0000000000528279
AUTHOR
Barbara Früh
Actinic Radiation and Photolysis Processes in the Lower Troposphere: Effect of Clouds and Aerosols
Within the German Tropospheric Research Program (TFS) a series of projects were performed focussing on aspects of radiation transfer and the effects of UV-radiation on air chemistry. The individual projects covered laboratory investigations, instrument development for photolysis processes as well as field studies of actinic radiation and comparison to model calculations. One and three-dimensional models were tested against field campaign data. The results confirm the improvement of measurement technology achieved through deployment of new techniques like spectroradiometry that offer a wider range of investigations than was previously attainable using chemical actinometry or fixed wavelength…
Ground-based measured and calculated spectra of actinic flux density and downward UV irradiance in cloudless conditions and their sensitivity to aerosol microphysical properties
Ground-based spectral measurements of actinic flux density (300–660 nm wavelength) and downward UV irradiance (300–324 nm) under cloudless conditions have been compared with the results of one-dimensional radiative transfer calculations employing concurrent airborne vertical profile measurements of aerosol particle size distributions. Good agreement (within ±10%) between measured and calculated spectra was found. The remaining differences were explained by uncertainties inherent in the aerosol particle microphysical input data and the column ozone content. A respective sensitivity analysis of the calculated spectra, which was based on the observed variability of microphysical properties, ha…
Measurement-based J(NO2) sensitivity in a cloudless atmosphere under low aerosol loading and high solar zenith angle conditions
Abstract The comparison between measured and simulated photodissociation frequencies of NO 2 , J( NO 2 ) , in a cloudless atmosphere in a recent paper by Fruh et al., 2000 (Journal of Geophysical Research 105, 9843–9857) revealed an overestimation of J(NO2) near ground level by model calculations compared with measurements and an underestimation in the upper part of the aerosol layer. A possible reason for the disagreement is the changing sun position during the vertical ascent. To resolve this problem we carried out a sensitivity study varying the solar zenith angle of 74° by 1.4° (which corresponds to the change of sun position during the vertical flight patterns). This results in a consi…
Precipitation and Temperature
Climatological studies indicate that climate change lead to an increase in the mean global temperature of around 0.5 °C until the end of the twentieth century. This warming impacts the atmospheric humidity, wind, radiation, and precipitation. However, the magnitude of changes is not equally distributed over the globe but differs markedly with regions, making a regionalization of the global information essential. The GLOWA-Danube project follows such a downscaling approach with the focus on the drainage basin of the Upper Danube River.
Three-dimensional solar radiation effects on the actinic flux field in a biomass-burning plume
[1] Three-dimensional (3-D) solar radiative transfer models describe radiative transfer under inhomogeneous atmospheric conditions more accurately than the commonly used one-dimensional (1-D) radiative transfer models that assume horizontal homogeneity of the atmosphere. Here results of 3-D radiative transfer simulations for a biomass-burning plume are presented and compared with local one-dimensional (l-1-D) simulations, i.e., 1-D simulations in every column of the model domain. The spatial distribution of the aerosol particles was derived from a 3-D atmospheric transport simulation. We studied the impact of 3-D radiative effects on the actinic flux within the plume center. The differences…
A pragmatic approach for downscaling precipitation in alpine-scale complex terrain
A statistical method is presented to downscale precipitation from a mesoscale atmospheric model simulation. The algorithm consists of two steps. First, local subscale variability is estimated based on a high resolution observed climatology. Second, there is a bias correction, which constrains the downscaled model climatology to be equal to the observed climatology on the coarse grid. Combining both steps results in a local scaling factor for each day of the climatological year. The method is applied to the upper Danube catchment which encompasses part of the European Alps and which is characterized by highly complex orography. The subgrid-scale variability described by the first part of the…