Spectroscopy along flerovium decay chains. II : Fine structure in odd-A289Fl

Fifteen correlated α-decay chains starting from the odd-A superheavy nucleus 289Fl were observed following the fusion-evaporation reaction 48Ca+244Pu. The results call for at least two parallel α-decay sequences starting from at least two different states of 289Fl. This implies that close-lying levels in nuclei along these chains have quite different spin-parity assignments. Further, observed α-electron and α-photon coincidences, as well as the α-decay fine structure along the decay chains, suggest a change in the ground-state spin assignment between 285Cn and 281Ds. Our experimental results, on the excited level structure of the heaviest odd-N nuclei to date, provide a direct testing groun…

Isomeric 13/2+ state in 201Fr

We have identified an isomeric state in 201Fr for which we propose a spin and parity of 13/2 +, and interpret it as arising from the π(i13/2 ) configuration. A half-life of 720(40) ns was measured, corresponding to B(M2) = 0.17(2) W.u., in good agreement with those of other 13/2 + → 9/2 − [π(i13/2 ) → π(h9/2 )] transitions observed in other nuclei in the region. The nuclei of interest were produced in a fusion-evaporation reaction and their decay properties were investigated using the GREAT spectrometer at the focal plane of the RITU gas-filled recoil separator. peerReviewed

New collective structures in Au179 and their implications for the triaxial deformation of the Pt178 core

Identification of new transitions feeding the high-spin isomers in $^{139}$Nd and $^{140}$Nd nuclei

The population of the high-spin isomers in 139Nd and 140Nd was investigated using the 96Zr(48Ca,xn) reaction and the JUROGAM + RITU + GREAT setup employing the recoil decay tagging technique. Three transitions feeding the 23/2+ isomer in 139Nd and two transitions feeding the 20+ isomer in 140Nd were identified. The newly observed transitions allowed the excitation energy of the isomer to be established in 139Nd and to assign configurations to the states and bands deexcited by the observed transitions in both nuclei. peerReviewed

In-beam and decay spectroscopy of very neutron deficient iridium nuclei

Iridium nuclei at and beyond the proton drip line have been studied via fusion evaporation reactions. A reaction of 92Mo(78Kr, p2n) at a beam energy of 360 MeV and target thickness 500 µg cm−2 was employed to study 167,167mIr. A reaction of 112Sn(58Ni, p2n) at a beam energy of 266 MeV and target thickness 500 µg cm−2 was used to study 169,169mIr. The experiments were performed at the University of Jyvaskyla utilizing the RITU separator in conjunction with the focal plane GREAT spectrometer and the JUROGAM Ge array at the target position. Excited states feeding both the ground state and isomeric state in 169Ir, excited states feeding the ground state of 167Ir and the ground state alpha decay…

Gamma-ray spectroscopy of191,193Bi

Very neutron-deficient Bi-191,Bi-193 nuclei have been studied at the Department of Physics, University of Jyvaskyla, Finland (JYFL) employing the Jurosphere II Ge-detector array coupled to the gas-filled recoil separator RITU and different tagging techniques. For the first time in heavy odd-mass nuclei, a collective band (oblate) is identified above the 2p-1h (1/2(+)) proton intruder state in Bi-191. In both Bi-191,Bi-193, a band based on isomeric 13/2(+) state has been observed and oblate deformation for this state has been deduced. ispartof: Acta Physica Polonica B vol:32 issue:3 pages:1019-1023 ispartof: location:POLAND, ZAKOPANE status: published

Some Remarks on the Discovery of 244Md

In two recent papers by Pore et al. and Khuyagbaatar et al., discovery of the new isotope Md244 was reported. The decay data, however, are conflicting. While Pore et al. report two isomeric states decaying by α emission with Eα(1)=8.66(2) MeV, T1/2(1)=0.4-0.1+0.4 s and Eα(2)=8.31(2) MeV, T1/2(2)≈6 s, Khuyagbaatar et al. [Phys. Rev. Lett. 125, 142504 (2020).PRLTAO0031-900710.1103/PhysRevLett.125.142504] report only a single transition with a broad energy distribution of Eα=(8.73-8.86) MeV and T1/2=0.30-0.09+0.19 s. The data published in Pore et al. are very similar to those published for Md245m [Eα=8.64(2), 8.68(2) MeV, T1/2=0.35-0.16+0.23 s [V. Ninov, F. P. Heßberger, S. Hofmann, H. Folger,…

Rich band structure and multiple long-lived isomers in the odd-odd 118Cs nucleus

One of the largest sets of collective excitations built on two-quasiparticle configurations in odd-odd nuclei of the proton-rich A≈120 mass region is reported in 118Cs. Several new rotational bands and long-lived isomers have been identified. The 8+ bandhead of the πh11/2⊗νh11/2 band is a short-lived isomer with a half-life in the nanosecond range, while the 7+ state below it is a long-lived isomer with a half-life of T1/2=0.55(6)μs. Two other long-lived isomers have been identified: a 66-keV transition detected at the MARA focal plane depopulates one of them, indicating a half-life in the microsecond range, while no depopulating transitions have been identified for the other, indicating a …

Backbending in the pear-shaped 223(90)Th nucleus: Evidence of a high-spin octupole to quadrupole shape transition in the actinides

International audience; Relatively neutron-rich thorium isotopes lie at the heart of a nuclear region of nuclei exhibiting octupole correlation effects. The detailed level structure of Th223 has been investigated in measurements of γ radiation following the fusion-evaporation channel of the Pb208(O18,3n)Th223 reaction at 85 MeV beam energy. The level structure has been extended up to spin 49/2, and 33 new γ rays have been added using triple-γ coincidence data. The spins and parities of the newly observed states have been confirmed by angular distribution ratios. In addition to the two known yrast bands based on a K=5/2 configuration, a non-yrast band has been established up to spin 35/2. We…

Spectroscopy of low-spin states in $^{157}\mathrm{Dy}$: Search for evidence of enhanced octupole correlations

Low-spin states of 157Dy have been studied using the JUROGAM II array, following the 155Gd ({\alpha}, 2n) reaction at a beam energy of 25 MeV. The level scheme of 157Dy has been expanded with four new bands. Rotational structures built on the [523]5/2- and [402]3/2+ neutron orbitals constitute new additions to the level scheme as do many of the inter- and intra-band transitions. This manuscript also reports the observation of cross I- to (I-1)- and I- to (I-1)+ E1 dipole transitions inter-linking structures built on the [523]5/2- (band 5) and [402]3/2+ (band 7) neutron orbitals. These interlacing band structures are interpreted as the bands of parity doublets with simplex quantum number s =…

First candidates for γ vibrational bands built on the [505]11/2⁻ neutron orbital in odd-A Dy isotopes

Rotational structures have been measured using the Jurogam II and GAMMASPHERE arrays at low spin following the 155Gd(α,2n)157Dy and 148Nd(12C,5n)155Dy reactions at 25 and 65 MeV, respectively. We report high-K bands, which are conjectured to be the first candidates of a Kπ=2+γ vibrational band, built on the [505]11/2− neutron orbital, in both odd-A155,157Dy isotopes. The coupling of the first excited K=0+ states or the so-called β vibrational bands at 661 and 676 keV in 154Dy and 156Dy to the [505]11/2− orbital, to produce a Kπ=11/2− band, was not observed in both 155Dy and 157Dy, respectively. The implication of these findings on the interpretation of the first excited 0+ states in the cor…

