0000000000315900
AUTHOR
Gregory A. Wurtz
Ultrafast hybrid plasmonics
Abstract We review our recent studies of electromagnetic coupling and associated temporal dynamics of molecular excitations with plasmonic resonances supported by either localized or extended planar geometries. We focus on coherent interactions between plasmon resonances and molecular excitations, which are experimentally challenging due to the very short (∼10–100 fs) coherence times of plasmons. Recent experimental results and theoretical analysis for observing and controlling coherences between molecular excitations and plasmonic polarizations are shown. Advances will explore new directions in ultrafast coherent control of molecular excited states and energy dissipation processes, as well…
Non-Linear Optical Properties of Hybridized Surface Plasmon Polaritonic Crystals: Observation of Optical Bistability
Summary form only given. The use of surface plasmons (SP) is recognized as being central to the development of nanoscale assemblies of photonic and opto-electronic devices. This is motivated by the spatially confined nature of these electromagnetic waves as well as their resonant behavior. Amongst plasmonic supporting structures, surface plasmonic crystals (SPCs) draw particular interest because of their tailored optical properties. A geometry common to SPCs consists in a periodic arrangement of holes or slits in a metal film. Their complex optical response is then governed by coherent interactions between Bloch modes at the film's interfaces and modes supported by the holes or slits. These…