Erratum: “Nanoscale x-ray imaging of spin dynamics in yttrium iron garnet” [J. Appl. Phys. 126, 173909 (2019)]

2021

Correlation between spin structure oscillations and domain wall velocities

2013

Magnetic sensing and logic devices based on the motion of magnetic domain walls rely on the precise and deterministic control of the position and the velocity of individual magnetic domain walls in curved nanowires. Varying domain wall velocities have been predicted to result from intrinsic effects such as oscillating domain wall spin structure transformations and extrinsic pinning due to imperfections. Here we use direct dynamic imaging of the nanoscale spin structure that allows us for the first time to directly check these predictions. We find a new regime of oscillating domain wall motion even below the Walker breakdown correlated with periodic spin structure changes. We show that the e…

Coherent Excitation of Heterosymmetric Spin Waves with Ultrashort Wavelengths

2017

In the emerging field of magnonics, spin waves are foreseen as signal carriers for future spintronic information processing and communication devices, owing to both the very low power losses and a high device miniaturisation potential predicted for short-wavelength spin waves. Yet, the efficient excitation and controlled propagation of nanoscale spin waves remains a severe challenge. Here, we report the observation of high-amplitude, ultrashort dipole-exchange spin waves (down to 80 nm wavelength at 10 GHz frequency) in a ferromagnetic single layer system, coherently excited by the driven dynamics of a spin vortex core. We used time-resolved x-ray microscopy to directly image such propagati…

Correlation between spin structure oscillations and domain wall velocities (presentation video)

2014

Magnetic sensing and logic devices based on the motion of magnetic domain walls rely on the precise and deterministic control of the position and the velocity of individual magnetic domain walls. Varying domain wall velocities have been predicted to result from intrinsic effects such as oscillating domain wall spin structure transformations and extrinsic pinning due to imperfections. We use direct dynamic imaging of the nanoscale spin structure to directly check these predictions. We find a new regime of oscillating domain wall motion even below the Walker breakdown correlated with periodic spin structure changes and we show that the extrinsic pinning from defects in the nanowire only affec…

Magnetic Skyrmions: Current-Induced Skyrmion Generation through Morphological Thermal Transitions in Chiral Ferromagnetic Heterostructures (Adv. Mate…

2018

Direct observation of spin wave focusing by a Fresnel lens

2020

Spin waves are discussed as promising information carrier for beyond complementary metal-oxide semiconductor data processing. One major challenge is guiding and steering of spin waves in a uniform film. Here, we explore the use of diffractive optics for these tasks by nanoscale real-space imaging using x-ray microscopy and careful analysis with micromagnetic simulations. We discuss the properties of the focused caustic beams that are generated by a Fresnel-type zone plate and demonstrate control and steering of the focal spot. Thus, we present a steerable and intense nanometer-sized spin-wave source. Potentially, this could be used to selectively illuminate magnonic devices like nano-oscill…

Switching by Domain-Wall Automotion in Asymmetric Ferromagnetic Rings

2017

A ring-shaped magnetic logic device offers two vortex states (clockwise and counterclockwise) to encode bits, with relative stability against external magnetic fields. The dynamics of magnetization switching in such structures, though, still need unraveling. The authors present direct experimental visualization of reproducible, robust switching in magnetic rings via domain-wall automotion, which does not require an applied field. Simulations reveal that annihilation of domain walls through automotion always occurs, with the detailed topology of the walls only influencing the dynamics locally, in line with the experimental results.

Peri-operative red blood cell transfusion in neonates and infants: NEonate and Children audiT of Anaesthesia pRactice IN Europe: A prospective Europe…

2022

BACKGROUND Little is known about current clinical practice concerning peri-operative red blood cell transfusion in neonates and small infants. Guidelines suggest transfusions based on haemoglobin thresholds ranging from 8.5 to 12���g���dl-1, distinguishing between children from birth to day 7 (week 1), from day 8 to day 14 (week 2) or from day 15 (���week 3) onwards. OBJECTIVE To observe peri-operative red blood cell transfusion practice according to guidelines in relation to patient outcome. DESIGN A multicentre observational study. SETTING The NEonate-Children sTudy of Anaesthesia pRactice IN Europe (NECTARINE) trial recruited patients up to 60 weeks' postmenstrual age undergoing anaesthe…

Current-Induced Skyrmion Generation through Morphological Thermal Transitions in Chiral Ferromagnetic Heterostructures.

