0000000000299319
AUTHOR
P. Taskinen
Collective structure of the neutron-rich nuclei, 110Ru and 112Ru
Abstract The collective structure of 110 Ru and 112 Ru has been studied at the IGISOL facility through the beta decay of 110 Tc and 112 Tc. Neutron-rich technetium isotopes were produced by the 238 U(p, f) reaction at 20 MeV bombarding energy. The new isotope 112 Tc was found to decay with a half-life of 280(30) ms. The observed energies of the 2 + and 4 + ground state band levels in 108,110,112 Ru are almost the same. However, a steady energy decrease of the proposed gamma band head is observed with increasing neutron number, suggesting importance of triaxiality in these nuclei. In fact, only in 192 Os the second 2 + state has been observed at lower excitation than in 112 Ru. The static de…
Discovery of New Fission Product Activities in the A=110–118 Mass Region
Neutron rich nuclei around the mass A=100 have recently attracted both theoretical and experimental interest since they are expected to form a new region of strong deformation. In contrary, very little experimental information is available in the adjacent transitional region A= 110–118. Due to expected isomerism in this region both low and high spin states can be studied via beta decay in many nuclei. The studies of these nuclides have many experimental difficulties. They are only weakly produced in thermal neutron induced fission and because all the elements in this mass region (Tc, Ru, Rh, Pd) have very high melting points they have not been available as beams of on-line isotope separator…
Separation of fission products by the ion guide fed isotope separator, IGISOL
Abstract The performance of the ion guide method in the on-line mass separation of fission products has been investigated. Activity was produced by bombarding nat. U targets with a beam of 20 MeV protons. All the mass chains from A = 95 through A = 120 have been scanned using conventional methods of nuclear spectroscopy. No chemical selectivity in the separation was observed; isotopes of highly nonvolatile elements from yttrium to palladium were produced with efficiencies equal to those for the more volatile ones. The boundary of known neutron-rich nuclides was reached throughout the mass region from A = 106 to A = 118. During the course of this preliminary study the new isotope 116 Rh was …
Studies of Weak Beta-Delayed Protons Emitted in the Decay of Odd-Z, Tz = -3/2 Nuclei
Radioactive decay of Tz = - 3/2 nuclides, 27P and 31Cl, predicted to be weak β-delayed proton precursors, have been looked for. Two proton groups having energies of 989 ± 15 and 1528 ± 20 keV and a half-life of 150 ± 25 ms were associated with the decay of 31Cl. The search for 27P is still under way, but the first qualitative results are briefly discussed.
Submillisecond On-Line Mass Separation of Nonvolatile Radioactive Elements: An Application of Charge Exchange and Thermalization Processes of Primary Recoil Ions in Helium
Transportation of thermalized primary recoil ions from nuclear reactions by helium flow has been investigated as a means of injecting short-lived radioactive nuclides into an on-line isotope separator. Several short-lived radioactive isotopes of highly nonvolatile elements such as B, Sc, Nb, and W have been separated. The efficiency for heavy nuclides with half-lives above 1 ms is between 1 and 10%. The shortest-lived activity identified in an on-line separation is the 182-\ensuremath{\mu}s isomeric state in $^{207}\mathrm{Bi}$.
First observation of the beta decay of117Pd and the discovery of a new isotope119Pd
In this paper we wish to report the first direct observations of the beta decays of117Pd and of a new isotope119Pd. The measuredβ-half-life is 4.3±0.3 s for117Pd. For119Pd, the existence of two beta-decaying states with the same half-life but of opposite parity cannot be excluded. The measured half-life for119Pd is 0.92±0.13 s. The observed beta half-lifes are in good agreement with the QRPA predictions. The observed level structure of117Ag and119Ag are discussed in the frame of the level systematics of the known odd Ag isotopes closer to stability.
