0000000000184141
AUTHOR
K. Valli
A simple method for filtering pump fluid vapors from circulated helium
Abstract A simple efficient ceramic filter has been introduced for separation of oil vapors from circulated helium. Oil vapors were observed to pass easily through standard cold-trap and zeolite filters. They behave in these filters in the same way as “carrier fragments” behave in the helium-jet recoil-transport method. The significance of this observation is discussed.
Transport of recoil atoms in a stream of liquid-air-cooled pure helium
Abstract Pure commercial helium cooled down to the temperature of liquid air (80 K) has been used for rapid transportation of recoil atoms over distances as long as 10 m. Transport efficiencies of several tens of per cent have been obtained for recoil atoms resulting from alpha decay or from decay by fission. The angle of divergence of the beam of recoil atoms at the exit of the transport capillary is measured to be (11±2)° for particles of mass number A = 211. Experimental results are discussed in terms of thermal diffusion. The elimination of carrier vapors will probably simplify the use of the helium-jet technique in on-line mass separators.
Beta-delayed particle emission of 36K
Abstract 36 Ar targets of 19 μg cm 2 thickness were made by a sandwich technique in which a 70 nm layer of Al was evaporated onto the implanted Al surface between five successive implantations of 36 Ar ions. The sources of 36 K were prepared by depositing the recoil atoms from the 36 Ar(p, n) 36 K reaction by means of a helium jet onto a fast transport tape. The measured delayed particle spectra revealed 11 proton groups (0.5 MeV E p E α 36 K. Total proton and α-particle branching ratios were measured to be 4.8 × 10 −4 and 3 × 10 −5 , respectively. Partial level widths and reduced proton and α-particle transition widths were determined for several individual levels with the aid of additiona…
Ein schnelles on-line trennsystem unter anwendung von helium-jet- und zentrifugentechnik
Abstract A centrifuge for continuous liquid-liquid phase separation is described. It is designed for rapid solvent extraction of short-lived radioactive isotopes (half-lives in the order of seconds). The centrifuge is characterized by simple construction and operation principle, easy handling, low cost, and a minimum hold-up time of less than five seconds (phase purity 99.0–99.9%). The on-line connection to a helium-jet transport system is described. Problems concerning the transfer of activities into a liquid phase from the helium-jet at atmospheric pressure are discussed.
Helium-jet ion guide for an on-line isotope separator
Abstract A new method based on helium-jet techniques permits primary recoil ions produced in radioactive decay or in nuclear reactions to be run directly through a mass separator. Test results with a 227 Ac source give promise of qualities complementary to those obtained with conventional ion sources. This, 69 ± 5 per cent of the recoil particles transported with pure, commercial helium are positive ions, and 66 ± 5 per cent of them are mass separated. Nearly equal efficiencies are expected for most chemical elements and compounds. The mass spectra are remarkably free from groups caused by impurities. The shortest achievable separation time is estimated to be of the order of one millisecond.
The squeezer ion guide
Abstract The properties of an ordinary ion guide can be improved by inserting a grid between the nozzle and the skimmer. When positive ions are transported, an electric potential lower than +10 V is connected to the grid and one of the order of − 10 V to the skimmer. Efficient focusing is achieved between the nozzle and the grid by a combined action of the viscous helium flow field and the weak electric field. The focusing device is called a “squeezer”. It can be extended by adding more grids, a second skimmer, and differential pumping. Contrary to the first grid, the additional elements act more or less like electrostatic lenses in medium vacuum. With the squeezer ion guide, ions created i…
Helium-jet transportation of recoil atoms into a liquid phase
Abstract A rapid inexpensive method has been developed for transportation of recoiling short-lived radioactive nuclides from a target chamber over distances of several meters into a liquid phase. This allows rapid radiochemical separation of different elements. The carrier-loaded helium-jet transport technique is employed without a pumping system. The method would appear to be applicable to most chemical elements. The transport efficiency is higher than 50% and the transport time can be made much shorter than 1 s. Radiochemical separation times of a few seconds were achieved.