2018

© 2018 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim Magnetic skyrmions promise breakthroughs in future memory and computing devices due to their inherent stability and small size. Their creation and current driven motion have been recently observed at room temperature, but the key mechanisms of their formation are not yet well-understood. Here it is shown that in heavy metal/ferromagnet heterostructures, pulsed currents can drive morphological transitions between labyrinth-like, stripe-like, and skyrmionic states. Using high-resolution X-ray microscopy, the spin texture evolution with temperature and magnetic field is imaged and it is demonstrated that with transient Joule heating, topologica…

Microanalytical methods for in-situ high-resolution analysis of rock varnish at the micrometer to nanometer scale

2015

Abstract A wide range of analytical techniques were used to investigate rock varnish from different locations (Negev, Israel; Knersvlakte, South Africa; Death Valley and Mojave Desert, California): a 200 nm-femtosecond laser ablation-inductively coupled plasma-mass spectrometer (LA-ICP-MS), an electron probe microanalyzer (EPMA), focused ion beam (FIB) slicing, and scanning transmission X-ray microscopy–near edge X-ray absorption fine structure spectroscopy (STXM–NEXAFS). This combination enables comprehensive high-spatial-resolution analysis of rock varnish. Femtosecond LA-ICP-MS and EPMA were used for quantitative determination of element concentrations. In-situ measurements were conducte…

Automotive domain wall propagation in ferromagnetic rings

2015

Automotive domain wall propagation is a self-propelling motion utilizing the energy stored in a particular energy reservoir of the spin structure to speed up domain wall beyond its equilibrium value given by external driving force and damping. Such a concept of DW motion is of great interest due to recent development of spintronic devices based on domain walls, where automotion could be used to assist or prevent domain wall pinning at low driving fields1-2. In turn, most of studies so far have been devoted to the automotion invoked by DW transformations from metastable to stable states3-4; appearing at sufficiently high magnetic fields strong and enough to trigger domain wall spin structure…

Nanoscale X-Ray Imaging of Spin Dynamics in Yttrium Iron Garnet

2019

Time-resolved scanning transmission x-ray microscopy (TR-STXM) has been used for the direct imaging of spin wave dynamics in thin film yttrium iron garnet (YIG) with spatial resolution in the sub 100 nm range. Application of this x-ray transmission technique to single crystalline garnet films was achieved by extracting a lamella (13x5x0.185 $\mathrm{\mu m^3}$) of liquid phase epitaxy grown YIG thin film out of a gadolinium gallium garnet substrate. Spin waves in the sample were measured along the Damon-Eshbach and backward volume directions of propagation at gigahertz frequencies and with wavelengths in a range between 100~nm and 10~$\mathrm{\mu}$m. The results were compared to theoretical …

Ptychographic imaging and micromagnetic modeling of thermal melting of nanoscale magnetic domains in antidot lattices

2020

CA extern Antidot lattices are potential candidates to act as bit patterned media for data storage as they are able to trap nanoscale magnetic domains between two adjacent holes. Here, we demonstrate the combination of micromagnetic modeling and x-ray microscopy. Detailed simulation of these systems can only be achieved by micromagnetic modeling that takes thermal effects into account. For this purpose, a Landau-Lifshitz-Bloch approach is used here. The calculated melting of magnetic domains within the antidot lattice is reproduced experimentally by x-ray microscopy. Furthermore, we compare conventional scanning transmission x-ray microscopy with resolution enhanced ptychography. Hence, we …

Enhanced Nonadiabaticity in Vortex Cores due to the Emergent Hall Effect.

