showing 51 related works from this author
Total absorption γ -ray spectroscopy of niobium isomers
2019
15 pags. 17 figs., 5 tabs.
Total absorption studies of high priority decays for reactor applications: 86Br and 91Rb
2017
Preliminary results from beta decay studies of nuclei that are important for reactor applications are presented. The beta decays have been studied using the total absorption technique (TAS) and the pure beams provided by the JYFLTRAP system at the IGISOL facility of the University of Jyväskylä. peerReviewed
New accurate measurements of neutron emission probabilities for relevant fission products
2017
We have performed new accurate measurements of the beta-delayed neutron emission probability for ten isotopes of the elements Y, Sb, Te and I. These are fission products that either have a significant contribution to the fraction of delayed neutrons in reactors or are relatively close to the path of the astrophysical r process. The measurements were performed with isotopically pure radioactive beams using a constant and high efficiency neutron counter and a low noise beta detector. Preliminary results are presented for six of the isotopes and compared with previous measurements and theoretical calculations. peerReviewed
The laser and optical system for the RIBF-PALIS experiment
2017
Abstract This paper describes the laser and optical system for the Parasitic radioactive isotope (RI) beam production by Laser Ion-Source (PALIS) in the RIKEN fragment separator facility. This system requires an optical path length of 70 m for transporting the laser beam from the laser light source to the place for resonance ionization. To accomplish this, we designed and implemented a simple optical system consisting of several mirrors equipped with compact stepping motor actuators, lenses, beam spot screens and network cameras. The system enables multi-step laser resonance ionization in the gas cell and gas jet via overlap with a diameter of a few millimeters, between the laser photons an…
Multi-nucleon transfer reactions at ion catcher facilities : a new way to produce and study heavy neutron-rich nuclei
2020
Abstract The production of very neutron-rich nuclides heavier than fission fragments is an ongoing experimental challenge. Multi-nucleon transfer reactions (MNT) have been suggested as a method to produce these nuclides. By thermalizing the reaction products in gas-filled stopping cells, we can deliver them as cooled high-quality beams to decay, laser and mass spectrometry experiments. High precision mass spectrometry will allow for the first time to universally and unambiguously identify the atomic and proton numbers of the ions produced in MNT reactions. In this way their ground and isomeric state properties can be studied in high-precision measurements. In experiments at IGISOL, Finland …
Experimental evidence on photo-assisted O− ion production from Al2O3 cathode in cesium sputter negative ion source
2020
The production of negative ions in cesium sputter ion sources is generally considered to be a pure surface process. It has been recently proposed that ion pair production could explain the higher-than-expected beam currents extracted from these ion sources, therefore opening the door for laser-assisted enhancement of the negative ion yield. We have tested this hypothesis by measuring the effect of various pulsed diode lasers on the O − beam current produced from Al 2O 3 cathode of a cesium sputter ion source. It is expected that the ion pair production of O − requires populating the 5d electronic states of neutral cesium, thus implying that the process should be provoked only with specific …
Electron capture on116In and implications for nuclear structure related to double-βdecay
2013
The electron capture decay branch of ${}^{116}$In has been measured to be $[2.46\ifmmode\pm\else\textpm\fi{}0.44(\mathrm{stat}.)\ifmmode\pm\else\textpm\fi{}0.39(\mathrm{syst}.)]\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}4}$ using Penning trap-assisted decay spectroscopy. The corresponding Gamow-Teller transition strength is shown to be compatible with the most recent value extracted from the $(p,n)$ charge-exchange reaction, providing a resolution to longstanding discrepancies. This transition can now be used as a reliable benchmark for nuclear-structure calculations of the matrix element for the neutrinoless double-$\ensuremath{\beta}$ decay of ${}^{116}$Cd and other nuclides.
Upgrades to the collinear laser spectroscopy experiment at the IGISOL
2020
Abstract We give an overview of recent changes to the collinear laser spectroscopy beamline in the IGISOL laboratory. We present a new data acquisition system, commissioning of a newly installed charge exchange cell, and cooler-voltage calibration measurements. Currently ongoing modifications to the RFQ cooler-buncher are also discussed.