Isomeric 13/2+ (νi13/2−1) state in 211Th

Using a fusion-evaporation reaction and a gas-filled recoil separator, an isomeric state [T12=83(8)μs] with a most likely spin and parity of 132+ has been identified in Th211. The isomeric state is mainly depopulated via a hindered internal M2 transition [B(M2)=0.0025(5) W.u.], but also a weak α-decay branch of 4(3)% was observed. The present observations fit well to the systematic pattern set by the previously identified states of the same spin and parity in this region of the nuclear chart. peerReviewed

First Study on Nihonium (Nh, Element 113) Chemistry at TASCA

Frontiers in Chemistry 9, 753738 (2021). doi:10.3389/fchem.2021.753738

Stability of the heaviest elements : K isomer in 250No

Decay spectroscopy of 250No has been performed using digital electronics and pulse-shape analysis of the fast nuclear decays for the first time. Previous studies of 250No reported two distinct fission decay lifetimes, related to the direct fission of the ground state and to the decay of an isomeric state but without the possibility to determine if the isomeric state decayed directly via fission or via internal electromagnetic transitions to the ground state. The data obtained in the current experiment allowed the puzzle to finally be resolved, attributing the shorter half-life of t1/2 = 3.8 ± 0.3 μs to the ground state and the longer half-life t1/2 = 34.9+3.9 −3.2 μs to the decay of an isom…

Shape coexistence in $^{178}$Hg

Lifetime measurements of excited states in 178 Hg have been performed using the 103 Rh ( 78 Kr , p 2 n ) reaction at a beam energy of 354 MeV. The recoil-decay tagging (RDT) technique was applied to select the 178 Hg nuclei and associate the prompt γ rays with the correlated characteristic ground-state α decay. Lifetimes of the four lowest yrast states of 178 Hg have been determined using the recoil distance Doppler-shift (RDDS) method. The experimental data are compared to theoretical predictions with focus on shape coexistence. The results confirm the shift of the deformed prolate structures to higher lying states but also indicate their increasing deformation with decreasing neutron numb…

In-beam gamma-ray and electron spectroscopy of $^{249,251}$Md

The odd-Z Md251 nucleus was studied using combined γ-ray and conversion-electron in-beam spectroscopy. Besides the previously observed rotational band based on the [521]1/2− configuration, another rotational structure has been identified using γ-γ coincidences. The use of electron spectroscopy allowed the rotational bands to be observed over a larger rotational frequency range. Using the transition intensities that depend on the gyromagnetic factor, a [514]7/2− single-particle configuration has been inferred for this band, i.e., the ground-state band. A physical background that dominates the electron spectrum with an intensity of ≃60% was well reproduced by simulating a set of unresolved ex…

A Recoil-Beta Tagging Study of N = Z nucleus [sup 66]As

A Recoil‐Beta Tagging (RBT) experiment was recently performed at the accelerator laboratory at the University of Jyvaskyla in order to identify T = 1 excited states in the medium‐heavy N = Z = 33 nucleus 66As. The fusion‐evaporation reaction 28Si(40Ca,pn)66As was employed at a beam energy of 75 MeV. The experiment was carried out utilising the JUROGAM II γ‐ray spectrometer in conjunction with the gas‐filled recoil separator RITU and the GREAT focal plane spectrometer system. The half‐lives and ordering of the two known isomeric states in 66As have been determined. In addition, several new prompt γ‐ray transitions from excited states both bypassing and decaying to the isomeric states in 66As…

Decays of new nuclides and isomers beyond the proton drip line - The influence of neutron configurations

Bozok University;Erciyes University;et al.;Istanbul University;Nigde University;The Turkish Atomic Energy Authority (TAEK)

De-excitation of the strongly coupled band in 177Au and implications for core intruder configurations in the light Hg isotopes

International audience; Excited states in the proton-unbound nuclide $^{177}$Au were populated in the $^92}$Mo($^{88}$Sr, p2n) reaction and identified using the Jurogam-II and GREAT spectrometers in conjunction with the RITU gas-filled separator at the University of Jyväskylä Accelerator Laboratory. A strongly coupled band and its decay path to the 11/2−α-decaying isomer have been identified using recoil-decay tagging. Comparisons with cranked Hartree-Fock-Bogoliubov (HFB) calculations based on Skyrme energy functionals suggest that the band has a prolate deformation and is based upon coupling the odd 1h11/2 proton hole to the excited 02+ configuration in the $^{178}$Hg core. Although these…

Decay studies of new isomeric states in 255No

The decay of excited states in 255No was investigated by applying the evaporation-residue–conversion-electron correlation technique. Two new isomeric states were observed in 255No together with the previously known one. Excitation energies of the isomeric states were estimated based on the energies of conversion electrons and γ rays from correlation chains. These results were in accord with theoretical calculations based on the mean-field models. A tentative decay scheme of isomeric states in 255No is proposed, and their Nilsson configurations are discussed. The energy decrease of the 11/2−[725] Nilsson level for heavy N=153 isotones as a function of increasing proton number is confirmed. p…

Chirality of 135 Nd reexamined : Evidence for multiple chiral doublet bands

One new pair of positive-parity chiral doublet bands have been identified in the odd-A nucleus 135Nd which together with the previously reported negative-parity chiral doublet bands constitute a third case of multiple chiral doublet (MχD) bands in the A ≈ 130 mass region. The properties of the MχD bands are well reproduced by constrained covariant density functional theory and particle rotor model calculations. The newly observed MχD bands in 135Nd represents an important milestone in supporting the existence of MχD in nuclei. peerReviewed

Exploring the boundaries of the nuclear landscape : α-decay properties of 211Pa

Employing the recoil ion transport unit (RITU) and a fusion-evaporation reaction, the α decay of 211Pa has been identified via the implantation-decay correlation technique through observation of chains up to four consecutive decays. An α-particle energy and half-life of 8320(40) keV and 3.8+4.6−1.4 ms, respectively, were measured, corresponding to favored α decay. In addition, more precise α-decay properties of 212Pa and 213Pa were obtained due to accumulated statistics. The present data were compared to those predicted by selected atomic mass models and it was used to estimate the possibility of observing proton emission from these isotopes. peerReviewed

Towards higher sensitivity at the RITU focal plane

The recently reconstructed focal plane detector system for the gas-filled recoil separator RITU was used to observe a new proton emitter 164Ir. The nuclide was produced via the p5n fusion evaporation channel using a 64Zn beam on a 106Cd target. The proton energy Ep = 1817(9) keV and half-life T1/2 = 113+62-30 μ s were used to characterize the decaying state to be [π h11/2 ν f7/2]9+. The new focal plane detector system and the results of the proton decay studies will be discussed. peerReviewed

Lifetime measurements of excited states in $^{162}$W and $^{164}$W and the evolution of collectivity in rare-earth nuclei

International audience; Lifetimes of the first excited 2+ states in the extremely neutron-deficient $^{162}$W and $^{164}$W nuclei have been measured using the recoil distance Doppler shift technique. Experimental B(E2) data for the isotopic chains of hafnium, tungsten, and osmium, from the midshell region near the β-stability line towards the N=82 closed shell and the most neutron-deficient nuclides, are compared with predictions of nuclear deformations and 21+→0g.s.+ reduced transition strengths from different classes of state-of-the-art theoretical model calculations. The results reveal striking differences and deficiencies in the predictive power of current nuclear structure models.

