isotopes cesium-137 (137Cs) and xenon-133 (133Xe) were released in large quantities. Cesium attached to particles in the ambient air, approximately according to their available ae…

lcsh:Chemistrylcsh:QD1-999lcsh:Physicslcsh:QC1-999Atmospheric Chemistry and Physics
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Evaluation of observed and modelled aerosol lifetimes using radioactive tracers of opportunity and an ensemble of 19 global models

2015

Abstract. Aerosols have important impacts on air quality and climate, but the processes affecting their removal from the atmosphere are not fully understood and are poorly constrained by observations. This makes modelled aerosol lifetimes uncertain. In this study, we make use of an observational constraint on aerosol lifetimes provided by radionuclide measurements and investigate the causes of differences within a set of global models. During the Fukushima Dai-Ichi nuclear power plant accident of March 2011, the radioactive isotopes cesium-137 (137Cs) and xenon-133 (133Xe) were released in large quantities. Cesium attached to particles in the ambient air, approximately according to their av…

[PHYS.PHYS.PHYS-AO-PH]Physics [physics]/Physics [physics]/Atmospheric and Oceanic Physics [physics.ao-ph][SDU.OCEAN]Sciences of the Universe [physics]/Ocean Atmosphere010504 meteorology & atmospheric sciences13. Climate action010501 environmental sciences01 natural sciences7. Clean energy0105 earth and related environmental sciences
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