0000000000288919
AUTHOR
D. Sugny
Simultaneous field-free molecular orientation and planar delocalization by THz laser pulses
This study shows the unexpected and counter-intuitive possibility of simultaneously orienting a molecule while delocalizing its molecular axis in a plane in field-free conditions. The corresponding quantum states are characterized and different control strategies using shaped THz laser pulses are proposed to reach such states at zero and nonzero temperatures. The robustness against temperature effects of a simple control procedure combining a laser and a THz pulse is shown. Such control strategies can be applied not only to linear molecules but also to symmetric top molecules.
Signatures of physical constraints in rotating rigid bodies
We study signatures of physical constraints on free rotations of rigid bodies. We show analytically that the physical or non-physical nature of the moments of inertia of a system can be detected by qualitative changes both in the Montgomery Phase and in the Tennis Racket Effect.
Robust quantum control by shaped pulse
Considering the problem of the control of a two-state quantum system by an external field, we establish a general and versatile method that allows the derivation of smooth pulses, suitable for ultrafast applications, that feature the properties of high-fidelity, robustness, and low area. Such shaped pulses can be viewed as a single-shot generalization of the composite pulse technique with a time-dependent phase.