0000000000208186
AUTHOR
M. B. Gómez-hornillos
New measurement of the 242Pu(n,γ) cross section at n-TOF-EAR1 for MOX fuels: Preliminary results in the RRR
The spent fuel of current nuclear reactors contains fissile plutonium isotopes that can be combined with 238U to make mixed oxide (MOX) fuel. In this way the Pu from spent fuel is used in a new reactor cycle, contributing to the long-term sustainability of nuclear energy. The use of MOX fuels in thermal and fast reactors requires accurate capture and fission cross sections. For the particular case of 242Pu, the previous neutron capture cross section measurements were made in the 70’s, providing an uncertainty of about 35% in the keV region. In this context, the Nuclear Energy Agency recommends in its “High Priority Request List” and its report WPEC-26 that the capture cross section of 242Pu…
First Measurement of Severalβ-Delayed Neutron Emitting Isotopes BeyondN=126
The β-delayed neutron emission probabilities of neutron rich Hg and Tl nuclei have been measured together with β-decay half-lives for 20 isotopes of Au, Hg, Tl, Pb, and Bi in the mass region N≳126. These are the heaviest species where neutron emission has been observed so far. These measurements provide key information to evaluate the performance of nuclear microscopic and phenomenological models in reproducing the high-energy part of the β-decay strength distribution. This provides important constraints on global theoretical models currently used in r-process nucleosynthesis.
GEANT4 simulation of the neutron background of the C6D6 set-up for capture studies at n_TOF
The neutron sensitivity of the C6D6 detector setup used at n_TOF facility for capture measurements has been studied by means of detailed GEANT4 simulations. A realistic software replica of the entire n_TOF experimental hall, including the neutron beam line, sample, detector supports and the walls of the experimental area has beeni mplemented in the simulations. The simulations have been analyzed in the same manner as experimental data, in particular by applying the Pulse Height Weighting Technique. The simulations have been validated against a measurement of the neutron background performed with anatC sample, showing an excellent agreement above 1 keV. At lower energies, an additional compo…
Total Absorption Spectroscopy of Fission Fragments Relevant for Reactor Antineutrino Spectra and Decay Heat Calculations
Volume: 111 Host publication title: WONDER-2015 Host publication sub-title: 4TH INTERNATIONAL WORKSHOP ON NUCLEAR DATA EVALUATION FOR REACTOR APPLICATIONS Isbn(print): 978-2-7598-1970-6 Beta decay of fission products is at the origin of decay heat and antineutrino emission in nuclear reactors. Decay heat represents about 7% of the reactor power during operation and strongly impacts reactor safety. Reactor antineutrino detection is used in several fundamental neutrino physics experiments and it can also be used for reactor monitoring and non-proliferation purposes. Rb-92,Rb-93 are two fission products of importance in reactor antineutrino spectra and decay heat, but their beta-decay properti…
Gamma/neutron competition above the neutron separation energy in delayed neutron emitters
To study the β-decay properties of some well known delayed neutron emitters an experiment was performed in 2009 at the IGISOL facility (University of Jyvaskyla in Finland) using Total Absorption -ray Spectroscopy (TAGS) technique. The aim of these measurements is to obtain the full β-strength distribution below the neutron separation energy (Sn) and the γ/neutron competition above. This information is a key parameter in nuclear technology applications as well as in nuclear astrophysics and nuclear structure. Preliminary results of the analysis show a significant γ-branching ratio above Sn. © Owned by the authors, published by EDP Sciences, 2014.
Total absorption spectroscopy of fission fragments relevant for reactor antineutrino spectra
International audience; The accurate determination of reactor antineutrino spectra remains a very active research topic for which new methods of study have emerged in recent years. Indeed, following the long-recognized reactor anomaly (measured antineutrino deficit in short baseline reactor experiments when compared with spectral predictions), the three international reactor neutrino experiments Double Chooz, Daya Bay and Reno have recently demonstrated the existence of spectral distortions in their measurements with respect to the same predictions. These spectral predictions were obtained through the conversion of integral beta-energy spectra obtained at the ILL research reactor. Several s…
Characterization of a neutron-beta counting system with beta-delayed neutron emitters
Abstract A new detection system for the measurement of beta-delayed neutron emission probabilities has been characterized using fission products with well known β-delayed neutron emission properties. The setup consists of BELEN-20, a 4π neutron counter with twenty 3He proportional tubes arranged inside a large polyethylene neutron moderator, a thin Si detector for β counting and a self-triggering digital data acquisition system. The use of delayed-neutron precursors with different neutron emission windows allowed the study of the effect of energy dependency on neutron, β and β–neutron rates. The observed effect is well reproduced by Monte Carlo simulations. The impact of this dependency on …
Total absorption γ-ray spectroscopy of beta delayed neutron emitters
Preliminary results of the data analysis of the beta decay of 94Rb using a novel - segmented- total absorption spectrometer are shown in this contribution. This result is part of a systematic study of important contributors to the decay heat problem in nuclear reactors. In this particular case the goal is to determine the beta intensity distribution below the neutron separation energy and the gamma/beta competition above.
