0000000000181537
AUTHOR
G. Sparn
LOCAL-MOMENT AND ITINERANT ANTIFERROMAGNETISM IN THE HEAVY-FERMION SYSTEM CE(CU1-XNIX)2GE2
Elastic and inelastic neutron-scattering studies on the system Ce(Cu1−xNix)2Ge2 are reported. These measurements are complemented by measurements of the magnetic susceptibility, high-field magnetization, heat capacity, thermal expansion, electrical resistivity and thermopower. The results reveal an interesting T-x phase diagram consisting of two different antiferromagnetic phases for x 0.5. Further experimental evidence for different types of antiferromagnetic ordering derives from a line-shape analysis of the quasielastic neutron-scattering intensity, from magnetization and thermopower experiments.
Neutron-scattering studies on CeM2Ge2(M=Ag, Au, and Ru)
The results of elastic, quasielastic, and inelastic neutron-scattering studies on polycrystalline CeM 2 Ge 2 (M=Ag, Au, and Ru) are presented. All compounds reveal long-range magnetic order at low temperatures. Ferromagnetic (M=Ru), antiferromagnetic (M=Au), and incommensurate (M=Ag) structures were detected. Using time-of-flight (TOF) techniques, the crystalline electric-field splittings were determined. With high-resolution TOF experiments the temperature and wave-vector dependence of the magnetic relaxation rate was studied
Alloying experiments on heavy fermion compounds
Abstract This paper is intended to demonstrate the usefulness of controlled alloying for the understanding of heavy-fermion physics: (1) Th-substitution for Ce in CeCu2Si2 emphasizes the dominating role of the dopant-induced strain fields in generating incoherent scattering and pair breaking, (2) replacement of Cu by Ni in Ce(Cu1-xNix)2Ge2 leads to phenomena which are interpreted as derived from a transition between local-moment and itinerant heavy-fermion magnetism, and (3) increasing Cu concentration in UCu4+xAl8-x is accompanied by an antiferromagnetic to nonmagnetic transition near xcr = 1.5 similar to what has been found before for several Ce-based systems. A heavy Fermi-liquid phase w…
Instabilities in heavy-fermion systems
Abstract We review (i) an itinerant antiferromagnetic phase transition below 4 K in Ni-rich Ce(Cu 1− x Ni x ) 2 Ge 2 systems, (ii) the coincidence at T = 0.63 K of both a structural lattice instability in “as-grown” (non-superconducting) CeCu 2 Si 2 single crystals and bulk superconductivity in annealed ones as well as (iii) antiferromagnetic and superconducting transitions at T N = 4.6 K and T c = 1 K, respectively, in the heavy-fermion compound UNi 2 Al 3 .
Alloying-induced transition from local-moment to itinerant heavy fermion magnetism in Ce(Cu1−xNix)2Ge2
Abstract A monotonous increase of the Kondo temperature in Ce(Cu1−xNix)2Ge2 from 7 (x = 0) to 30 K (x = 1) is accompanied by drastic changes of ground state properties: for x⩽0.2, a modulated magnetic structure (q01 = (0.28, 0.28, 0.54)) involving Kondo-reduced local Ce moments ( μ s = 0.74μ B Ce for x = 0) forms below TN1(x). TN1 = 4. 1 K for CeCu2Ge2 is strongly depressed upon increasing x. At x ≲ 0.2, a different modulation develops below TN2(x) which becomes maximum (≃4 K) for x = 0.5. Since this is characterized by a very small value of q02 (=(0, 0, 0.13) at x = 0.5) and a gradually decreasing ordered moment (reaching μs ≲ 0.2μB/Ce for x ⩾0.65), we ascribe it to “heavy fermion band mag…
Magnetic order in the heavy fermion system Ce(Cu1−xNix)2Ge2
Abstract The magnetic phase diagram of the heavy fermion (HF) systems Ce(Cu 1−x Ni x ) 2 Ge 2 is discussed utilizing results of transport, thermodynamic and neutron-scattering measurements. While the Kondo temperature increases monotonically with x, a complex x-dependence is found for the Neel temperature, associated with a transition from local-moment to itinerant HF magnetism.