Strong γ-ray emission from neutron unbound states populated in β-decay: Impact on (n,γ) cross-section estimates
2017
J. L. Taín et al. -- 6 pags., 7 figs., 1 tab. -- Open Access funded by Creative Commons Atribution Licence 4.0
Total Absorption Spectroscopy of Fission Fragments Relevant for Reactor Antineutrino Spectra and Decay Heat Calculations
2015
Volume: 111 Host publication title: WONDER-2015 Host publication sub-title: 4TH INTERNATIONAL WORKSHOP ON NUCLEAR DATA EVALUATION FOR REACTOR APPLICATIONS Isbn(print): 978-2-7598-1970-6 Beta decay of fission products is at the origin of decay heat and antineutrino emission in nuclear reactors. Decay heat represents about 7% of the reactor power during operation and strongly impacts reactor safety. Reactor antineutrino detection is used in several fundamental neutrino physics experiments and it can also be used for reactor monitoring and non-proliferation purposes. Rb-92,Rb-93 are two fission products of importance in reactor antineutrino spectra and decay heat, but their beta-decay properti…
Total absorption spectroscopy of fission fragments relevant for reactor antineutrino spectra
2016
International audience; The accurate determination of reactor antineutrino spectra remains a very active research topic for which new methods of study have emerged in recent years. Indeed, following the long-recognized reactor anomaly (measured antineutrino deficit in short baseline reactor experiments when compared with spectral predictions), the three international reactor neutrino experiments Double Chooz, Daya Bay and Reno have recently demonstrated the existence of spectral distortions in their measurements with respect to the same predictions. These spectral predictions were obtained through the conversion of integral beta-energy spectra obtained at the ILL research reactor. Several s…
Radioactive ion beam manipulation at the IGISOL-4 facility
2020
The IGISOL-4 facility in the JYFL Accelerator Laboratory of the University of Jyvaskyla (JYFL-ACCLAB) produces low-energy radioactive ion beams, primarily for nuclear spectroscopy, utilizing an ion guide-based, ISOL-type mass separator. Recently, new ion manipulation techniques have been introduced at the IGISOL-4 including the application of the PI-ICR (Phase-Imaging Ion Cyclotron Resonance) technique at the JYFLTRAP Penning trap, as well as commissioning of a Multi-Reflection Time-Of-Flight (MR-TOF) separator/spectrometer. The successful operation of the MR-TOF also required significant improvement of the Radio-Frequency Quadrupole (RFQ) cooler and buncher device beam pulse time structure…
Characterization of a neutron-beta counting system with beta-delayed neutron emitters
2016
Abstract A new detection system for the measurement of beta-delayed neutron emission probabilities has been characterized using fission products with well known β-delayed neutron emission properties. The setup consists of BELEN-20, a 4π neutron counter with twenty 3He proportional tubes arranged inside a large polyethylene neutron moderator, a thin Si detector for β counting and a self-triggering digital data acquisition system. The use of delayed-neutron precursors with different neutron emission windows allowed the study of the effect of energy dependency on neutron, β and β–neutron rates. The observed effect is well reproduced by Monte Carlo simulations. The impact of this dependency on …
Isomer and decay studies for the rp process at IGISOL
2012
This article reviews the decay studies of neutron-deficient nuclei within the mass region \ensuremathA=56--100 performed at the Ion-Guide Isotope Separator On-Line (IGISOL) facility in the University of Jyväskylä over last 25 years. Development from He-jet measurements to on-line mass spectrometry, and eventually to atomic mass measurements and post-trap spectroscopy at IGISOL, has yielded studies of around 100 neutron-deficient nuclei over the years. The studies form a solid foundation to astrophysical rp -process path modelling. The focus is on isomers studied either via spectroscopy or via Penning-trap mass measurements. The review is complemented with recent results on the ground and is…
Exploring the mass surface near the rare-earth abundance peak via precision mass measurements at JYFLTRAP
2019