α-spectroscopy studies of the new nuclides 165Pt and 170Hg

The new nuclides 165Pt and 170Hg were produced in the reactions 92Mo(78Kr,5n) and 96Ru(78Kr,4n) at bombarding energies of 418 MeV and 390 MeV, respectively. For 170Hg an α-particle energy of Eα=7590(30)keV and half-life of t1/2=0.08+0.40−0.04ms were deduced, while for 165Pt the corresponding values were 7272(14) keV and 0.26+0.26−0.09ms. Comparison of the reduced α-decay widths with systematics indicates that both α decays are unhindered. Although combining the measured α-decay Q values with extrapolated masses suggests that both new nuclides are unbound to two-proton emission by more than 1 MeV, their α-decay half-lives are too short for this decay mode to compete. Improved data were also …

Characterizing the atomic mass surface beyond the proton drip line via a-decay measurements of the s1/2 ground state of 165Re and the h11/2 isomer in 161Ta

The a-decay chains originating from the s1/2 and h11/2 states in 173Au have been investigated following fusion-evaporation reactions. Four generations of a radioactivities have been correlated with 173Aum leading to a measurement of the a decay of 161Tam. It has been found that the known a decay of 161Ta, which was previously associated with the decay of the ground state, is in fact the decay of an isomeric state. This work also reports on the first observation of prompt g rays feeding the ground state of 173Au. This prompt radiation was used to aid the study of the a-decay chain originating from the s1/2 state in 173Au. Three generations of a decays have been correlated with this state lea…

Shell-Structure and Pairing Interaction in Superheavy Nuclei: Rotational Properties of the Z=104 Nucleus (256)Rf

The rotational band structure of the Z ¼ 104 nucleus 256Rf has been observed up to a tentative spin of 20@ using state-of-the-art -ray spectroscopic techniques. This represents the first such measurement in a superheavy nucleus whose stability is entirely derived from the shell-correction energy. The observed rotational properties are compared to those of neighboring nuclei and it is shown that the kinematic and dynamic moments of inertia are sensitive to the underlying single-particle shell structure and the specific location of high-j orbitals. The moments of inertia therefore provide a sensitive test of shell structure and pairing in superheavy nuclei which is essential to ensure the val…

Lifetime measurements of excited states in ¹⁶³W and the implications for the anomalous B(E2) ratios in transitional nuclei

This letter reports lifetime measurements of excited states in the odd-N nucleus $^{163}$W using the recoil-distance Doppler shift method to probe the core polarising effect of the i13/2 neutron orbital on the underlying soft triaxial even-even core. The ratio B(E2:21/2+→17/2+)/B(E2:17/2+→13/2+) is consistent with the predictions of the collective rotational model. The deduced B(E2) values provide insights into the validity of collective model predictions for heavy transitional nuclei and a geometric origin for the anomalous B(E2) ratios observed in nearby even-even nuclei is proposed.

Reinvestigation of the excited states in the proton emitter $^{151}$Lu: particle-hole excitations across the $N=Z=64$ subshell

The excited states of the proton emitter $^{151}$Lu were reinvestigated in a recoil-decay tagging experiment at the Accelerator Laboratory of the University of Jyv\"askyl\"a (JYFL). The level scheme built on the ground state of $^{151}$Lu was updated with five new $\gamma$-ray transitions. Large-scale shell model calculations were carried out to interpret the experimental level scheme. It is found that the excitation energies of states above the $27/2^-$ and $23/2^+$ isomeric levels can be sensitive to excitations from $g_{7/2}$ and $d_{5/2}$ to single-particle orbitals above $N=Z=64$.

First candidates for $\gamma$ vibrational bands built on the $[505]11/{2}^{-}$ neutron orbital in odd-$A$ Dy isotopes

Rotational structures have been measured using the Jurogam II and GAMMASPHERE arrays at low spin following the 155Gd({\alpha},2n)157Dy and 148Nd(12C, 5n)155Dy reactions at 25 and 65 MeV, respectively. We report high-K bands, which are conjectured to be the first candidates of a K{\pi}= 2+ {\gamma} vibrational band, built on the [505]11/2- neutron orbital, in both odd-A 155, 157Dy isotopes. The coupling of the first excited K=0+ states or the so-called \b{eta} vibrational bands at 661 and 676 keV in 154Dy and 156Dy to the [505]11/2- orbital, to produce a K{\pi}=11/2- band, was not observed in both 155Dy and 157Dy, respectively. The implication of these findings on the interpretation of the f…

Identification of sub-μs isomeric states in the odd-odd nucleus 178Au

The neutron-deficient gold (Z=79) isotopes in the vicinity of the neutron midshell N=104 provide prolific examples of shape coexistence and isomerism at low excitation energy. They can be probed via a number of different experimental techniques. In this study, two new isomeric states with half-lives of 294(7) and 373(9) ns have been observed in the neutron-deficient odd-odd nuclide 178Au (N=99) in an experiment at the RITU gas-filled separator at JYFL, Jyväskylä. This result was achieved due to the use of a segmented planar germanium detector with a high efficiency at low energies. By applying the recoil-decay tagging technique, they were assigned to decay to two different long-lived α-deca…

Neutron excitations in 119Ba

The neutron-deficient 119Ba nucleus has been studied using the 58Ni(64Zn,2pn) reaction and the JUROGAM 3 γ-ray detector array coupled to the MARA recoil-mass separator setup. One new rotational band and several low-lying states are newly identified. A half-life of T1/2=0.36(2)μs has been measured for the 5/2− bandhead of the νh11/2 band. The two previously known rotational bands are confirmed, except for the higher part of the +1/2 signature partner of the positive-parity band. Configurations are assigned based on the analysis of the observed quasiparticle alignments whose nature is unveiled by the calculations using the particle number conserving cranked shell model. peerReviewed

Decay of a 19(-) isomeric state in Lu-156

A multiparticle spin-trap isomeric state having a half-life of 179(4) ns and lying 2601 keV above the yrast 10(+) state in Lu-156 has been discovered. The Lu-156 nuclei were produced by bombarding isotopically enriched Cd-106 targets with beams of Ni-58 ions, separated in flight using the gas-filled separator RITU and their decays were measured using the GREAT spectrometer. Analysis of the main decay path that populates yrast states observed previously suggests a spin-parity assignment of 19(-) for the isomeric state, which is consistent with isomeric states identified in the N = 85 isotones. Comparison with other decay paths in Lu-156 indicates that the [pi h(11/)(2)(-1) circle times nu h(…

Signatures of enhanced octupole correlations at high spin in 136Nd

Experimental signatures of moderately enhanced octupole correlations at high spin in 136Nd are indicated for the first time. The extracted dipole moments of two negative-parity bands are only two times smaller than those of the lanthanide nuclei with N≈90 which present well-established octupole correlations. Calculations using the cranked quasiparticle random phase approximation and a model of quadrupole-octupole rotations with octupole vibrations reveal the structure of the bands and the enhanced octupole correlations at high spin in 136Nd. peerReviewed

Studies of SHE at SHIP

An overview of present experimental investigation of superheavy elements is given. The data are compared with theoretical descriptions. Results are reported from an experiment to confirm production of element 112 isotopes in irradiation of 238UF4 with 48Ca. One spontaneous fission event was measured, which agrees with three events of previously measured data which had been assigned to the decay of 283112. However, more experimental work is needed in order to obtain an independent and unambiguous confirmation of previous results.