2016

We present a combined theoretical and experimental study, investigating the origin of the enhanced non-adiabaticity of magnetic vortex cores. Scanning transmission X-ray microscopy is used to image the vortex core gyration dynamically to measure the non-adiabaticity with high precision, including a high confidence upper bound. Using both numerical computations and analytical derivations, we show that the large non-adiabaticity parameter observed experimentally can be explained by the presence of local spin currents arising from a texture-induced emergent Hall effect. This enhanced non-adiabaticity is only present in two- and three-dimensional magnetic textures such as vortices and skyrmions…

Difficult tracheal intubation in neonates and infants. NEonate and Children audiT of Anaesthesia pRactice IN Europe (NECTARINE)

2021

Background: Neonates and infants are susceptible to hypoxaemia in the perioperative period. The aim of this study was to analyse interventions related to anaesthesia tracheal intubations in this European cohort and identify their clinical consequences. Methods: We performed a secondary analysis of tracheal intubations of the European multicentre observational trial (NEonate and Children audiT of Anaesthesia pRactice IN Europe [NECTARINE]) in neonates and small infants with difficult tracheal intubation. The primary endpoint was the incidence of difficult intubation and the related complications. The secondary endpoints were the risk factors for severe hypoxaemia attributed to difficult airw…

Corrigendum to ‘Difficult tracheal intubation in neonates and infants. NEonate and Children audiT of Anaesthesia pRactice IN Europe (NECTARINE):a pro…

2021

The authors regret that errors were present in the above article. On page 1174, in the second paragraph of the Statistical methods section, the second sentence should read as follows: The incidence of difficult intubation was determined including those whose tracheas were already intubated and is reported as a percentage with a 95% exact binomial CI. On page 1175, in the third paragraph of the Statistical methods section ‘mean standardised difference (MSD)’ should read ‘standardised mean difference (SMD)’ The authors would like to apologise for any inconvenience caused.

Morbidity and mortality after anaesthesia in early life:results of the European prospective multicentre observational study, neonate and children aud…

2021

Background: Neonates and infants requiring anaesthesia are at risk of physiological instability and complications, but triggers for peri-anaesthetic interventions and associations with subsequent outcome are unknown. Methods: This prospective, observational study recruited patients up to 60 weeks' postmenstrual age undergoing anaesthesia for surgical or diagnostic procedures from 165 centres in 31 European countries between March 2016 and January 2017. The primary aim was to identify thresholds of pre-determined physiological variables that triggered a medical intervention. The secondary aims were to evaluate morbidities, mortality at 30 and 90 days, or both, and associations with critical …

Time-resolved imaging of pulse-induced magnetization reversal with a microwave assist field

2015

AbstractThe reversal of the magnetization under the influence of a field pulse has been previously predicted to be an incoherent process with several competing phenomena such as domain wall relaxation, spin wave-mediated instability regions and vortex-core mediated reversal dynamics. However, there has been no study on the direct observation of the switching process with the aid of a microwave signal input. We report a time-resolved imaging study of magnetization reversal in patterned magnetic structures under the influence of a field pulse with microwave assistance. The microwave frequency is varied to demonstrate the effect of resonant microwave-assisted switching. We observe that the swi…

Synchronous precessional motion of multiple domain in a ferromagnetic nanowire by perpendicular field pulses

2014

Magnetic storage and logic devices based on magnetic domain wall motion rely on the precise and synchronous displacement of multiple domain walls. The conventional approach using magnetic fields does not allow for the synchronous motion of multiple domains. As an alternative method, synchronous current-induced domain wall motion was studied, but the required high-current densities prevent widespread use in devices. Here we demonstrate a radically different approach: we use out-of-plane magnetic field pulses to move in-plane domains, thus combining field-induced magnetization dynamics with the ability to move neighbouring domain walls in the same direction. Micromagnetic simulations suggest …

Dynamics and topological mass of skyrmionic spin structures (presentation video)