The JYFLTRAP double Penning trap at the Ion Guide Isotope Separator On-Line (IGISOL) facility has been used to measure the atomic masses of 13 neutron-rich rare-earth isotopes. Eight of the nuclides, $^{161}$Pm, $^{163}$Sm, $^{164,165}$Eu, $^{167}$Gd, and $^{165,167,168}$Tb, were measured for the first time. The systematics of the mass surface has been studied via one- and two-neutron separation energies as well as neutron pairing-gap and shell-gap energies. The proton-neutron pairing strength has also been investigated. The impact of the new mass values on the astrophysical rapid neutron capture process has been studied. The calculated abundance distribution results in a better agreement w…
New insights into triaxiality and shape coexistence from odd-mass Rh109
2018
Rapid shape evolutions near A = 100 are now the focus of much attention in nuclear science. Much of the recent work has been centered on isotopes with Z <= 40, where the shapes are observed to transition between near-spherical to highly deformed with only a single pair of neutrons added. At higher Z, the shape transitions become more gradual as triaxiality sets in, yet the coexistence of varying shapes continues to play an important role in the low-energy nuclear structure, particularly in the odd-Z isotopes. This work aims to characterize competing shapes in the triaxial region between Zr and Sn isotopes using ultrafast timing techniques to measure lifetimes of excited states in the neutro…
Isotope shifts from collinear laser spectroscopy of doubly charged yttrium isotopes
2018
Collinear laser spectroscopy has been performed on doubly charged ions of radioactive yttrium in order to study the isotope shifts of the 294.6-nm $5s\phantom{\rule{0.16em}{0ex}}^{2}S_{1/2}\ensuremath{\rightarrow}5p\phantom{\rule{0.16em}{0ex}}^{2}P_{1/2}$ line. The potential of such an alkali-metal-like transition to improve the reliability of atomic-field-shift and mass-shift factor calculations, and hence the extraction of nuclear mean-square radii, is discussed. Production of yttrium ion beams for such studies is available at the IGISOL IV Accelerator Laboratory, Jyv\"askyl\"a, Finland. This newly recommissioned facility is described here in relation to the on-line study of accelerator-p…
A new off-line ion source facility at IGISOL
2019
An off-line ion source station has been commissioned at the IGISOL (Ion Guide Isotope Separator On-Line) facility. It offers the infrastructure needed to produce stable ion beams from three off-line ion sources in parallel with the radioactive ion beams produced from the IGISOL target chamber. This has resulted in improved feasibility for new experiments by offering reference ions for Penning-trap mass measurements, laser spectroscopy and atom trap experiments.
High-precision mass measurements and production of neutron-deficient isotopes using heavy-ion beams at IGISOL
2019
An upgraded ion-guide system for the production of neutron-deficient isotopes with heavy-ion beams has been commissioned at the IGISOL facility with an $^{36}\mathrm{Ar}$ beam on a $^{\mathrm{nat}}\mathrm{Ni}$ target. It was used together with the JYFLTRAP double Penning trap to measure the masses of $^{82}\mathrm{Zr}, ^{84}\mathrm{Nb}, ^{86}\mathrm{Mo}, ^{88}\mathrm{Tc}$, and $^{89}\mathrm{Ru}$ ground states and the isomeric state $^{88}\mathrm{Tc}^{m}$. Of these, $^{89}\mathrm{Ru}$ and $^{88}\mathrm{Tc}^{m}$ were measured for the first time. The precision of measurements of $^{82}\mathrm{Zr}, ^{84}\mathrm{Nb}$, and $^{88}\mathrm{Tc}$ was significantly improved. The literature value for $^…
Total absorption γ -ray spectroscopy of the β -delayed neutron emitters Br87 , Br88 , and Rb94
2017
We investigate the decay of 87,88Br and 94Rb using total absorption γ -ray spectroscopy. These important fission products are β-delayed neutron emitters. Our data show considerable βγ intensity, so far unobserved in high-resolution γ -ray spectroscopy, from states at high excitation energy. We also find significant differences with the β intensity that can be deduced from existing measurements of the β spectrum. We evaluate the impact of the present data on reactor decay heat using summation calculations. Although the effect is relatively small it helps to reduce the discrepancy between calculations and integral measurements of the photon component for 235U fission at cooling times in the r…
Characterization and performance of the DTAS detector
2018
11 pags., 16 figs., 3 tabs.