In-beam γ-ray spectroscopy of 94Ag

A recoil-beta-tagging experiment has been per formed to study the excited T = 0 and T = 1 states in the odd–odd N = Z nucleus 94Ag, populated via the 40Ca(58Ni,1p3n)94Ag reaction. The experiment was con ducted using the MARA recoil separator and JUROGAM3 array at the Accelerator Laboratory of the University of Jyväskylä. Through correlating fast, high-energy beta decays at the MARA focal plane with prompt γ rays emitted at the reaction target, a number of transitions between excited states in 94Ag have been identified. The timing characteris tics of these transitions confirm that they fall within decay sequences that feed the short-lived T = 1 ground state of 94Ag. The transitions are propo…

Complete set of proton excitations in 119Cs

The very neutron-deficient strongly deformed 119Cs nucleus has been studied using the 58Ni(64Zn,3p) reaction and the JUROGAM 3 γ-ray detector array coupled to the MARA recoil-mass separator setup. The excitation energies of all observed bands have been determined, spins and parities have been firmly assigned to most of the observed states. The previously known and the newly identified rotational bands have been extended to very high spin and excitation energy. The configurations of the observed bands are discussed using the particle number conserving cranked shell model. The present study establishes the largest set of rotational bands observed in the proton-rich A≈120 mass region. peerRevi…

Lifetime Measurements of Excited States in $^{172}$Pt and the Variation of Quadrupole Transition Strength with Angular Momentum

Lifetimes of the first excited 2 + and 4 + states in the extremely neutron-deficient nuclide 172 Pt have been measured for the first time using the recoil-distance Doppler shift and recoil-decay tagging techniques. An unusually low value of the ratio B ( E 2 : 4 + 1 → 2 + 1 ) / B ( E 2 : 2 + 1 → 0 + gs ) = 0.55 ( 19 ) was found, similar to a handful of other such anomalous cases observed in the entire Segré chart. The observation adds to a cluster of a few extremely neutron-deficient nuclides of the heavy transition metals with neutron numbers N ≈ 90 – 94 featuring the effect. No theoretical model calculations reported to date have been able to explain the anomalously low B ( E 2 : 4 + 1 → …

Lifetime measurements of yrast states in ¹⁷⁸ Pt using the charge plunger method with a recoil separator

Abstract Lifetime measurements in \(^{178}\)Pt with excited states de-exciting through \(\gamma\)-ray transitions and internal electron conversions have been performed. Ionic charges were selected by the in-flight mass separator MARA and measured at the focal plane in coincidence with the \(4^{+}_{1}→2^{+}_{1}\) 257 keV γ-ray transition detected using the JUROGAM 3 spectrometer. The resulting charge-state distributions were analysed using the differential decay curve method (DDCM) framework to obtain a lifetime value of 430(20) ps for the \(2^{+}_{1}\) state. This work builds on a method that combines the charge plunger technique with the DDCM analysis. As an alternative analysis, ions were…

Precision measurements of proton emission from the ground states of 156Ta and 160Re

The decays of the πd3/2 ground states of 156Ta and 160Re have been studied in detail using the GREAT spectrometer. More than 7000 160Re nuclei were produced in reactions of 290- and 300-MeV 58Ni ions with an isotopically enriched 106Cd target and separated in flight using the RITU separator. The proton and α decays of the πd3/2 level were confirmed and the half-life and branching ratios of this state were determined with improved precision to be t1/2=611±7 μs and bp=89±1% and bα=11±1%, respectively. The α-decay branch populated the ground state of 156Ta, allowing improved values for the proton-decay energy and half-life to be obtained (Ep=1011±5 keV; t1/2=106±4 ms). The β decay of this leve…

Alpha decay study of 218U; a search for the sub-shell closure at Z=92

Neutron-deficient uranium isotopes were studied via α spectroscopic methods. A low-lying α-decaying isomeric state was found in 218U. The new isomeric state was assigned spin and parity I π = 8+. The isomer decays by α emission with an energy E = 10678(17) keV and with a half-life T 1/2 = (0.56 -0.14 +0.26 ) ms. The known alpha-decay properties of the ground state of 218U was measured with improved statistics. The ground-state α-decay has an energy E = 8612(9) keV and a half-life T 1/2 = (0.51 -0.10 +0.17 ) ms.

Refined description of the positive-parity bands and the extent of octupole correlations in 120Ba

Three new negative-parity bands have been identified in 120Ba, two of them forming a strongly coupled band. The previously known negative-parity band is significantly extended to high spin, while the lower part of the yrare positive-parity band has been modified. From the analysis of the band properties and comparison with the neighboring nuclei a coherent description of all bands is achieved. In particular, a simple explanation of the evolution of the positive-parity bands at high spin is proposed, including the possible occupation of the νf7/2[541]1/2− intruder orbital. Cranked Nilsson-Strutinsky calculations reveal similar quadrupole deformations but different triaxiality of the bands, w…

Production cross section and decay study of $^{243}$Es and $^{249}$Md

In the study of the odd-$Z$, even-$N$ nuclei $^{243}$Es and $^{249}$Md, performed at the University of Jyv\"askyl\"a, the fusion-evaporation reactions $^{197}$Au($^{48}$Ca,2$n$)$^{243}$Es and $^{203}$Tl($^{48}$Ca,2$n$)$^{249}$Md have been used for the first time. Fusion-evaporation residues were selected and detected using the RITU gas-filled separator coupled with the focal-plane spectrometer GREAT. For $^{243}$Es, the recoil decay correlation analysis yielded a half-life of $24 \pm 3$s, and a maximum production cross section of $37 \pm 10$ nb. In the same way, a half-life of $26 \pm 1$ s, an $\alpha$ branching ratio of 75 $\pm$ 5%, and a maximum production cross section of 300 $\pm$ 80 nb…

Structure of the Odd-A, Shell-Stabilized NucleusNo102253

In-beam {gamma}-ray spectroscopic measurements have been made on {sub 102}{sup 253}No. A single rotational band was identified up to a probable spin of 39/2({Dirac_h}/2{pi}), which is assigned to the 7/2{sup +}[624] Nilsson configuration. The bandhead energy and the moment of inertia provide discriminating tests of contemporary models of the heaviest nuclei. Novel methods were required to interpret the sparse data set associated with cross sections of around 50 nb. These methods included comparisons of experimental and simulated spectra, as well as testing for evidence of a rotational band in the {gamma}{gamma} matrix.