2014

Skyrmions are topologically protected particle-like configurations, with a topological complexity described by their Skyrmion number. In magnetic systems, they have been numerically predicted to exhibit rich dynamics, such as the gyrotropic and breathing modes, dominated by their topology. Recent experimental advances brought their static manipulation well under control. However, their dynamical behaviour is largely unexplored experimentally. In this work, we provide with the first direct observation of eigenmode skyrmion dynamics. In particular, we present dynamical imaging data with high temporal and spatial resolution to demonstrate the GHz gyrotropic mode of a single skyrmion bubble, as…

Direct observation of coherent magnons with suboptical wavelengths in a single crystalline ferrimagnetic insulator

2019

In the field of magnetism, spin waves are a subject of great interest for fundamental and application-oriented research. Time-resolved scanning transmission x-ray microscopy, a technique that allows for direct spin-wave imaging below the optical resolution limit, is usually limited to thin layers deposited on x-ray transparent membranes. Here, the authors report on a preparation routine that makes single-crystalline materials accessible to this powerful technique. The latter is subsequently implemented on the ferrimagnetic insulator yttrium iron garnet, where spin waves down to 100-nm wavelength are observed.

Local control of domain wall dynamics in ferromagnetic rings

2015

Ferromagnetic nanorings are of great interest due to prospective applications in memory and logic devices based on domain wall (DW) motion.1-3A key-prerequisite for their realization is a reproducible domain wall spin structure with a well-controllable wall velocity. We have found that DW propagation in magnetic ring is characterized by non-constant vortex DW velocity even below Walker breakdown4 (as opposed to straight wires). Several studies have been devoted to the optimization of ring reversal on a global scale using out-of plane field5 or flux charges emanating from neighboring rings if placed in close proximity6. However, these methods involve DW pinning and vortex nucleation processe…

Local Domain-Wall Velocity Engineering via Tailored Potential Landscapes in Ferromagnetic Rings

2016

One vein of spintronics research seeks to harness propagating magnetic domain walls for information processing. The authors engineer a potential landscape via local variations in a ring geometry, and image the motion of domain walls in rotating magnetic fields to quantify the contribution of the spatially varying potential to wall dynamics. Domain-wall velocity depends on ring width, being highest where the ring is widest, and such a potential thus could be selected to synchronize velocities and enable applications.

Magnetic states in low-pinning high-anisotropy material nanostructures suitable for dynamic imaging

2013

We present magnetic domain states in a material configuration with high (perpendicular) magnetic anisotropy and particularly low magnetic pinning. This material, a B-doped Co/Pt multilayer configuration, exhibits a strong magnetic contrast in x-ray transmission experiments, making it apt for dynamic imaging with modern synchrotron techniques, providing high spatial and high temporal resolution simultaneously. By analyzing the static spin structures in nanodisks at variable external fields, we show that CoB/Pt multilayers exhibit low enough domain wall pinning to manipulate the domain pattern with weak stimuli and in particular to move domains and domain walls. We demonstrate in a proof-of-p…

Localized domain wall nucleation dynamics in asymmetric ferromagnetic rings revealed by direct time-resolved magnetic imaging

2016

We report time-resolved observations of field-induced domain wall nucleation in asymmetric ferromagnetic rings using single direction field pulses and rotating fields. We show that the asymmetric geometry of a ring allows for controlling the position of nucleation events, when a domain wall is nucleated by a rotating magnetic field. Direct observation by scanning transmission x-ray microscopy (STXM) reveals that the nucleation of domain walls occurs through the creation of transient ripplelike structures. This magnetization state is found to exhibit a surprisingly high reproducibility even at room temperature and we determine the combinations of field strengths and field directions that all…

Skyrmion Hall effect revealed by direct time-resolved X-ray microscopy

2016

Magnetic skyrmions are highly promising candidates for future spintronic applications such as skyrmion racetrack memories and logic devices. They exhibit exotic and complex dynamics governed by topology and are less influenced by defects, such as edge roughness, than conventionally used domain walls. In particular, their finite topological charge leads to a predicted "skyrmion Hall effect", in which current-driven skyrmions acquire a transverse velocity component analogous to charged particles in the conventional Hall effect. Here, we present nanoscale pump-probe imaging that for the first time reveals the real-time dynamics of skyrmions driven by current-induced spin orbit torque (SOT). We…

