0000000000524739

AUTHOR

David Leimbach

0000-0002-4587-1067

showing 4 related works from this author

Nuclear moments put a new spin on the structure of 131In

2021

Abstract In spite of the high-density and strongly correlated nature of the atomic nucleus, experimental and theoretical evidence suggests that around particular 'magic' numbers of nucleons, nuclear properties are governed by a single unpaired nucleon1,2. A microscopic understanding of the extent of this behaviour and its evolution in neutron-rich nuclei remains an open question in nuclear physics 3-5. A textbook example is the electromagnetic moments of indium (Z = 49) 6, which are dominated by a hole with respect to the proton magic number Z = 50 nucleus. They exhibit a remarkably constant behaviour over a large range of odd-mass isotopes, previously interpreted as pure "single-particle b…

PhysicsCondensed matter physicsNuclear TheoryStructure (category theory)Nuclear ExperimentSpin-½
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Upgrades of the GANDALPH photodetachment detector towards the determination of the electron affinity of astatine

2020

The Gothenburg ANion Detector for Affinity measurements by Laser PHotodetachment (GANDALPH) has recently been built for measurements of electron affinities (EA) of radioisotopes. A first measurement campaign is aimed towards the determination of the EA of astatine, the rarest naturally occurring element on earth. In this work we present several upgrades of GANDALPH which have been implemented in order to facilitate EA measurements of radioisotopes where only low intensity ion beams (< 1pA) can be produced.

0303 health sciencesNuclear and High Energy PhysicsMaterials scienceDetectorchemistry.chemical_elementLaser01 natural scienceslaw.inventionIon03 medical and health scienceschemistrylawElectron affinity0103 physical sciencesAtomic physics010306 general physicsAstatineInstrumentation030304 developmental biologyNuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms
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A graphene-based neutral particle detector

2019

A neutral particle detector is presented, in which the traditionally used target material, indium tin oxide (ITO), is replaced by graphene. The graphene-based detector enables collinear photodetachment measurements at a significantly shorter wavelength of light down to 230 nm compared to ITO-based detectors, which are limited at 335 nm. Moreover, the background signal from the photoelectric effect is drastically reduced when using graphene. The graphene based detector, reaching 1.7 eV further into the UV energy range, allows increased possibilities for photodetachment studies of negatively charged atoms, molecules, and clusters.A neutral particle detector is presented, in which the traditio…

010302 applied physicsRange (particle radiation)Materials sciencePhysics and Astronomy (miscellaneous)business.industryGrapheneDetector02 engineering and technologyPhotoelectric effect021001 nanoscience & nanotechnology01 natural sciencesSignallaw.inventionIndium tin oxideWavelengthlaw0103 physical sciencesOptoelectronics0210 nano-technologybusinessNeutral particleApplied Physics Letters
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The electron affinity of astatine

2020

One of the most important properties influencing the chemical behavior of an element is the electron affinity (EA). Among the remaining elements with unknown EA is astatine, where one of its isotopes, 211At, is remarkably well suited for targeted radionuclide therapy of cancer. With the At− anion being involved in many aspects of current astatine labeling protocols, the knowledge of the electron affinity of this element is of prime importance. Here we report the measured value of the EA of astatine to be 2.41578(7) eV. This result is compared to state-of-the-art relativistic quantum mechanical calculations that incorporate both the Breit and the quantum electrodynamics (QED) corrections and…

Atomic Physics (physics.atom-ph)ENERGIESGeneral Physics and AstronomyElectron01 natural sciences7. Clean energyPhysics - Atomic PhysicsElectronegativityastatiinielectron affinityPhysics::Atomic Physicslcsh:SciencePhysicsMultidisciplinary010304 chemical physicsIsotopeQELECTRONEGATIVITYMultidisciplinary SciencesHalogenScience & Technology - Other Topicsddc:500Atomic physicsBASIS-SET CONVERGENCE[CHIM.RADIO]Chemical Sciences/RadiochemistryRadioactive decayChemical physicsAstrophysics::High Energy Astrophysical PhenomenaScienceComputer Science::Neural and Evolutionary ComputationOther Fields of PhysicsPOTENTIALSFOS: Physical scienceschemistry.chemical_elementphysics.atom-phGeneral Biochemistry Genetics and Molecular BiologyArticleIonElectron affinity0103 physical sciences[CHIM]Chemical Sciences010306 general physicsAstatineDETECTORScience & TechnologySTABILITYRadiochemistry500General Chemistrychemistrylcsh:Qastatine
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