Spectroscopy along flerovium decay chains. III : Details on experiment, analysis, 282Cn, and spontaneous fission branches

Flerovium isotopes (element Z=114) were produced in the fusion-evaporation reactions 48Ca+242,244Pu and studied with an upgraded TASISpec decay station placed in the focal plane of the gas-filled separator TASCA at the GSI Helmholtzzentrum für Schwerionenforschung in Darmstadt, Germany. Twenty-nine flerovium decay chains were identified by means of correlated implantation, α decay, and spontaneous fission events. Data analysis aspects and statistical assessments, primarily based on measured rates of various events, which laid the foundation for the comprehensive spectroscopic information on the flerovium decay chains, are presented in detail. Various decay scenarios of an excited state obse…

New collective structures in 179Au and their implications for the triaxial deformation of the 178Pt core

The extremely neutron-deficient isotope 179Au has been studied by a combination of in-beam γ-ray and isomeric-decay spectroscopy. For in-beam spectroscopy, the recoil-isomer tagging technique was employed, using the known 3/2−, T1/2=328 ns isomer. A new rotational band, associated with the unfavored signature band of the 1h9/2⊕2f7/2 proton-intruder configuration, was revealed. A previously unknown, high-spin isomeric state with an excitation energy of 1743(17) keV and T1/2=2.16(8)µs was discovered. Five decay paths were identified, some of them feeding previously unknown non-yrast excited states, associated with the 1i13/2 proton-intruder configuration. Calculations based on the particle-pl…

An innovative Superconducting Recoil Separator for HIE-ISOLDE

International audience; The ISOLDE Scientific Infrastructure at CERN offers a unique range of post-accelerated radioactive beams. The scientific program can be improved with the “Isolde Superconducting Recoil Separator” (ISRS), an innovative spectrometer able to deliver unprecedented (A, Z) resolution. In this paper we present an overview of the physics and ongoing technical developments.

Identification of excited states in 107,52Te55

Excited states in the extremely neutron-deficient nucleus 107Te have been identified from two separate experiments using the recoil-decay tagging technique. Two connected structures were observed on the basis of γγ-coincidence relations and tentatively assigned as built on the mixed-parentage νg7/2d5/2 and νh11/2 intruder configurations. The observed structures were compared with large-scale shell-model calculations and total Routhian surface calculations. Collective behavior was discovered to persist in the νh11/2 band of 107Te which highlights the shape-polarizing effect of a single valence neutron occupying the h11/2 intruder orbit as the N=50 shell closure is approached. peerReviewed

On the adsorption and reactivity of element 114, flerovium

Flerovium (Fl, element 114) is the heaviest element chemically studied so far. To date, its interaction with gold was investigated in two gas-solid chromatography experiments, which reported two different types of interaction, however, each based on the level of a few registered atoms only. Whereas noble-gas-like properties were suggested from the first experiment, the second one pointed at a volatile-metal-like character. Here, we present further experimental data on adsorption studies of Fl on silicon oxide and gold surfaces, accounting for the inhomogeneous nature of the surface, as it was used in the experiment and analyzed as part of the reported studies. We confirm that Fl is highly v…

Discovery of the proton emitting nucleus $^{159}$Re

Fund. para Cienc. Tecnol., FCT, Minist. Cienc. Tecnol.;Fundacao Calouste Gulbenkian;Fundacao Luso-Americana

Shape coexistence at the proton drip-line: First identification of excited states in 180Pb

Excited states in the extremely neutron-deficient nucleus, 180Pb, have been identified for the first time using the JUROGAM II array in conjunction with the RITU recoil separator at the Accelerator Laboratory of the University of Jyvaskyla. This study lies at the limit of what is presently achievable with in-beam spectroscopy, with an estimated cross-section of only 10 nb for the 92Mo(90Zr,2n)180Pb reaction. A continuation of the trend observed in 182Pb and 184Pb is seen, where the prolate minimum continues to rise beyond the N=104 mid-shell with respect to the spherical ground state. Beyond mean-field calculations are in reasonable correspondence with the trends deduced from experiment.

Decay spectroscopy of 171,172Os and 171,172,174Ir

We report on a study of the α-decay fine structure and the associated Eα−Eγ correlations in the decays of 171,172Os and 171,172,174Ir. In total, 13 new α-decay energy lines have been resolved, and three new γ-ray transitions have been observed following the new decay branches to 168Re and 167W. The weak α-decay branch from the bandhead of the νi13/2 band in 171Os observed in this work highlights an unusual competition between α, β, and electromagnetic decays from this isomeric state. The nucleus 171Os is therefore one of few nuclei observed to exhibit three different decay modes from the same excited state. The nuclei of interest were produced in 92Mo(83Kr,xpyn) fusion-evaporation reactions…

Observation ofK=1/2octupole deformed bands in227Th

High-spin states in 227Th have been populated using the reaction 226Ra(α,3n)227Th at a bombarding energy of 33 MeV. The high-spin rotational structures of this nucleus have been refined and extended. In addition, the linking of these structures with the low-spin states known from 231U α decay has allowed a comprehensive decay scheme of this nucleus to be assembled for the first time. Four previously known rotational bands are interpreted as Coriolis coupled Kπ=1/2+ and Kπ=1/2− bands, in agreement with predictions using a reflection-asymmetric mean field approach. The determination of decoupling parameters for these bands is consistent with the a(Kπ=1/2+)=−a(Kπ=1/2−) rigid octupole rotor exp…

Alpha decay studies of translead nuclei at the proton drip line

Extensive α-decay studies of the very neutron deficient isotopes 191Po, 195Rn, and 196Rn have been performed at the RITU gas-filled recoil separator. The recoil-α–(α) correlation technique and the α–γ coincidence technique have been utilized to unambiguously connect the observed α-decays to proper nuclei. Illustrative examples on how the α-decay can yield spectroscopic information on the nuclei studied will be presented. peerReviewed

Mass-140 isomers near the proton dripline

An experiment has been performed in Jyvaskyla, Finland, using Jurogam in conjunction with RITU and GREAT. This experiment populated several extremely neutron-deficient nuclei around the mass-140 region of the nuclei chart, using the 92Mo(54Fe, α2n) reaction at 245 MeV. Analysis of these data has revealed several previously unobserved isomeric states, in several nuclei. One of these has been assigned to 143Dy with a half-life of 1.2 ± 0.3 µs. The energies of the prompt γ rays in the band built upon the isomer are in agreement with those previously observed.

A charge plunger device to measure the lifetimes of excited nuclear states where transitions are dominated by internal conversion

A charge plunger device has been commissioned based on the DPUNS plunger (Taylor et al., 2013) using the in-flight mass separator MARA at the University of Jyväskylä. The 152Sm(32S,4n)180Pt reaction was used to populate excited states in 180Pt. A lifetime measurement of the 21+ state was performed by applying the charge plunger technique, which relies on the detection of the charge state-distribution of recoils rather than the detection of the emitted γ rays. This state was a good candidate to test the charge plunger technique as it has a known lifetime and depopulates through a converted transition that competes strongly with γ-ray emission. The lifetime of the 21+ state was measured to be…

Characteristics of segmented super clover detector in close geometry decay measurements

Characteristics of the segmented Super Clover germanium detector response in close geometries have been studied. Results obtained with localising hit pattern recognition are compared with results from add-back and individual crystal analysis. The detector has been used at the focal plane of a gas filled recoil separator to detect isomeric gamma-rays from the nuclei produced in the 150Sm(42Ca,4n)188Pb reaction. Coincidence data from the detector was analysed and the level scheme below the 1.2 μ s isomeric state in 188Pb could be deduced. peerReviewed