Spectroscopic factor and proton formation probability for the d3/2 proton emitter 151Lu
The quenching of the experimental spectroscopic factor for proton emission from the short-lived $d_{3/2}$ isomeric state in $^{151m}$Lu was a long-standing problem. In the present work, proton emission from this isomer has been reinvestigated in an experiment at the Accelerator Laboratory of the University of Jyv\"{a}skyl\"{a}. The proton-decay energy and half-life of this isomer were measured to be 1295(5) keV and 15.4(8) $\mu$s, respectively, in agreement with another recent study. These new experimental data can resolve the discrepancy in the spectroscopic factor calculated using the spherical WKB approximation. Using the R-matrix approach it is found that the proton formation probabilit…
Total Absorption Study of Beta Decays Relevant for Nuclear Applications and Nuclear Structure
Abstract An overview is given of our activities related to the study of the beta decay of neutron rich nuclei relevant for nuclear applications. Recent results of the study of the beta decay of 87,88 Br using a new segmented total absorption spectrometer are presented. The measurements were performed at the IGISOL facility using trap-assisted total absorption spectroscopy.
New Beta-delayed Neutron Measurements in the Light-mass Fission Group
A new accurate determination of beta-delayed neutron emission probabilities from nuclei in the low mass region of the light fission group has been performed. The measurements were carried out using the BELEN 4π neutron counter at the IGISOL-JYFL mass separator in combination with a Penning trap. The new results significantly improve the uncertainties of neutron emission probabilities for {sup 91}Br, {sup 86}As, {sup 85}As, and {sup 85}Ge nuclei.
Total Absorption Spectroscopy of Fission Fragments Relevant for Reactor Antineutrino Spectra Determination
8 pags., 3 figs., 1 tab. ; Presented at the XXXIV Mazurian Lakes Conference on Physics, Piaski, Poland, September 6–13, 2015.
β -decay half-lives and β -delayed neutron emission probabilities for several isotopes of Au, Hg, Tl, Pb, and Bi, beyond N=126
Background: Previous measurements of Beta-delayed neutron emitters comprise around 230 nuclei, spanning from the 8He up to 150La. Apart from 210Tl, with a minuscule branching ratio of 0.07%, no other neutron emitter is measured yet beyond A = 150. Therefore new data are needed, particularly in the heavy mass region around N=126, in order to guide theoretical models and to understand the formation of the third r-process peak at A 195. Purpose: To measure both, Beta-decay half-lives and neutron branching ratios of several neutron-rich Au, Hg, Tl, Pb and Bi isotopes beyond N = 126. Method: Ions of interest are produced by fragmentation of a 238U beam, selected and identifed via the GSI-FRS fra…
The 236U neutron capture cross-section measured at the n TOF CERN facility
International audience; The $^{236}$U isotope plays an important role in nuclear systems, both for future and currently operating ones. The actual knowledge of the capture reaction of this isotope is satisfactory in the thermal region, but it is considered insufficient for Fast Reactor and ADS applications. For this reason the $^{236} \text{U}(n, \gamma)$ reaction cross-section has been measured for the first time in the whole energy region from thermal energy up to 1 MeV at the n_TOF facility with two different detection systems: an array of C$_6$D$_6$ detectors, employing the total energy deposited method, and a 4$\pi$ total absorption calorimeter (TAC), made of 40 BaF$_2$ crystals. The t…
High precision measurement of the radiative capture cross section of 238U at the n_TOF CERN facility
The importance of improving the accuracy on the capture cross-section of 238U has been addressed by the Nuclear Energy Agency, since its uncertainty significantly affects the uncertainties of key design parameters for both fast and thermal nuclear reactors. Within the 7th framework programme ANDES of the European Commission three different measurements have been carried out with the aim of providing the 238U(n,γ) cross-section with an accuracy which varies from 1 to 5%, depending on the energy range. Hereby the final results of the measurement performed at the n-TOF CERN facility in a wide energy range from 1 eV to 700 keV will be presented. © The Authors, published by EDP Sciences, 2017.