Enhancedγ-Ray Emission from Neutron Unbound States Populated inβDecay
2015
Total absorption spectroscopy is used to investigate the β-decay intensity to states above the neutron separation energy followed by γ-ray emission in (87,88)Br and (94)Rb. Accurate results are obtained thanks to a careful control of systematic errors. An unexpectedly large γ intensity is observed in all three cases extending well beyond the excitation energy region where neutron penetration is hindered by low neutron energy. The γ branching as a function of excitation energy is compared to Hauser-Feshbach model calculations. For (87)Br and (88)Br the γ branching reaches 57% and 20%, respectively, and could be explained as a nuclear structure effect. Some of the states populated in the daug…
First experiment with the NUSTAR/FAIR Decay Total Absorption γ-Ray Spectrometer (DTAS) at the IGISOL IV facility
2015
V. Guadilla et al. ; 4 págs.; 4 figs.; 1 tab.
Characterization of a cylindrical plastic {\beta}-detector with Monte Carlo simulations of optical photons
2017
V. Guadilla et al. -- 5 pags., 8 figs., tab.
Isomeric fission yield ratios for odd-mass Cd and In isotopes using the Phase-Imaging Ion-Cyclotron-Resonance technique
2018
Isomeric yield ratios for the odd-$A$ isotopes of $^{119-127}$Cd and $^{119-127}$In from 25-MeV proton-induced fission on natural uranium have been measured at the JYFLTRAP double Penning trap, by employing the Phase-Imaging Ion-Cyclotron-Resonance technique. With the significantly improved mass resolution of this novel method isomeric states separated by 140 keV from the ground state, and with half-lives of the order of 500 ms, could be resolved. This opens the door for obtaining new information on low-lying isomers, of importance for nuclear structure, fission and astrophysics. In the present work the experimental isomeric yield ratios are used for the estimation of the root-mean-square a…
Intracavity Frequency Doubling and Difference Frequency Mixing for Pulsed ns Ti:Sapphire Laser Systems at On-Line Radioactive Ion Beam Facilities
2015
Intra-cavity second harmonic generation of a Titanium:sapphire (Ti:sa) laser system has been used to improve the conversion efficiency to the second harmonic. Over the course of several experiments performance data spanning the whole wavelength range of a Ti:sa has been collected, which may be used as a guideline for future experiments. An average output power of up to 3.7 W was achieved, resulting in a conversion efficiency of >75 % to the second harmonic. A wavelength coverage from 340-525 nm has been demonstrated. To extend the wavelength range of the solid state laser system, difference frequency mixing has been applied to the intra-cavity doubled light and the fundamental output of a s…
Large Impact of the Decay of Niobium Isomers on the Reactor ν¯e Summation Calculations
2019
Even mass neutron-rich niobium isotopes are among the principal contributors to the reactor antineutrino energy spectrum. They are also among the most challenging to measure due to the refractory nature of niobium, and because they exhibit isomeric states lying very close in energy. The beta-intensity distributions of Nb-100gs,Nb-100m and Nb-102gs,Nb-02m beta decays have been determined using the total absorption.-ray spectroscopy technique. The measurements were performed at the upgraded Ion Guide Isotope Separator On-Line facility at the University of Jyvaskyla. Here, the double Penning trap system JYFLTRAP was employed to disentangle the beta decay of the isomeric states. The new data ob…
Status and development of the MARA low-energy branch
2018
The MARA Low-Energy Branch is under development at the Accelerator Laboratory of the University of Jyvaskylä. The facility will be employed for laser ionisation and spectroscopy studies and for mass measurements of nuclei close to the proton drip line. This article presents an updated status of the ongoing development of the different parts of this facility, including the buffer gas cell, the ion transport system, the laser system and the detector stations. peerReviewed
TAGS measurements of $^{100}$Nb ground and isomeric states and $^{140}$Cs for neutrino physics with the new DTAS detector
2016
V. Guadilla et al. -- 4 pags., 6 figs. -- Open Access funded by Creative Commons Atribution Licence 4.0
Experimental study of 100Tc β decay with total absorption γ -ray spectroscopy
2017