Offline commissioning of a new gas cell for the MARA Low-Energy Branch

Results of offline commissioning tests for a new dedicated gas cell for the Mass Analysing Recoil Apparatus (MARA) Low-Energy Branch are reported. Evacuation time, ion survival and transport efficiency in helium buffer gas were characterized with a radioactive 223Ra 𝛼-recoil source. Suppression of the ion signal, originating from non-neutralized species in the gas cell, was explored with 219Rn ions, the daughter recoil of 223Ra, as a function of voltage applied to one of the ion-collector electrodes. Two-step laser resonance ionization of stable tin isotopes produced inside the gas cell from a heated bronze filament was demonstrated, and broadening of the atomic resonances in argon buffer …

New gas-filled mode of the large-acceptance spectrometer VAMOS

A new gas-filled operation mode of the large-acceptance spectrometer VAMOS at GANIL is reported. A beam rejection factor greater than 10(10) is obtained for the Ca-40+Sm-150 system at 196 MeV. The unprecedented transmission efficiency for the evaporation residues produced in this reaction is estimated to be around 80% for alpha x n channels and above 95% for x ny p channels. A detailed study of the performance of the gas-filled VAMOS and future developments are discussed. This new operation mode opens avenues to explore the potential of fusion reactions in various kinematics. (C) 2010 Elsevier B.V. All rights reserved.

Shape coexistence in183Tl

Probing structural changes in the very neutron-deficient Os isotopes with recoil-decay tagging

In recent years, the exploitation of the iecoil-decay tagging (RDT) technique with,large arrays of germanium detectors has revealed much information about the structure of heavy nuclei approaching the proton drip line. The yrast bands of the N <= 93 osmium isotopes have been identified in a campaign of tagging experiments using various spectrometer arrays coupled to the RITU gas-filled separator based at the University of Jyvaskyla. Trends in the yrast state excitation energies have indicated a transition from gamma-soft triaxial to near-spherical shapes with decreasing neutron number. Recent experimental results for Os-162 obtained with the JUROGAM and GREAT spectrometers also indicate the…

Recoil Isomer Tagging on Proton-Rich Odd–Odd N=77 Isotones 142Tb and 144Ho

The isomeric structure of the N=77 isotones 14265Tb and 14467Ho have been studied with the 92Mo(54Fe, xpn) fusion evaporation reaction at the University of Jyväskylä. The Jurospehere II germanium array was employed in conjunction with the RITU gas filled recoil separator. The feeding and decay of a 500(20) ns isomeric state in 144Ho has been established for the first time together with states built upon the known 15 μs isomer in 142Tb. The behavior of these new structures above the isomers suggest that they are low deformation configurations which display signs of triaxiality. peerReviewed

Delayed and In-beam Spectroscopy on Francium and Astatine Nuclei at the Proton Drip Line

Delayed and in‐beam spectroscopy on francium and astatine nuclei at and beyond the proton drip line has been performed. In neutron deficient astatine nuclei a shift to deformed shapes as a function of decreasing neutron has been obtained. In neutron deficient francium isotope the same shift is evident.

Probing structures of exotic heavy nuclei

The JYFL gas-filled recoil separator RITU, combined with Ge detector arrays, has successfully been employed in Recoil-Decay-Tagging (RDT) experiments in order to probe, for the first time, structures of several very neutron deficient heavy nuclei. In this contribution new data for light even-mass Hg, Pb and Po nuclei are shown and discussed. peerReviewed

The Structure of Heavy Octupole and Superheavy Quadrupole Deformed Nuclei

We report here experimental attempts to determine the sign of the electric dipole moment (relative to the electric octupole moment) in the octupole deformed nucleus 226Ra. Sensitivity to this quantity is observed in the measured yields of γ-ray transitions following very low energy Coulomb excitation. Recent progress is also reported in the development of new spectroscopic techniques that promise to elucidate the structure of deformed superheavy nuclei in the region of 254No. The 4+ → 2+ transition in 254No, as well as higher spin transitions, has been identified using recoil-tagged conversion electron spectroscopy. peerReviewed

Prolate yrast cascade in183Tl

The yrast sequence in ${}^{183}\mathrm{Tl}$ has been studied for the first time in recoil-mass selected \ensuremath{\gamma}-ray spectroscopic measurements. A rotational-like cascade of seven transitions is established down to the band head with probable spin and parity ${(13/2}^{+}).$ Unlike in the adjacent odd-mass Tl nuclei, prompt \ensuremath{\gamma} decay from the yrast band to a lower lying weakly deformed (oblate) structure is not observed. These features are consistent with the predicted drop of the prolate band head in ${}^{183}\mathrm{Tl}$ compared to ${}^{185}\mathrm{Tl}.$ The implications for the prolate energy minimum in odd-mass Tl nuclei at the neutron ${i}_{13/2}$ midshell $(…

Spectroscopy of proton-rich 66^Se up to J^{\pi} = 6^+: isospin-breaking effect in the A = 66 isobaric triplet

Candidates for three excited states in the 66^Se have been identified using the recoil-{\beta} tagging method together with a veto detector for charged-particle evaporation channels. These results allow a comparison of mirror and triplet energy differences between analogue states across the A = 66 triplet as a function of angular momentum. The extracted triplet energy differences follow the negative trend observed in the f_7/2 shell. Shell-model calculations indicate a continued need for an additional isospin non-conserving interaction in addition to the Coulomb isotensor part as a function of mass.

High K bands in mid-supershell nuclei

The spectrum of prompt conversion electrons emitted by excited 254No nuclei has been measured, revealing discrete lines arising from transitions within the ground state band. A striking feature is a broad distribution that peaks near 100 keV and comprises high multiplicity electron cascades, probably originating from M1 transitions within rotational bands built on high K states. Evidence for the existence of isomeric states in 254No is presented. peerReviewed

Evidence for enhanced collectivity in Te-I-Xe nuclei near the N = Z = 50 double shell closure

Gamma‐ray transitions have been identified for the first time in the extremely neutron‐deficient Tz = 1 nuclide 110Xe and the energies of the three lowest excited states in the ground‐state band have been deduced. A level scheme has also been constructed for the proton‐unbound, Tz = 3/2 nuclide 109I, exhibiting band structures built on g7/2 and h11/2 states in a weakly deformed, triaxial nucleus. In addition, a third band is proposed to be built on a g7/2 orbital coupled to an octupole‐vibrational phonon of the 108Te core. The results were obtained in a recoil‐decay tagging experiment using the 58Ni(54Fe,2n/p2n) reaction at a beam energy of 195 MeV. The experiment was performed using the hi…

Isomer spectroscopy in254No

Isomeric states in No-254 were investigated using a calorimetric method. Two different isomers were found with half-lives of T-1/2 = 266 +/- 2 ms and T-1/2 = 184 +/- 3 mu s, respectively. The domin ...

In-beam γ-ray and electron spectroscopy of Md249,251

The odd-Z 251Md nucleus was studied using combined γ-ray and conversion-electron in-beam spectroscopy. Besides the previously observed rotational band based on the [521]1/2− configuration, another rotational structure has been identified using γ−γ coincidences. The use of electron spectroscopy allowed the rotational bands to be observed over a larger rotational frequency range. Using the transition intensities that depend on the gyromagnetic factor, a [514]7/2− single-particle configuration has been inferred for this band, i.e., the ground-state band. A physical background that dominates the electron spectrum with an intensity of ≃60% was well reproduced by simulating a set of unresolved ex…

Spectroscopy of Kr 70 and isospin symmetry in the T=1 fpg shell nuclei SPECTROSCOPY of Kr 70 and ISOSPIN SYMMETRY ... D. M. DEBENHAM et al.

