0000000000603048

AUTHOR

Margherita Maiuri

showing 2 related works from this author

Strong Exciton-Coherent Phonon Coupling in Single-Layer MoS2

2020

Broadband transient absorption with sub-20fs temporal resolution, supported by ab-initio calculations, quantitatively provides the strength of exciton-coherent phonon coupling in 1L-MoS2, showing a resonant profile around the C exciton.

PhysicsCouplingPhononExcitonCondensed Matter::Mesoscopic Systems and Quantum Hall EffectMolecular physicsPhoton countingCondensed Matter::Materials Sciencesymbols.namesakeTemporal resolutionUltrafast laser spectroscopysymbolsRaman spectroscopyRaman scatteringThe 22nd International Conference on Ultrafast Phenomena 2020
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Strongly Coupled Coherent Phonons in Single-Layer MoS 2

2019

We present a transient absorption setup combining broadband detection over the visible-UV range with high temporal resolution ($\sim$20fs) which is ideally suited to trigger and detect vibrational coherences in different classes of materials. We generate and detect coherent phonons (CPs) in single layer (1L) MoS$_2$, as a representative semiconducting 1L-transition metal dichalcogenide (TMD), where the confined dynamical interaction between excitons and phonons is unexplored. The coherent oscillatory motion of the out-of-plane $A'_{1}$ phonons, triggered by the ultrashort laser pulses, dynamically modulates the excitonic resonances on a timescale of few tens fs. We observe an enhancement by…

ramanspectroscopyPhononExcitonGeneral Physics and AstronomyFOS: Physical sciences02 engineering and technologyApplied Physics (physics.app-ph)thz phonons010402 general chemistry01 natural sciencesMolecular physicssymbols.namesakephotoinduced bandgap renormalizationtransient absorption spectroscopyUltrafast laser spectroscopyMesoscale and Nanoscale Physics (cond-mat.mes-hall)General Materials Sciencepulsesexciton−phonon interactionPhysicsab initio calculationCondensed Matter - Materials ScienceCondensed Matter - Mesoscale and Nanoscale Physicstransition metal dichalcogenidesgrapheneGeneral Engineeringmonolayer mos2ResonanceMaterials Science (cond-mat.mtrl-sci)excitationmonodynamicsPhysics - Applied Physics021001 nanoscience & nanotechnology0104 chemical sciencesAmplitudeOrders of magnitude (time)coherent phononsexciton-phonon interactionsymbols0210 nano-technologyRaman spectroscopyExcitationACS Nano
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