0000000000315717

AUTHOR

Zhiyong Qin

showing 3 related works from this author

Cross section limits for theCm248(Mg25,4n−5n)Hs268,269reactions

2009

We report on an attempt to produce and detect $^{268}\mathrm{Hs}$ and $^{269}\mathrm{Hs}$ in the nuclear fusion reaction $^{25}\mathrm{Mg}+^{248}\mathrm{Cm}$ using the gas phase chemistry apparatus COMPACT. No decay chains attributable to the decay of hassium isotopes were observed during the course of this experiment. From the nonobservation of $^{269}\mathrm{Hs}$ we derive a cross section limit of 0.4 pb (63% confidence limit) for the reaction $^{248}\mathrm{Cm}(^{25}\mathrm{Mg},4n)^{269}\mathrm{Hs}$ at a center-of-target beam energy of 140 MeV. The evaluated cross section limit for the $^{248}\mathrm{Cm}(^{25}\mathrm{Mg},5n)^{268}\mathrm{Hs}$ reaction depends on the assumed half-life of …

PhysicsNuclear and High Energy PhysicsCross section (physics)chemistryFissionAnalytical chemistrychemistry.chemical_elementNuclear fusionAlpha decayBeam energyHassiumGas phasePhysical Review C
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Decomposition studies of group 6 hexacarbonyl complexes. Part 1: Production and decomposition of Mo(CO)6 and W(CO)6

2015

Abstract Chemical studies of superheavy elements require fast and efficient techniques, due to short half-lives and low production rates of the investigated nuclides. Here, we advocate for using a tubular flow reactor for assessing the thermal stability of the Sg carbonyl complex – Sg(CO)6. The experimental setup was tested with Mo and W carbonyl complexes, as their properties are established and supported by theoretical predictions. The suggested approach proved to be effective in discriminating between the thermal stabilities of Mo(CO)6 and W(CO)6. Therefore, an experimental verification of the predicted Sg–CO bond dissociation energy seems to be feasible by applying this technique. By in…

Inorganic chemistryMetal carbonyl02 engineering and technology010402 general chemistry01 natural sciences7. Clean energythermal stability540 ChemistryseaborgiumThermal stabilityNuclideGas compositionPhysical and Theoretical Chemistrycarbonyl complexegroup 6ChemistrytransactinideTransition metals021001 nanoscience & nanotechnologyDecompositionBond-dissociation energy0104 chemical sciencesVolumetric flow rateYield (chemistry)570 Life sciences; biologyPhysical chemistry0210 nano-technology
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Observation of the3nEvaporation Channel in the Complete Hot-Fusion ReactionMg26+Cm248Leading to the New Superheavy NuclideHs271

2008

The analysis of a large body of heavy ion fusion reaction data with medium-heavy projectiles ($6\ensuremath{\le}Z\ensuremath{\le}18$) and actinide targets suggests a disappearance of the $3n$ exit channel with increasing atomic number of the projectile. Here, we report a measurement of the excitation function of the reaction $^{248}\mathrm{Cm}(^{26}\mathrm{Mg},xn)^{274\mathrm{\text{\ensuremath{-}}}x}\mathrm{Hs}$ and the observation of the new nuclide $^{271}\mathrm{Hs}$ produced in the $3n$ evaporation channel at a beam energy well below the Bass fusion barrier with a cross section comparable to the maxima of the $4n$ and $5n$ channels. This indicates the possible discovery of new neutron-r…

Excitation functionPhysicsNuclear TheoryGeneral Physics and AstronomyTransactinide elementNuclear fusionNeutronNuclideActinideAlpha decayAtomic numberAtomic physicsNuclear ExperimentPhysical Review Letters
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