The recoil-β tagging technique has been used in conjunction with the Ca40(S32,2n) reaction at a beam energy of 88 MeV to identify transitions associated with the decay of the 2+ and, tentatively, 4+ states in the nucleus Kr70. These data are used, along with previously published data, to examine the triplet energy differences (TED) for the mass 70 isobars. The experimental TED values are compared with shell model calculations, performed with the JUN45 interaction in the fpg model space, that include a J=0 isospin nonconserving (INC) interaction with an isotensor strength of 100 keV. The agreement is found to be very good up to spin 4 and supports the expectation for analog states that all t…

Evidence against the wobbling nature of low-spin bands in 135Pr

International audience; The electromagnetic character of the ΔI=1 transitions connecting the 1- to 0-phonon and the 2- to 1-phonon wobbling bands should be dominated by an E2 component, due to the collective motion of the entire nuclear charge. In the present work it is shown, based on combined angular correlation and linear polarization measurements, that the mixing ratios of all analyzed connecting transitions between low-lying bands in 135Pr interpreted as 0-, 1-, and 2-phonon wobbling bands, have absolute values smaller than one. This indicates predominant M1 magnetic character, which is incompatible with the proposed wobbling nature. All experimental observables are instead in good agr…

In-beam spectroscopic study of $^{244}$Cf

The ground-state rotational band of the neutron-deficient californium ( Z = 98 ) isotope 244 Cf was identified for the first time and measured up to a tentative spin and parity of I π = 20 + . The observation of the rotational band indicates that the nucleus is deformed. The kinematic and dynamic moments of inertia were deduced from the measured γ -ray transition energies. The behavior of the dynamic moment of inertia revealed an up-bend due to a possible alignment of coupled nucleons in high- j orbitals starting at a rotational frequency of about ℏ ω = 0.20 MeV . The results were compared with the systematic behavior of the even-even N = 146 isotones as well as with available theoretical c…

Tilted precession bands in $^{135}$Nd

International audience; Two new excited bands built on the πh11/2 configuration have been identified in Nd135 in addition to the known πh11/2 band. The energy spectra of the excited bands and the available electromagnetic transition probabilities are in good agreement with theoretical results obtained using quasiparticle-plus-triaxial-rotor model calculations. The properties of the bands identify them as tilted precession bands instead of wobbling bands. Our results give a new insight into the interpretation of the low-lying bands in odd-A mass nuclei, and can stimulate future studies to address the nuclear triaxiality.

Study of non-fusion products in the 50Ti + 249Cf reaction

Physics letters / B B 784, 199 - 205 (2018). doi:10.1016/j.physletb.2018.07.058

Spectroscopy of the neutron-deficient isobars 163 Re and 163 W using tagging techniques

Bozok University;Erciyes University;et al.;Istanbul University;Nigde University;The Turkish Atomic Energy Authority (TAEK)

Experimental observation of the M1 scissors mode in $^{254}No$

Physics letters / B 834, 137479 (2022). doi:10.1016/j.physletb.2022.137479

Evidence for octupole collectivity in 172Pt

Excited states in the extremely neutron-deficient nucleus 172Pt were populated via 96Ru(78Kr,2p) and 92Mo(83Kr,3n) reactions. The level scheme has been extended up to an excitation energy of  ~ 5 MeV and tentative spin-parity assignments up to Iπ = 18+. Linear polarization and angular distribution measurements were used to determine the electromagnetic E1 character of the dipole transitions connecting the positive-parity ground-state band with an excited side-band, firmly establishing it as a negative-parity band. The lowest member of this negative-parity structure was firmly assigned spin-parity 3-. In addition, we observed an E3 transition from this 3- state to the ground state, providing…

Studies of 225,226U alpha decay chains

Studies of 225,226U α -decay chains produced via heavy ion induced fusion reactions of 22Ne + 208Pb → 230U and of 18O + 208Pb → 226Th were carried out using the JYFL gas-filled magnetic recoil separator RITU. The data obtained for α -decays of 225,226U, 221,222Th, 218Ra and 213Rn concerning their α -particle energies, half-lives and α -decay fine structures are compared to previous investigations. peerReviewed

Lifetime measurements of excited states in W-162 and W-164 and the evolution of collectivity in rare-earth nuclei

WOS: 000400140500006

Decay and in-beam studies of neutron-deficient Po and Ra isotopes at JYFL

An extensive program to study the production, decay properties, and nuclear structure of very neutron-deficient polonium and radium nuclei is underway at the Department of Physics, University of Jyvaskyla, Finland (JYFL). The main tools used in these studies are the gas-filled recoil separator RITU and various germanium gamma-ray arrays. In the course of these studies, among others the following new isotopes have been produced: Ra-204, Ra-203, and Ra-202. Isomeric alpha decaying states have been discovered in Ra-203 and Po-191. Fine structure in the decay of Po-192 to the oblate and prolate band heads in Pb-188 has been observed. In-beam gamma-ray spectra have been, for the first time, meas…

Investigation of 246Fm : in-beam spectroscopy at the limits\u2028

β and γ bands in N = 88, 90, and 92 isotones investigated with a five-dimensional collective Hamiltonian based on covariant density functional theory : Vibrations, shape coexistence, and superdeformation

A comprehensive systematic study is made for the collective β and γ bands in even-even isotopes with neutron numbers N=88 to 92 and proton numbers Z=62(Sm) to 70 (Yb). Data, including excitation energies, B(E0) and B(E2) values, and branching ratios from previously published experiments are collated with new data presented for the first time in this study. The experimental data are compared to calculations using a five-dimensional collective Hamiltonian (5DCH) based on the covariant density functional theory (CDFT). A realistic potential in the quadrupole shape parameters V(β,γ) is determined from potential energy surfaces (PES) calculated using the CDFT. The parameters of the 5DCH are fixe…

Identification of isomeric states in the N=73 neutron-deficient nuclei 132Pr and 130La

Decays from isomeric states in the neutron-deficient N=73 nuclei 132Pr and 130La have been observed for the first time. Half-lives of 486(70) ns and 2.46(4) μs were measured for two isomeric states in 132Pr. The decay from the 486ns (8 -) isomer has been interpreted as a hindered E1 transition from the bandhead state of the excited πh 11/2νg 7/2 configuration. The decay from the 2.5 μs (8 +) isomer is consistent with the Weisskopf estimate for a low-energy E2 transition. An analogous 0.74(3) μs decay from an (8 +) isomer in the neighboring isotone 130La has also been observed which similarly can be explained if the transition has E2 character. The Weisskopf interpretation for the isomer hin…

High-spin intruder band in $^{107}$In

High-spin states in the neutron deficient nucleus $^{107}$In were studied via the $^{58}$Ni($^{52}$Cr, 3p) reaction. In-beam $\gamma$ rays were measured using the JUROGAM detector array. A rotational cascade consisting of ten $\gamma$-ray transitions which decays to the 19/2$^{+}$ level at 2.002 MeV was observed. The band exhibits the features typical for smooth terminating bands which also appear in rotational bands of heavier nuclei in the A$\sim$100 region. The results are compared with Total Routhian Surface and Cranked Nilsson-Strutinsky calculations.

