0000000000342233

AUTHOR

Richard G. Haire

showing 3 related works from this author

First Observation of Atomic Levels for the Element Fermium (Z=100)

2003

The atomic level structure of the element fermium was investigated for the first time using a sample of $2.7\ifmmode\times\else\texttimes\fi{}{10}^{10}$ atoms of the isotope $^{255}\mathrm{F}\mathrm{m}$ with a half-life of 20.1 h. The atoms were evaporated from a filament and stored in the argon buffer gas of an optical cell. Atomic levels were sought by the method of resonance ionization spectroscopy using an excimer-dye-laser combination. Two atomic levels were found at wave numbers $(25\text{ }099.8\ifmmode\pm\else\textpm\fi{}0.2)$ and $(25\text{ }111.8\ifmmode\pm\else\textpm\fi{}0.2)\text{ }\text{ }{\mathrm{c}\mathrm{m}}^{\ensuremath{-}1}$. Partial transition rates to the $5{f}^{12}7{s}…

PhysicschemistryFermiumResonance ionizationSaturation (graph theory)General Physics and Astronomychemistry.chemical_elementAtomic physicsGround stateSpectroscopyPhysical Review Letters
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First Determination of the Ionization Potential of Actinium and First Observation of Optical Transitions in Ferminm

2002

For the determination of the first ionization potential of actinium, 227Ac was electrodeposited on a Ta backing and covered with ~1 μm Zr. From this filament, Ac atoms were evaporated at ≥ 1250 °C. By resonant excitation with UV light of 388.67 nm and subsequent excitation with light of ca. 568 nm, Ac was ionized in an external electrical field. By determining the ionization thresholds as a function of the electrical field strength and by extrapolation to zero field strength, the first ionization potential of 43398(3) cm−1 = 5.3807(3) eV was measured.About 1 ng of 255Fm, half life 20.1 h, was prepared at ORNL by milking from 255Es produced in the High Flux Isotope Reactor and shipped to Mai…

Nuclear and High Energy PhysicsChemistryBuffer gasAnalytical chemistryThermal ionizationchemistry.chemical_elementIonActiniumNuclear Energy and EngineeringExcited stateIonizationAtomic physicsIonization energyExcitationJournal of Nuclear Science and Technology
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Resonance ionization spectroscopy of fermium (Z=100)

2003

Laser spectroscopy has been applied for the first time to measure resonant transition frequencies of fermium (Zs 100). A number of 2.7=10 atoms was electrodeposited on a Ta filament and covered with a 1 mm Ti layer. Fm 10

ChemistryFermiumBuffer gasAnalytical chemistrychemistry.chemical_elementPhotoionizationActinideAtomic and Molecular Physics and OpticsAnalytical ChemistryProtein filamentIonizationAtomic physicsSpectroscopyAbsorption (electromagnetic radiation)InstrumentationSpectroscopySpectrochimica Acta Part B: Atomic Spectroscopy
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