The β decay of 100Tc has been studied by using the total absorption γ -ray spectroscopy technique at the Ion Guide Isotope Separator On-Line facility in Jyväskylä. In this work the new Decay Total Absorption γ -ray Spectrometer in coincidence with a cylindrical plastic β detector has been employed. The β intensity to the ground state obtained from the analysis is in good agreement with previous high-resolution measurements. However, differences in the feeding to the first-excited state as well as weak feeding to a new level at high excitation energy have been deduced from this experiment. Theoretical calculations performed in the quasiparticle random-phase approximation framework are also r…
Study of the β decay of fission products with the DTAS detector
2017
Total Absorption Spectroscopy measurements of the β decay of 103Mo and 103Tc, important contributors to the decay heat summation calculation in reactors, are reported in this work. The analysis of the experiment, performed at IGISOL with the new DTAS detector, show new β intensity that was not detected in previous measurements with Ge detectors. peerReviewed
Characterization of a neutron–beta counting system with beta-delayed neutron emitters
2016
A new detection system for the measurement of beta-delayed neutron emission probabilities has been characterized using fission products with well known β-delayed neutron emission properties. The setup consists of BELEN-20, a 4π neutron counter with twenty 3He proportional tubes arranged inside a large polyethylene neutron moderator, a thin Si detector for β counting and a selftriggering digital data acquisition system. The use of delayed-neutron precursors with different neutron emission windows allowed the study of the effect of energy dependency on neutron, β and β-neutron rates. The observed effect is well reproduced by Monte Carlo simulations. The impact of this dependency on the accura…
Photo-enhanced O−, H− and Br− ion production in caesium sputter negative ion source : no evidence for resonant ion pair production
2022
It has been proposed that the negative ion yield of a caesium sputter ion source could be enhanced by promoting neutral caesium atoms to electronically excited 7p states supporting resonant ion pair production. We have tested this hypothesis by illuminating the cathode of a caesium sputter ion source with an adjustable wavelength laser and measuring its effect on the extracted beam currents of O−, H− and Br− anions. The laser exposure causes the beam currents to increase but the effect is independent of the wavelength in the range of 440-460 nm, which leads us to conclude that there is no evidence for resonant ion pair production. The photon-induced beam current enhancement scales with the …
Large Impact of the Decay of Niobium Isomers on the Reactor ¯νe Summation Calculations
2019
Even mass neutron-rich niobium isotopes are among the principal contributors to the reactor antineutrino energy spectrum. They are also among the most challenging to measure due to the refractory nature of niobium, and because they exhibit isomeric states lying very close in energy. The β-intensity distributions of 100gs;100mNb and 102gs;102mNb β decays have been determined using the total absorption γ-ray spectroscopy technique. The measurements were performed at the upgraded Ion Guide Isotope Separator On-Line facility at the University of Jyväskylä. Here, the double Penning trap system JYFLTRAP was employed to disentangle the β decay of the isomeric states. The new data obtained in this …
Characterization of a cylindrical plastic β-detector with Monte Carlo simulations of optical photons
2017
In this work we report on the Monte Carlo study performed to understand and reproduce experimental measurements of a new plastic β-detector with cylindrical geometry. Since energy deposition simulations differ from the experimental measurements for such a geometry, we show how the simulation of production and transport of optical photons does allow one to obtain the shapes of the experimental spectra. Moreover, taking into account the computational effort associated with this kind of simulation, we develop a method to convert the simulations of energy deposited into light collected, depending only on the interaction point in the detector. This method represents a useful solution when extens…
Resonance laser ionization developments for IGISOL-4
2012
The work presented in this thesis concentrates on the development of the FURIOS laser ion source towards e cient and selective production of low energy radioactive ion beams. This includes design and development of the ion guide and hot cavity catcher systems for laser ion source use, and the development of in-source and in-jet laser spectroscopy techniques. The work has been carried out at the IGISOL facility in the Accelerator laboratory of the University of Jyväskylä. The FURIOS facility was upgraded and developed during the move to the IGISOL-4 facility. The laser transport was greatly improved in order to allow a large fraction of the initial laser intensity to be transported into the …
