0000000000464546
AUTHOR
Md. Z. Hoque
Stratégies de contrôle pour la manipulation spatiale de molécules
Talk given by E. Hertz; National audience
Observation of laser-induced field-free permanent planar alignment of molecules
International audience; Permanent planar alignment of gas-phase linear molecules is achieved by a pair of delayed perpendicularly polarized short laser pulses. The experiment is performed in a supersonic jet, ensuring a relatively high number density of molecules with moderately low rotational temperature. The effect is optically probed on a femtosecond time scale by the use of a third short pulse, enabling a time-resolved birefringence detection performed successively in two perpendicular planes of the laboratory frame. The technique allows for an unambiguous estimation of the molecular planar delocalization produced within the polarization plane of the pulse pair after the turn-off of the…