0000000000376492
AUTHOR
Calem Hoffman
Superallowed α Decay to Doubly Magic Sn100
We report the first observation of the ^{108}Xe→^{104}Te→^{100}Sn α-decay chain. The α emitters, ^{108}Xe [E_{α}=4.4(2) MeV, T_{1/2}=58_{-23}^{+106} μs] and ^{104}Te [E_{α}=4.9(2) MeV, T_{1/2}<18 ns], decaying into doubly magic ^{100}Sn were produced using a fusion-evaporation reaction ^{54}Fe(^{58}Ni,4n)^{108}Xe, and identified with a recoil mass separator and an implantation-decay correlation technique. This is the first time α radioactivity has been observed to a heavy self-conjugate nucleus. A previous benchmark for study of this fundamental decay mode has been the decay of ^{212}Po into doubly magic ^{208}Pb. Enhanced proton-neutron interactions in the N=Z parent nuclei may result …
Fission Barrier of Superheavy Nuclei and Persistence of Shell Effects at High Spin: Cases ofNo254andTh220
We report on the first measurement of the fission barrier height in a heavy shell-stabilized nucleus. The fission barrier height of No-254 is measured to be B-f = 6.0 +/- 0.5 MeV at spin 15 (h) over bar and, by extrapolation, B-f = 6.6 +/- 0.9 MeV at spin 0 (h) over bar. This information is deduced from the measured distribution of entry points in the excitation energy versus spin plane. The same measurement is performed for Th-220 and only a lower limit of the fission barrier height can be determined: B-f (I) > 8 MeV. Comparisons with theoretical fission barriers test theories that predict properties of superheavy elements.
Exploring the stability of super heavy elements: First Measurement of the Fission Barrier of $^{254} $No
The gamma-ray multiplicity and total energy emitted by the heavy nucleus 254No have been measured at 2 different beam energies. From these measurements, the initial distributions of spin I and excitation energy E * of 254No were constructed. The distributions display a saturation in excitation energy, which allows a direct determination of the fission barrier. 254No is the heaviest shell-stabilized nucleus with a measured fission barrier. © Owned by the authors, published by EDP Sciences, 2014.
Proton decay of 108I and its significance for the termination of the astrophysical rp-process
Abstract Employing the Argonne Fragment Mass Analyzer and the implantation-decay-decay correlation technique, a weak 0.50(21)% proton decay branch was identified in 108I for the first time. The 108I proton-decay width is consistent with a hindered l = 2 emission, suggesting a d 5 2 origin. Using the extracted 108I proton-decay Q value of 597(13) keV, and the Q α values of the 108I and 107Te isotopes, a proton-decay Q value of 510(20) keV for 104Sb was deduced. Similarly to the 112,113Cs proton-emitter pair, the Q p ( I 108 ) value is lower than that for the less-exotic neighbor 109I, possibly due to enhanced proton-neutron interactions in N ≈ Z nuclei. In contrast, the present Q p ( Sb 104 …
Stability and synthesis of superheavy elements: Fighting the battle against fission – example of $^{254}$No
International audience; Superheavy nuclei exist solely due to quantum shell effects,which create a pocket in the potential-energy surface of the nucleus, thusproviding a barrier against spontaneous fission. Determining the height ofthe fission barrier and its angular-momentum dependence is important toquantify the role that microscopic shell corrections play in enhancing andextending the limits of nuclear stability. In this talk, the first measurement ofa fission barrier in the very heavy nucleus 254No will be presented.
Decay and Fission Hindrance of Two- and Four-QuasiparticleKIsomers inRf254
Two isomers decaying by electromagnetic transitions with half-lives of 4.7(1.1) and 247(73) μs have been discovered in the heavy ^{254}Rf nucleus. The observation of the shorter-lived isomer was made possible by a novel application of a digital data acquisition system. The isomers were interpreted as the K^{π}=8^{-}, ν^{2}(7/2^{+}[624],9/2^{-}[734]) two-quasineutron and the K^{π}=16^{+}, 8^{-}ν^{2}(7/2^{+}[624],9/2^{-}[734])⊗8^{-}π^{2}(7/2^{-}[514],9/2^{+}[624]) four-quasiparticle configurations, respectively. Surprisingly, the lifetime of the two-quasiparticle isomer is more than 4 orders of magnitude shorter than what has been observed for analogous isomers in the lighter N=150 isotones. …
First Exploration of Neutron Shell Structure below Lead and beyond N=126
The nuclei below lead but with more than 126 neutrons are crucial to an understanding of the astrophysical r process in producing nuclei heavier than A∼190. Despite their importance, the structure and properties of these nuclei remain experimentally untested as they are difficult to produce in nuclear reactions with stable beams. In a first exploration of the shell structure of this region, neutron excitations in ^{207}Hg have been probed using the neutron-adding (d,p) reaction in inverse kinematics. The radioactive beam of ^{206}Hg was delivered to the new ISOLDE Solenoidal Spectrometer at an energy above the Coulomb barrier. The spectroscopy of ^{207}Hg marks a first step in improving our…
New constraints on the Al25(p,γ) reaction and its influence on the flux of cosmic γ rays from classical nova explosions
The astrophysical $^{25}\mathrm{Al}(p,\ensuremath{\gamma})\phantom{\rule{0.16em}{0ex}}^{26}\mathrm{Si}$ reaction represents one of the key remaining uncertainties in accurately modeling the abundance of radiogenic $^{26}\mathrm{Al}$ ejected from classical novae. Specifically, the strengths of key proton-unbound resonances in $^{26}\mathrm{Si}$, that govern the rate of the $^{25}\mathrm{Al}(p,\ensuremath{\gamma})$ reaction under explosive astrophysical conditions, remain unsettled. Here, we present a detailed spectroscopy study of the $^{26}\mathrm{Si}$ mirror nucleus $^{26}\mathrm{Mg}$. We have measured the lifetime of the ${3}^{+}$, 6.125-MeV state in $^{26}\mathrm{Mg}$ to be $19(3)\phanto…