Half-life and configuration of the 1/2+ intruder state in203Bi
The decay properties of theJπ=1/2+,Eexc=1,098 keV state in203Bi were studied. The state was populated via the204Pb(p, 2n) reaction and the activity was studied with the ion guide isotope separator on-line system IGISOL. The half-life of the 1/2+ state was measured to beT1/2=303 ±5 ms. From this value the partial half-lives of the three depopulating branches 1/2+ →7/2− (E3), 1/2+→5/2− (E3 +M2) and 1/2+→9/2 g.s. − (M4) were deduced. Since all the transitions are configuration forbidden in first order, a detailed study of second-order shell-model configuration mixing could be performed.
Half-life measurements for neutron-rich Tc, Ru, Rh, and Pd isotopes. Identification of the new isotopesTc111,Ru113, andRh113
The decays of three new neutron-rich nuclides $^{111}\mathrm{Tc}$, $^{113}\mathrm{Ru}$, and $^{113}\mathrm{Rh}$ have been observed at an on-line isotope separator facility. In addition, the beta decays of several other n-rich isotopes with Ag100 have been studied for the first time. The new half-lives reported in this work include: $^{111}\mathrm{Tc}$ [${T}_{1/2}$=0.30(3) s], $^{111}\mathrm{Ru}$ [2.12(7) s], $^{112}\mathrm{Ru}$ [1.75(7) s], $^{113}\mathrm{Ru}$ [0.80(10) s], $^{113}\mathrm{Rh}$ [2.72(22) s], and $^{118}\mathrm{Pd}$ [2.24(17) s]. In general, these results support the microscopic theoretical half-life predictions below Z=50.
New Neutron-Rich Nuclei and Isomers Produced in Symmetric Fisson
The novel method for rapid on-line mass separation, the IGISOL, is described. The method has been shown applicable to mass separation of short-lived proton-induced fission products without any chemical dependence on radionuclide. Recent results on isomeric states with half-lives of the order of milliseconds produced directly in proton-induced fission of 238U and separated with the IGISOL are presented. The future plans for connection of the new K-130 cyclotron of the University of Jyvaskyla with the IGISOL are reviewed.
Gamow-Teller decay of118Pd and of neighbouring even isotopes of palladium
Neutron-rich isotopes of palladium were produced via the fission of238U by 20 MeV protons. These isotopes were selected using the ion guide-fed on-line mass-separator facility IGISOL at Jyvaskyla. Their decays were studied byβ-ray,γ-ray and conversion-electron spectroscopy. For114Pd and116Pd, the decay schemes established previously were confirmed; additionally multipolarities were determined for a few transitions. In the case of118Pd, only an approximate half-life was known from a previous radiochemical experiment. In the present study, 15 gamma transitions were observed, most of which were placed in a decay scheme. The half-life and the decay energy were found to beT1/2=1.9±0.1 s andQβ=4.…
Spin-flip? ? decay of even-even deformed nuclei110Ru and112Ru
Neutron-rich nuclides110Ru and112Ru produced in symmetric fission of238U by 20 MeV protons have been studied at the IGISOL facility by means ofβ-ray,γ-ray and conversion electron spectroscopy. A total of 12 and 6γ-transitions were observed in the decays of110Ru and112Ru, respectively. Multipolarities were determined for a few transitions. The beta decay half-life was determined to be 11.6±0.6 s for110Ru and 1.75±0.07 s for112Ru. As a side product, a new value of 2.1±0.3 s for theβ half-life of the112Rh 1+ state was obtained. The decay energy measured with the plastic scintillator was 2.81 ±0.05 MeV for110Ru and 4.52 ±0.08 MeV for112Ru. The beta decay schemes of110Ru and112Ru isotopes indica…
Gamow-Teller Beta Decay of Neutron Rich Tc, Ru, Rh and Pd Isotopes
During recent experiments at the IGISOL-facility several new neutron rich nuclides have been discovered, including the first direct observations of the beta decays of 111Tc, 112Ru, 113Ru, 114Ru, 113Rh, 115Rh, 116Rh and 118Pd. The role of the νg7/2 → πg9/2 transformation in the beta decays of the odd-odd 110–116Rh and the even-even 114–118Pd isotopes is shown to be dominant. The experimental results are compared with shell model calculations including deformation and pairing.