Precise measurements of half-lives and branching ratios for the ββ mirror transitions in the decay of 23Mg and 27Si
2017
Half-lives and branching ratios for the two mirror ββ decays of 23Mg and 27Si have been measured at the University of Jyväskylä with the IGISOL facility. The results obtained, T1/2=11.303(3)T1/2=11.303(3) s and T1/2=4.112(2)T1/2=4.112(2) s for the half-lives of 23Mg and 27Si , respectively, are 7 and 8 times more precise than the averages of previous measurements. The values obtained for the super-allowed branching ratios of 23Mg and 27Si are B.R.=92.18(8)%B.R.=92.18(8)% and B.R.=99.74(2)%B.R.=99.74(2)% , respectively. The result for 23Mg is three times more precise than the average of the previous measurements, while for 27Si the precision has not been improved, the average of the previous…
Total absorption γ-ray spectroscopy of the β-delayed neutron emitters 87Br, 88Br, and 94Rb
2017
We investigate the decay of 87,88Br and 94Rb using total absorption γ -ray spectroscopy. These important fission products are β-delayed neutron emitters. Our data show considerable βγ intensity, so far unobserved in high-resolution γ -ray spectroscopy, from states at high excitation energy. We also find significant differences with the β intensity that can be deduced from existing measurements of the β spectrum. We evaluate the impact of the present data on reactor decay heat using summation calculations. Although the effect is relatively small it helps to reduce the discrepancy between calculations and integral measurements of the photon component for 235U fission at cooling times in the r…
The electron affinity of astatine
2020
One of the most important properties influencing the chemical behavior of an element is the electron affinity (EA). Among the remaining elements with unknown EA is astatine, where one of its isotopes, 211At, is remarkably well suited for targeted radionuclide therapy of cancer. With the At− anion being involved in many aspects of current astatine labeling protocols, the knowledge of the electron affinity of this element is of prime importance. Here we report the measured value of the EA of astatine to be 2.41578(7) eV. This result is compared to state-of-the-art relativistic quantum mechanical calculations that incorporate both the Breit and the quantum electrodynamics (QED) corrections and…
Opportunities for Fundamental Physics Research with Radioactive Molecules
2023
Molecules containing short-lived, radioactive nuclei are uniquely positioned to enable a wide range of scientific discoveries in the areas of fundamental symmetries, astrophysics, nuclear structure, and chemistry. Recent advances in the ability to create, cool, and control complex molecules down to the quantum level, along with recent and upcoming advances in radioactive species production at several facilities around the world, create a compelling opportunity to coordinate and combine these efforts to bring precision measurement and control to molecules containing extreme nuclei. In this manuscript, we review the scientific case for studying radioactive molecules, discuss recent atomic, mo…
β Decay of 127Cd and Excited States in 127In
2019
A dedicated spectroscopic study of the β decay of 127Cd was conducted at the IGISOL facility at the University of Jyväskylä. Following high-resolution mass separation in a Penning trap, β−γ−γcoincidences were used to considerably extend the decay scheme of 127In. The β-decaying 3/2+ and 11/2− states in 127Cd have been identified with the 127Cd ground state and the 283-keV isomer. Their respective half-lives have been measured to 0.45(128)s and 0.36(4) s. The experimentally observed βfeeding to excited states of 127In and the decay scheme of 127In are discussed in conjunction with large-scale shell-model calculations. peerReviewed
Total Absorption Spectroscopy of Fission Fragments Relevant for Reactor Antineutrino Spectra and Decay Heat Calculations
2016
Beta decay of fission products is at the origin of decay heat and antineutrino emission in nuclear reactors. Decay heat represents about 7% of the reactor power during operation and strongly impacts reactor safety. Reactor antineutrino detection is used in several fundamental neutrino physics experiments and it can also be used for reactor monitoring and non-proliferation purposes. 92,93Rb are two fission products of importance in reactor antineutrino spectra and decay heat, but their β-decay properties are not well known. New measurements of 92,93Rb β-decay properties have been performed at the IGISOL facility (Jyväskylä, Finland) using Total Absorption Spectroscopy (TAS). TAS is complemen…
