0000000000433406
AUTHOR
Damir Dominko
Static and dynamic properties of low-temperature order in the one-dimensional semiconductor(NbSe4)3I
We investigated static and dynamic lattice properties in a quasi-one-dimensional charge-ordered semiconductor ${({\mathrm{NbSe}}_{4})}_{3}\mathrm{I}$ by using Raman, femtosecond pump-probe spectroscopy and x-ray diffraction. In addition to a well-documented pseudo-Jahn-Teller ferrodistortive structural transition at ${T}_{C}=274$ K, where the displacements of Nb ions lead to ferroelectric (FE) in-chain polarization with opposite direction in adjacent chains, all methods suggest an additional lowering of symmetry at ${T}^{*}\ensuremath{\approx}160$ K. Although antiferroelectric (AFE) phase is partially formed at ${T}_{C}$, our results consistently point to an enhancement of the interchain or…
Optical control of vibrational coherence triggered by an ultrafast phase transition
Femtosecond time-resolved x-ray diffraction is employed to study the dynamics of the periodic lattice distortion (PLD) associated with the charge-density-wave (CDW) in K0.3MoO3. Using a multi-pulse scheme we show the ability to extend the lifetime of coherent oscillations of the PLD about the undistorted structure through re-excitation of the electronic states. This suggests that it is possible to enter a regime where the symmetry of the potential energy landscape corresponds to the high symmetry phase but the scattering pathways that lead to the damping of coherent dynamics are still controllable by altering the electronic state population. The demonstrated control over the coherence time …
Néel Spin-Orbit Torque Driven Antiferromagnetic Resonance in Mn2Au Probed by Time-Domain THz Spectroscopy
We observe the excitation of collective modes in the terahertz (THz) range driven by the recently discovered Neel spin-orbit torques (NSOTs) in the metallic antiferromagnet Mn_{2}Au. Temperature-dependent THz spectroscopy reveals a strong absorption mode centered near 1 THz, which upon heating from 4 to 450 K softens and loses intensity. A comparison with the estimated eigenmode frequencies implies that the observed mode is an in-plane antiferromagnetic resonance (AFMR). The AFMR absorption strength exceeds those found in antiferromagnetic insulators, driven by the magnetic field of the THz radiation, by 3 orders of magnitude. Based on this and the agreement with our theory modeling, we inf…
Single crystal-like thin films of blue bronze
Abstract Pulsed laser deposition technique was employed to grow thin films of K 0.3 M o O 3 on A l 2 O 3 (1-102) and S r T i O 3 (510) substrates. Structural and imaging characterization revealed good quality films with well oriented grains of few microns in length. Both non-selective (transport) and order-selective (femtosecond pump-probe spectroscopy) probes revealed charge density wave properties that are very close to those of the single crystals. The films exhibit metal-semiconductor phase transition in resistivity, pump-probe data show phase transition at the same temperature as the single crystal and the threshold for the photo-induced phase transition is approximately the same as in…