0000000000588093
AUTHOR
H Sirringhaus
Tuning the effective spin-orbit coupling in molecular semiconductors
The control of spins and spin to charge conversion in organics requires understanding the molecular spin-orbit coupling (SOC), and a means to tune its strength. However, quantifying SOC strengths indirectly through spin relaxation effects has proven diffi- cult due to competing relaxation mechanisms. Here we present a systematic study of the g-tensor shift in molecular semiconductors and link it directly to the SOC strength in a series of high mobility molecular semiconductors with strong potential for future devices. The results demonstrate a rich variability of the molecular g-shifts with the effective SOC, depending on subtle aspects of molecular composition and structure. We correlate t…
Research data supporting the paper "Tuning the effective spin-orbit coupling in molecular semiconductors"
We here present the data underlying the paper "Tuning the effective spin-orbit coupling in molecular semiconductors" accepted at Nature Communications on 24 February 2017. For contributions of the authors to the data and experimental details, please refer to the original paper.