Laser and decay spectroscopy of the short-lived isotope Fr214 in the vicinity of the N=126 shell closure

High-resolution laser spectroscopy with the Collinear Resonance Ionisation Spectroscopy (CRIS) experiment at CERN-ISOLDE

The Collinear Resonance Ionisation Spectroscopy (CRIS) experiment at CERN has achieved high-resolution resonance ionisation laser spectroscopy with a full width at half maximum linewidth of 20(1) MHz for 219;221Fr, and has measured isotopes as short lived as 5 ms with 214Fr. This development allows for greater precision in the study of hyperfine structures and isotope shifts, as well as a higher selectivity of singleisotope, even single-isomer, beams. These achievements are linked with the development of a new laser laboratory and new data-acquisition systems. publisher: Elsevier articletitle: High-resolution laser spectroscopy with the Collinear Resonance Ionisation Spectroscopy (CRIS) exp…

Resonance laser ionization spectroscopy of tellurium

Abstract Resonance ionization schemes for tellurium are investigated with a resonance ionization laser ion source and Ti:Sapphire lasers for fundamental research applications. We present the first three-step resonance ionization spectra of atomic Te. Several autoionizing Rydberg series converging to the first excited state of Te+ are observed and assigned to 5p3 (2Do3/2) ns and nd configurations. Our results include confirmation and significant expansion of the Rydberg series previously reported as well as observation of three new series. From the series convergence limits the ionization potential of tellurium is revised to be 72,669.006(42)stat(20)sys cm−1.

Combined high-resolution laser spectroscopy and nuclear decay spectroscopy for the study of the low-lying states inFr206,At202, andBi198

High-resolution laser spectroscopy was performed on $^{206}\mathrm{Fr}$ with the collinear resonance ionization spectroscopy (CRIS) experiment at CERN-ISOLDE. The hyperfine structure and isotope shift of the ground, first isomeric and second isomeric states were measured. The hyperfine components were unambiguously assigned to each nuclear state by means of laser-assisted nuclear decay spectroscopy. The branching ratios in the $\ensuremath{\alpha}$ decay of $^{206}\mathrm{Fr}$ and $^{202}\mathrm{At}$ were also measured for the first time with isomerically purified beams. The extracted hindrance factors allow determination of the spin of the ground, first isomeric, and second isomeric states…

Use of a Continuous Wave Laser and Pockels Cell for Sensitive High-Resolution Collinear Resonance Ionization Spectroscopy

New technical developments have led to a 2 orders of magnitude improvement of the resolution of the collinear resonance ionization spectroscopy (CRIS) experiment at ISOLDE, CERN, without sacrificing the high efficiency of the CRIS technique. Experimental linewidths of 20(1) MHz were obtained on radioactive beams of francium, allowing us for the first time to determine the electric quadrupole moment of the short lived [t1/2=22.0(5) ms]219Fr Qs=−1.21(2) eb, which would not have been possible without the advantages offered by the new method. This method relies on a continuous-wave laser and an external Pockels cell to produce narrow-band light pulses, required to reach the high resolution in t…

Rydberg and autoionizing states of tellurium studied by laser resonance ionization spectroscopy

Multistep laser-resonance-ionization spectroscopy of tellurium (Te) has been performed at TRIUMF's off-line laser ion source test stand. Six clean and regular even-parity Rydberg series $5{p}^{3}$ $({^{4}S}_{3/2}^{\ensuremath{\circ}})$ $np\phantom{\rule{4pt}{0ex}}^{3}P_{0,1,2}$, $np\phantom{\rule{4pt}{0ex}}^{5}P_{1,2}$, and $nf\phantom{\rule{4pt}{0ex}}^{3}F_{2}/^{5}F_{1,2}$ were observed. The ionization potential of Te was extracted from the measured series as $72669.114{(56)}_{\mathrm{stat}}{(45)}_{\mathrm{sys}}\phantom{\rule{4pt}{0ex}}{\mathrm{cm}}^{\ensuremath{-}1}$. Excited from two different intermediate levels, seven odd-parity autoionization Rydberg series converging to the $5{s}^{2}…