0000000000595539
AUTHOR
Jean-pierre Hermier
Single-molecule controlled emission in planar plasmonic cavities
International audience; We study the fluorescence emission from single dye molecules in coplanar plasmonic cavities composed of a thin gold film surrounded by two in-plane surface plasmon Bragg mirrors. We first discuss the effect of the presence of Bragg mirrors on the radiation diagram of surface plasmon coupled emission. Then, we investigate the role of the planar cavity size by single-molecule fluorescence lifetime imaging. Experimental data are compared to numerical simulations of the decay rates calculated as a function of the molecule orientation and position within the cavity. The creation of new decay channels by coupling to the cavity modes is also discussed. We measure a plasmoni…
Colloidal Quantum Dot Integrated Light Sources for Plasmon Mediated Photonic Waveguide Excitation
We operate micron-sized CdSe/CdS core–shell quantum dot (QD) clusters deposited onto gold patches as integrated light sources for the excitation of photonic waveguides. The surface plasmon mode launched by the QD fluorescence at the top interface of the gold patches are efficiently coupled to photonic modes sustained by titanium dioxide ridge waveguides. We show that, despite a large effective index difference, the plasmonic and the photonic modes can couple with a very high efficiency provided the vertical offset between the two kinds of waveguides is carefully controlled. Based on the effective index contrast of the plasmonic and the photonic modes, we engineer in-plane integrated hybrid …