0000000000658987
AUTHOR
S.k. Mitra
A wind tunnel study on the drop-to-particle conversion
Abstract An experimental study was carried out to investigate the processes which occur during drop-to-particle conversion in atmospheric clouds whose drops are evaporating. The experiment was carried out in the Mainz vertical wind tunnel and in a 4-m high fall shaft. Drops consisting of aqueous solutions of NaCl, (NH 4 ) 2 SO 4 , and salts of artificial and natural ocean water, containing various kinds of solid, water-insoluble particles such as clays, were studied. The aerosol particles produced by the evaporation of drops had diameters in the range 0.1–1 μm, 5–20 μm, 40–80 μm and 100–300 μm. The shape and fall mode of these particles are discussed. It was found that the aerosol particles…
A laboratory study on the scavenging of SO2 by snow crystals
Abstract A laboratory experiment is described where the uptake of SO2 by dendritic snow crystals was studied. In a first experimental series the uptake of SO2 was investigated during the growth of the snow crystals from water vapor with and without the presence of H2O2 in the air. In a second series of experiments we studied the uptake of SO2 by snow crystals which had completed their growth. The results of our experiments showed that under both conditions SO2 became scavenged by snow crystals. The uptake of SO2 was particularly pronounced during the growth of the snow crystals, and at temperatures close to 0°C where a quasi-liquid layer exists at the surface of ice. As expected, the SO2 up…