0000000000880568
AUTHOR
Paraskevas Tzallas
Laser-induced field-free alignment of the OCS molecule
We investigate the dynamical alignment of jet-cooled OCS molecules induced by a short laser pulse. The alignment is measured through the orientational contribution of the optical Kerr effect using a second weak laser pulse as a probe. Maximum alignment is observed at conditions close to saturation of ionization. The results are analysed with a quantum mechanical model solving for the rotational dynamics.
Tracking Autoionizing-Wave-Packet Dynamics at the 1-fs Temporal Scale
We present time-resolved studies and Fourier transform spectroscopy of inner-shell excited states undergoing Auger decay and doubly excited autoionizing states, utilizing coherent extreme-ultraviolet (XUV) radiation continua. Series of states spanning a range of ∼4 eV are excited simultaneously. An XUV probe pulse tracks the oscillatory and decaying evolution of the formed wave packet. The Fourier transform of the measured trace reproduces the spectrum of the series. The present work paves the way for ultrabroadband XUV spectroscopy and studies of ultrafast dynamics in all states of matter.