Excited states in 217Ra populated in the α decay of 221Th

Fine structure in the α decay of 22190Th, populating excited states in 21788Ra, was studied using αγ-coincidence spectroscopy. Two α-decay branches from 221Th have been newly observed, with Eα(keV)[bα(%)]=7951(8)[0.14(3)] and 8247(3)[1.51(12)], together with three previously known branches. Also, two new states in 217Ra were identified at E = 177 and 227 keV. The ground-state configurations of the odd-A, N = 131 transitional isotones above 208Pb are interpreted from their α-decay fine structure systematics and considered in terms of predictions using spherical shell and reflection-asymmetric models. peerReviewed

α-decay spectroscopy of the N = 130 isotones 218Ra and 220Th: Mitigation of α-particle energy summing with implanted nuclei

An analysis technique has been developed in order to mitigate energy summing due to sequential short-lived α decays from nuclei implanted into a silicon detector. Using this technique, α-decay spectroscopy of the N=130 isotones 218Ra (Z=88) and 220Th (Z=90) has been performed. The energies of the α particles emitted in the 218Ra→214Rn and 220Th→216Ra ground-state-to-ground-state decays have been measured to be 8381(4) keV and 8818(13) keV, respectively. The half-lives of the ground states of 218Ra and 220Th have been measured to be 25.99(10) μs and 10.4(4) μs, respectively. The half-lives of the ground states of the α-decay daughters, 214Rn and 216Ra, have been measured to be 259(3) ns and …

Delayed or absent π(h11/2)2 alignment in 111Xe

Excited states have been identified in the very neutron-deficient N = Z + 3 nucleus 111Xe for the first time, using the 58Ni(58Ni, αn) heavy-ion fusion-evaporation reaction. γ -ray transitions have been unambiguously assigned to 111Xe by correlation with the characteristic 111Xe → 107Te → 103Sn α-decay chain using the method of recoil-decay tagging. Inspection of γ γ -coincidence data has shown that five of the transitions form a rotational-like sequence. Excitation-energy systematics suggest that the sequence could be the favored signature partner of a band built on an h11/2 neutron. Aligned angular momenta of states in the band have been compared to analogous bands in neighboring xenon is…

Population of a low-spin positive-parity band from high-spin intruder states in Au: The two-state mixing effect

The extremely neutron-deficient isotopes $^{177,179}$Au were studied by means of in-beam γ-ray spectroscopy. Specific tagging techniques, α-decay tagging in $^{177}$Au and isomer tagging in $^{179}$Au, were used for these studies. Feeding of positive-parity, nearly spherical states, which are associated with 2d3/2 and 3s1/2 proton-hole configurations, from the 1i13/2 proton-intruder configuration was observed in $^{177}$Au. Such a decay path has no precedent in odd-Au isotopes and it is explained by the effect of mixing of wave functions of the initial state.

Nanosecond-Scale Proton Emission from Strongly Oblate-Deformed ^{149}Lu.

Using the fusion-evaporation reaction ^{96}Ru(^{58}Ni,p4n)^{149}Lu and the MARA vacuum-mode recoil separator, a new proton-emitting isotope ^{149}Lu has been identified. The measured decay Q value of 1920(20) keV is the highest measured for a ground-state proton decay, and it naturally leads to the shortest directly measured half-life of 450_{-100}^{+170}  ns for a ground-state proton emitter. The decay rate is consistent with l_{p}=5 emission, suggesting a dominant πh_{11/2} component for the wave function of the proton-emitting state. Through nonadiabatic quasiparticle calculations it was concluded that ^{149}Lu is the most oblate deformed proton emitter observed to date.

Application of ultra-fast timing techniques to the study of exotic and weakly produced nuclei

Ultra-fast time-delayed techniques have been recently applied in a number of studies where exotic nuclei were identified using advanced selection techniques. These include large Compton-suppressed Ge arrays, in-flight separators or recoil separators. Some of the new results are discussed in this presentation. Besides the results for $^{32}$Mg and $^{96}$Pd, they include the first determination of the half-life of the $8^+$ state in $^{80}$Ge, $T_1/2$ = 2.95(6) ns, and significantly more precise results for $^{51}$Mn (3680 keV level) and $^{48}$V (421 keV level), $T_1/2$ = 1760(40) ps and $T_1/2$ $\leq$ 135 ps, respectively. Development of new scintillators will steadily improve precision an…

Single-particle states and parity doublets in odd-Z 221Ac and 225Pa from α-decay spectroscopy

Low-lying states in the odd-Z isotopes 22189Ac132 and 22591Pa134 have been studied using α-particle and αγ-coincidence spectroscopy in the 225Pa→221Ac→217Fr decay chain. Ground-state spin and parity assignments of Iπ = 5/2− are proposed for both 221Ac and 225Pa, with the odd proton occupying the Ω = 5/2 orbital of the quadrupole-octupole deformed shell model in both nuclei. In 221Ac, excited states in the bands based on the Ω = 5/2 and Ω = 3/2 orbitals have been identified, including proposed parity-doublet states. The results suggest that reflection-asymmetric deformation of the ground state persists in the odd-A members of the isotope chains down to N = 132 for Ac and N = 134 for Pa, befo…

Experimental study of 1/2(+) isomers in At-199,At-201

Using fusion-evaporation reactions, a gas-filled recoil separator, and recoil-electron and recoil-electron-alpha tagging techniques, a new isomeric 1/2(+) state [T-1/2 = 45(3) ms] in At-201 is identified, and an earlier reported corresponding state [T-1/2 = 273(9) ms] in At-199 is confirmed. The 1/2(+) state is suggested to originate from an intruder pi(s(1/2))(-1) configuration. In addition, nuclear structure of states below and above this 1/2(+) state are studied in both nuclei. The isomer decays through a cascade of an E3 transition followed by a mixed M1/E2 transition to the 9/2(-) ground state, and it is interpreted to be fed from nearly spherical 3/2(+) and 5/2(+) states originating f…

The influence of quasineutron configurations on 161Ta and nearby odd-A Nuclei

Several strongly coupled bands in the neutron‐deficient nucleus 161Ta have been identified and quasiparticle configuration assignments have been made on the basis of rotational alignments and cranked shell model calculations. The level scheme elucidated for 161Ta highlights the competition between the ν(h9/2) and ν(i13/2) orbitals to form the yrast spectrum. The band structures in 161Ta also provide new insights into the structural features of other heavy odd‐A nuclei populated with much lower reaction cross sections in this region at the proton drip line.

117番元素Ts合成のための48Ca+249Bk融合反応

We have performed an experiment to synthesize the element 117 (Ts) with the $^{48}$Ca+$^{249}$Bk fusion reaction. Four $\alpha$-decay chains attributed to the element 117 were observed. Two of them were long decay chains which can be assigned to the one originating from the $\alpha$ decay of $^{294}$Ts. The other two were short decay chains which are consistent with the one originating from the $\alpha$ decay of $^{293}$Ts. We have compared the present results with the literature data, and found that our present results mostly confirmed the literature data, leading to the firm confirmation of the synthesis of the element 117.