Direct imaging of high frequency multimode spin wave propagation in cobalt iron waveguides using X ray microscopy beyond 10 GHz

2020

Spin Wave Emission from Vortex Cores under Static Magnetic Bias Fields

2021

We studied the influence of a static in-plane magnetic field on the alternating-field-driven emission of nanoscale spin waves from magnetic vortex cores. Time-resolved scanning transmission X-ray microscopy was used to image spin waves in disk structures of synthetic ferrimagnets and single ferromagnetic layers. For both systems, it was found that an increasing magnetic bias field continuously displaces the wave-emitting vortex core from the center of the disk toward its edge without noticeably altering the spin-wave dispersion relation. In the case of the single-layer disk, an anisotropic lateral expansion of the core occurs at higher magnetic fields, which leads to a directional rather th…

Characterization and differentiation of rock varnish types from different environments by microanalytical techniques

2017

© 2017 Elsevier B.V. We investigated rock varnishes collected from several locations and environments worldwide by a broad range of microanalytical techniques. These techniques were selected to address the challenges posed by the chemical and structural complexity within the micrometer- to nanometer-sized structures in these geological materials. Femtosecond laser ablation-inductively coupled plasma-mass spectrometry (fs LA-ICP-MS), scanning transmission X-ray microscopy-near edge X-ray adsorption fine structure spectroscopy (STXM-NEXAFS) in combination with scanning electron microscopy (SEM) of focused ion beam (FIB) ultra-thin (100–200 nm) sections, conventional and polarization microscop…

Dynamic domain wall chirality rectification by rotating magnetic fields

2015

We report on the observation of magnetic vortex domain wall chirality reversal in ferromagnetic rings that is controlled by the sense of rotation of a magnetic field. We use time-resolved X-ray microscopy to dynamically image the chirality-switching process and perform micromagnetic simulations to deduce the switching details from time-resolved snapshots. We find experimentally that the switching occurs within less than 4 ns and is observed in all samples with ring widths ranging from 0.5 μm to 2 μm, ring diameters between 2 μm and 5 μm, and a thickness of 30 nm, where a vortex domain wall is present in the magnetic onion state of the ring. From the magnetic contrast in the time-resolved im…

Imaging Spin Dynamics on the Nanoscale Using X-Ray Microscopy

2015

The dynamics of emergent magnetic quasiparticles, such as vortices, domain walls and bubbles are studied by scanning transmission X-ray microscopy (STXM), combining magnetic (XMCD) contrast with about 25 nm lateral resolution as well as 70 ps time resolution. Essential progress in the understanding of magnetic vortex dynamics is achieved by vortex core reversal observed by sub-GHz excitation of the vortex gyromode, either by ac magnetic fields or spin transfer torque. The basic switching scheme for this vortex core reversal is the generation of a vortex-antivortex pair. Much faster vortex core reversal is obtained by exciting azimuthal spin wave modes with (multi-GHz) rotating magnetic fiel…

Dynamic domain wall chirality rectification by rotating magnetic fields

2015

RIPHeart (Remote Ischemic Preconditioning for Heart Surgery) Study: Myocardial Dysfunction, Postoperative Neurocognitive Dysfunction, and 1 Year Foll…

2018

Background Remote ischemic preconditioning ( RIPC ) has been suggested to protect against certain forms of organ injury after cardiac surgery. Previously, we reported the main results of RIPHeart (Remote Ischemic Preconditioning for Heart Surgery) Study, a multicenter trial randomizing 1403 cardiac surgery patients receiving either RIPC or sham‐ RIPC . Methods and Results In this follow‐up paper, we present 1‐year follow‐up of the composite primary end point and its individual components (all‐cause mortality, myocardial infarction, stroke and acute renal failure), in a sub‐group of patients, intraoperative myocardial dysfunction assessed by transesophageal echocardiography and the incidenc…