Total Absorption Spectroscopy Study ofRb92Decay: A Major Contributor to Reactor Antineutrino Spectrum Shape
The antineutrino spectra measured in recent experiments at reactors are inconsistent with calculations based on the conversion of integral beta spectra recorded at the ILL reactor. (92)Rb makes the dominant contribution to the reactor antineutrino spectrum in the 5-8 MeV range but its decay properties are in question. We have studied (92)Rb decay with total absorption spectroscopy. Previously unobserved beta feeding was seen in the 4.5-5.5 region and the GS to GS feeding was found to be 87.5(25)%. The impact on the reactor antineutrino spectra calculated with the summation method is shown and discussed.
Fission fragment angular distribution of 232Th(n,f) at the CERN n TOF facility
The angular distribution of fragments emitted in neutron-induced fission of 232Th was measured in the white spectrum neutron beam at the n_TOF facility at CERN. A reaction chamber based on Parallel Plate Avalanche Counters (PPAC) was used, where the detectors and the targets have been tilted 45 degrees with respect to the neutron beam direction in order to cover the full angular range of the fission fragments. A GEANT4 simulation has been developed to study the setup efficiency. The data analysis and the preliminary results obtained for the 232Th(n,f) between fission threshold and 100 MeV are presented here.
Direct mass measurements ofSe68andY80
The masses of neutron-deficient nuclides near the $N=Z$ line with $A=64\text{\ensuremath{-}}80$ have been determined using a direct time-of-flight technique which employed a cyclotron as a high-resolution spectrometer. The measured atomic masses for $^{68}\mathrm{Se}$ and $^{80}\mathrm{Y}$ were 67.9421(3) u and 79.9344(2) u, respectively. The new values agree with the 2003 Atomic Mass Evaluation. The result for $^{68}\mathrm{Se}$ confirms that this nucleus is a waiting point of the rp-process, and that for $^{80}\mathrm{Y}$ resolves the conflict between earlier measurements. Using the present results and the 2003 Atomic Mass Evaluation compilation, the empirical interaction between the last…
β-delayed neutron emission measurements around the third r-process abundance peak
This contribution summarizes an experiment performed at GSI (Germany) in the neutron-rich region beyond N=126. The aim of this measurement is to provide the nuclear physics input of relevance for r-process model calculations, aiming at a better understanding of the third r-process abundance peak. Many exotic nuclei were measured around 211Hg and 215Tl. Final ion identification diagrams are given in this contribution. For most of them, we expect to derive halflives and and β-delayed neutron emission probabilities. The detectors used in this experiment were the Silicon IMplantation and Beta Absorber (SIMBA) detector, based on an array of highly segmented silicon detectors, and the BEta deLayE…
Measurement of the 241Am neutron capture cross section at the n-TOF facility at CERN
New neutron cross section measurements of minor actinides have been performed recently in order to reduce the uncertainties in the evaluated data, which is important for the design of advanced nuclear reactors and, in particular, for determining their performance in the transmutation of nuclear waste. We have measured the 241 Am(n,γ) cross section at the n TOF facility between 0.2 eV and 10 keV with a BaF2 Total Absorption Calorimeter, and the analysis of the measurement has been recently concluded. Our results are in reasonable agreement below 20 eV with the ones published by C. Lampoudis et al. in 2013, who reported a 22% larger capture cross section up to 110 eV compared to experimental …
β-decay and β-delayed Neutron Emission Measurements at GSI-FRS Beyond N=126, for r-process Nucleosynthesis
New measurements of very exotic nuclei in the neutron-rich region beyond N=126 have been performed at the GSI facility with the fragment separator (FRS). The aim of the experiment is to determine half-lives and β-delayed neutron emission branching ratios of isotopes of Hg, Tl and Pb in this region. This contribution summarizes final counting statistics for identification and for implantation, as well as the present status of the data analysis of the half-lives. In summary, isotopes of Pt, Au, Hg, Tl, Pb, Bi, Po, At, Rn and Fr were clearly identified and several of them (208-211Hg, 211-215Tl, 214-218Pb) were implanted with enough statistics to determine their half-lives. About half of them a…
Collective excitations in the transitional nuclei 163Re and 165Re
Excited states in the neutron-deficient nuclei 163 75 Re88 and 165 75 Re90 were populated in the 106Cd(60Ni, p2nγ ) and 92Mo(78Kr, 3p2nγ ) fusion-evaporation reactions at bombarding energies of 270 and 380 MeV, respectively. γ rays were detected at the target position using the JUROGAM spectrometer while recoiling ions were separated in-flight by the RITU gas-filled recoil separator and implanted in the GREAT spectrometer. The energy level schemes for 163Re and 165Re were identified using recoil-decay correlation techniques. At low spin, the yrast bands of these isotopes consist of signature partner bands based on a single πh11/2 quasiproton configuration. The bands display large energy spl…