Separation of fission products by the ion guide fed isotope separator, IGISOL
Abstract The performance of the ion guide method in the on-line mass separation of fission products has been investigated. Activity was produced by bombarding nat. U targets with a beam of 20 MeV protons. All the mass chains from A = 95 through A = 120 have been scanned using conventional methods of nuclear spectroscopy. No chemical selectivity in the separation was observed; isotopes of highly nonvolatile elements from yttrium to palladium were produced with efficiencies equal to those for the more volatile ones. The boundary of known neutron-rich nuclides was reached throughout the mass region from A = 106 to A = 118. During the course of this preliminary study the new isotope 116 Rh was …
Transport efficiency of the helium-jet recoil-transport method with pure helium
Abstract New techniques have been developed for measuring the transport efficiency of the helium-jet recoil-transport method in the transport of radioactive recoil atoms. The dependence of the transport efficiency on main equipment parameters was studied experimentally using pure commercial-grade helium. The results are given in terms of helium mass throughput, capillary parameters and location of a catcher foil. High to moderate efficiencies were observed at transport distances shorter than 20 cm. Efficiencies obtained with pure helium at distances longer than 1 m are low, typically less than 1%. Possibilities for further development of the method are briefly discussed.
Focusing ions by viscous drag and weak electric fields in an ion guide
Abstract A new special ion guide has one or more grids at low electric potential in the space between nozzle and skimmer. Viscous drag caused by helium flow is used together with weak electric fields for focusing ions through the skimmer. A typical yield through the skimmer is 75% of that through the nozzle. The focusing device is called a “squeezer”. Most properties of the “squeezer ion guide” are similar to those of an ordinary ion guide. Because the kinetic energies are only of the order of 10 eV, however, problems caused by ion scattering are greatly reduced as compared to ordinary ion guides.
A study of a helium-jet ion guide for an on-line isotope separator
Abstract A new method based on helium-jet techniques permits primary recoil ions, produced in radioactive decay or in nuclear reactions to be run directly through a mass separator. Results obtained with a 227 Ac source promise qualities complementary with those obtained with conventional ion sources and indicate an overall efficiency of the order of 10%. Preliminary results with 20 Na recoils from the 20 Ne(p,n)-reaction indicate that most of the ionic species transported out from the target chamber are negatively charged.
The carrier-loaded helium-jet transport method
Abstract The suitability of commercial helium loaded with small amounts of different gases or vapors for the transport of radioactive reaction products over distances of several meters has been investigated experimentally. Negative results were obtained with gaseous carriers. Transport efficiencies of 50 to 100% were obtained with carrier vapors. The vapor appears to form droplets in the system. The recoils are adsorbed physically by the droplets and carried with them through a capillary. There appears to be an active mechanism that forces the heavy constituents to the centre of the capillary cross section. The heavy constituents emerge from the capillary as a very narrow beam. Collection o…
Efficiency of an on-line isotope separator system employing cooled and NaCl-loaded He-jet methods
Abstract A pure helium-jet at liquid nitrogen temperature coupled to a Nielsen type ion source, and a NaCl-loaded helium-jet coupled to a hollow-cathode ion source have been investigated as means to connect a cyclotron target chamber on-line to a mass separator. Technical details and performances of some critical parts of the system are described. Total separation efficiencies measured under various experimental conditions for several nuclides vary between 0.01 and 1.0%.
Collinear fast atomic-beam laser spectroscopy at riken garis/igisol
We have constructed a fast atomic-beam collinear laser spectroscopy system connected to the on-line isotope separator facility GARIS/IGISOL at RIKEN. This system is potentially powerful in studying refractory elements. To test the system, an off-line collinear experiment was made on stable Hf isotopes produced by means of laser ablation technique. For production of radioactive Hf isotopes, the use of the inverse kinematics of a fusion reaction,9Be(166Er,xn)175-xHf, was investigated. The radioactive isotope169Hf was successfully extracted from GARIS/IGISOL and accelerated up to 30 keV.
Velocity distribution of ion beams from the RIKEN IGISOL
Abstract A direct measurement of the velocity distribution of ion beams from an ion-guide isotope separator on-line (IGISOL) was carried out at RIKEN with a technique of laser spectroscopy. The skimmer-potential and gas-cell pressure dependence of the velocity distribution were also measured. The velocity distribution was found to be about two times narrower than that estimated from the mass resolving power (MRP). It is pointed out that the velocity spread deduced from MRP is considerably overestimated at various conditions. The way of improvement to make the velocity distribution of the ion beam from the IGISOL narrower and the feasibility of fast atomic-beam collinear laser spectroscopy a…