RAPTOR : A new collinear laser ionization spectroscopy and laser-radiofrequency double-resonance experiment at the IGISOL facility
2023
RAPTOR, Resonance ionization spectroscopy And Purification Traps for Optimized spectRoscopy, is a new collinear resonance ionization spectroscopy device constructed at the Ion Guide Isotope Separator On-Line (IGISOL) facility at the University of Jyv\"askyl\"a, Finland. By operating at beam energies of under 10 keV, the footprint of the experiment is reduced compared to more traditional collinear laser spectroscopy beamlines. In addition, RAPTOR is coupled to the JYFLTRAP Penning trap mass spectrometer, opening a window to laser-assisted nuclear-state selective purification, serving not only the mass measurement program, but also supporting post-trap decay spectroscopy experiments. Finally,…
Electron capture on 116In and implications for nuclear structure related to double-\beta decay
2013
The electron capture decay branch of 116In has been measured to be [2.46 ± 0.44(stat.) ± 0.39(syst.)] × 10−4 using Penning trap-assisted decay spectroscopy. The corresponding Gamow-Teller transition strength is shown to be compatible with the most recent value extracted from the (p, n) charge-exchange reaction, providing a resolution to longstanding discrepancies. This transition can now be used as a reliable benchmark for nuclearstructure calculations of the matrix element for the neutrinoless double-β decay of 116Cd and other nuclides. peerReviewed
Photo-assisted O− and Al− production with a cesium sputter ion source
2021
It has been recently proposed that the production of negative ions with cesium sputter ion sources could be enhanced by laser-assisted resonant ion pair production. We have tested this hypothesis by measuring the effect of pulsed diode lasers at various wavelengths on the O− and Al− beam current produced from Al2O3 cathode of a cesium sputter ion source. The experimental results provide evidence for the existence of a wavelength-dependent photo-assisted enhancement of negative ion currents but cast doubt on its alleged resonant nature as the effect is observed for both O− and Al− ions at laser energies above a certain threshold. The beam current transients observed during the laser pulses s…
Towards in-jet resonance ionization spectroscopy : An injection-locked Titanium:Sapphire laser system for the PALIS-facility
2018
This article presents a pulsed narrowband injection-locked Titanium:Sapphire laser aimed for high-resolution in-jet resonance ionization spectroscopy at the SLOWRI/PALIS at RIKEN. The laser has been integrated into the PALIS laser laboratory enabling it to be utilized with the existing broadband Titanium:Sapphire and dye lasers. The seed efficiency has been evaluated to be close to unity over the master laser wavelength range ∼ 753 to 791 nm, and the slope efficiency, namely the ratio of the pump power to the output power, was determined to be ∼ 30 % at 780 nm. A two-step ionization scheme with 386.4016 nm first step and 286.731 nm second step into an autoionizing state was developed for re…
New lifetime measurements in 109 Pd and the onset of deformation at N = 60
2015
Several new subnanosecond lifetimes were measured in 109Pd using the fast-timing βγγ (t) method. Fission fragments of the A = 109 mass chain were produced by bombarding natural uranium with 30 MeV protons at the Jyvaskyl ¨ a Ion Guide Isotope Separator On-Line (IGISOL) facility. Lifetimes were obtained for excited states ¨ in 109Pd populated following β decay of 109Rh. The new lifetimes provide some insight into the evolution of nuclear structure in this mass region. In particular, the distinct structure of the two low-lying 7/2+ states occurring systematically across the Pd isotopic chain is supported by the new lifetime measurements. The available nuclear data indicate a sudden increase i…
r Process (n, γ) Rate Constraints from the γ Emission of Neutron Unbound States in β decay
2017
Total absorption gamma-ray spectroscopy is used to measure accurately the intensity of γγ emission from neutron-unbound states populated in the ββ-decay of delayed-neutron emitters. From the comparison of this intensity with the intensity of neutron emission a constraint on the (n, γγ) cross section for highly unstable neutron-rich nuclei can be deduced. A surprisingly large γγ branching was observed for a number of isotopes which might indicate the need to increase by a large factor the Hauser-Feshbach (n, γγ) cross-section estimates that impact on r process abundance calculations. peerReviewed