Absolute measurement of quadratic nonlinearities from phase-matched second-harmonic generation in a single KTP crystal cut as a sphere
We determine within an accuracy of ∼10% the absolute magnitude of the quadratic effective coefficients of types I and II phase-matched second-harmonic generation from conversion efficiency measurements in a single nonlinear crystal cut as a sphere. The agreement is good with measurements performed in thin parallelepipedal samples. The material studied is KTiOPO4, for which improved Sellmeier equations are given.
Optimized blue light generation in optically contacted walk-off compensated RbTiOAsO4 and KTiOP1−yAsyO4
Abstract We study type II 1.32 μm second harmonic generation (SHG) in a RbTiOAsO 4 optically contacted walk-off compensated device. The reduction of the effective walk-off angle by a factor of 3.7 with respect to KTiOPO 4 for the same interaction leads to an enhancement by a factor of 10 of the conversion efficiency. A model is proposed for both type I and type II SHG in such a structure. The angular tuning curve is a multi-peaked one, as predicted by the model. The enhancement of the SHG conversion efficiency allows us to optimize the generation of blue laser light at 440 nm: a specially designed KTiOP 0.98 As 0.02 O 4 solid solution crystal achieves angular non-critical phase matching at …
Optical, thermal, electrical, damage, and phase-matching properties of lithium selenoindate
LiInSe2, a biaxial nonlinear crystal transparent from 0.54 to 10 µm, is successfully grown in large sizes with good optical quality. We summarize all characteristics and physical properties of LiInSe2 essential for nonlinear frequency conversion.
Optical, thermal, electrical, damage, and phase-matching properties of lithium selenoindate
Lithium selenoindate (LiInSe2) is a new nonlinear chalcogenide biaxial crystal, related to LiInS2 and transparent from 0.54 to 10 μm at the 50% level (10 mm thickness), which has been successfully grown in large sizes and with good optical quality. We report on what we believe to be new physical properties that are relevant for laser and nonlinear optical applications and summarize all relevant characteristics, both from the literature and as measured in the present work. With respect to AgGaS(e)2 ternary chalcopyrite materials, LiInSe2 displays a nearly isotropic thermal expansion behavior with three- to five-times-larger thermal conductivities associated with high optical damage threshold…