A novel experimental system for the KDK measurement of the 40K decay scheme relevant for rare event searches

Potassium-40 ($^{40}$K) is a long-lived, naturally occurring radioactive isotope. The decay products are prominent backgrounds for many rare event searches, including those involving NaI-based scintillators. $^{40}$K also plays a role in geochronological dating techniques. The branching ratio of the electron capture directly to the ground state of argon-40 has never been measured, which can cause difficulty in interpreting certain results or can lead to lack of precision depending on the field and analysis technique. The KDK (Potassium (K) Decay (DK)) collaboration is measuring this decay. A composite method has a silicon drift detector with an enriched, thermally deposited $^{40}$K source …

Recoil-α-fission and recoil-α–α-fission events observed in the reaction 48Ca + 243Am

Products of the fusion-evaporation reaction 48Ca + 243Am were studied with the TASISpec set-up at the gas-filled separator TASCA at the GSI Helmholtzzentrum für Schwerionenforschung, Darmstadt, Germany. Amongst the detected thirty correlated α-decay chains associated with the production of element Z=115, two recoil-α-fission and five recoil-α-α-fission events were observed. The latter five chains are similar to four such events reported from experiments performed at the Dubna gas-filled separator, and three such events reported from an experiment at the Berkeley gas-filled separator. The four chains observed at the Dubna gas-filled separator were assigned to start from the 2n-evaporation ch…

Low-lying states in Ra219 and Rn215 : Sampling microsecond α -decaying nuclei

Short-lived α-decaying nuclei "northeast" of 208Pb in the chart of nuclides were studied using the reaction 48Ca+243Am with the decay station TASISpec at TASCA, GSI Darmstadt. Decay energies and times from pile-up events were extracted with a tailor-made pulse-shape analysis routine and specific α-decay chains were identified in a correlation analysis. Decay chains starting with the even-even 220Ra and its odd-A neighbors, 219Fr, and 219,221Ra, with a focus on the 219Ra→215Rn decay, were studied by means of α-γ spectroscopy. A revised α-decay scheme of 219Ra is proposed, including a new decay branch from a previously not considered isomeric state at 17 keV excitation energy. Conclusions on …

Development of a Reference Database for Beta-Delayed Neutron Emission

Beta-delayed neutron emission is important for nuclear structure and astrophysics as well as for reactor applications. Significant advances in nuclear experimental techniques in the past two decades have led to a wealth of new measurements that remain to be incorporated in the databases. We report on a coordinated effort to compile and evaluate all the available beta-delayed neutron emission data. The different measurement techniques have been assessed and the data have been compared with semi-microscopic and microscopic-macroscopic models. The new microscopic database has been tested against aggregate total delayed neutron yields, time-dependent group parameters in 6-and 8-group re-present…

Commissioning of the BRIKEN beta-delayed neutron detector for the study of exotic neutron-rich nuclei

Beta-delayed neutron emission (Beta-n) is a form of radioactive decay in which an electron, an anti-neutrino and one or more neutrons are emitted. This process arises if the energy window of the decay Q_Beta is greater than the neutron separation energy S n of the daughter. The probability in each decay of emitting neutrons is called the Pn value. This form of decay plays a key role in the synthesis of chemical elements in the Universe via the rapid neutron capture process, or r-process. The r-process proceeds far from the valley of nuclear stability, and leads to very neutron-rich nuclei that then decay to the line of stability. Most of these nuclei are ßn emitters. The initial abundance d…

New subshell closure atN=58emerging in neutron-rich nuclei beyondNi78

The structure of neutron-rich nuclei beyond $^{78}\mathrm{Ni}$ was studied using postaccelerated radioactive beams of $^{83,84,85}\mathrm{Ga}$ utilizing $\ensuremath{\beta} \ensuremath{\gamma}$ and $\ensuremath{\beta}\ensuremath{-}n \ensuremath{\gamma}$ spectroscopy. Our data, when combined with energy level systematics, suggests a possible new spherical subshell closure at $N=58$ is created by the nearly degenerated $\ensuremath{\nu}3{s}_{1/2}$ and $\ensuremath{\nu}2{d}_{5/2}$ orbitals being well separated from other orbitals above $N=50$. The near degeneracy of these states could be evidenced by isomerism in this region. The energies of the ${2}_{1}^{+}$ and proposed ${4}_{1}^{+}$ states …

Ca48+Bk249Fusion Reaction Leading to ElementZ=117: Long-Livedα-DecayingDb270and Discovery ofLr266

The superheavy element with atomic number Z=117 was produced as an evaporation residue in the 48Ca+249Bk fusion reaction at the gas-filled recoil separator TASCA at GSI Darmstadt, Germany. The radioactive decay of evaporation residues and their α-decay products was studied using a detection setup that allowed measuring decays of single atomic nuclei with half-lives between sub-μs and a few days. Two decay chains comprising seven α decays and a spontaneous fission each were identified and are assigned to the isotope 294-117 and its decay products. A hitherto unknown α-decay branch in 270Db (Z=105) was observed, which populated the new isotope 266Lr (Z=103). The identification of the long-liv…

Shell structure beyond the proton drip line studied via proton emission from deformed 141Ho

Abstract Fine structure in proton emission from the 7 / 2 − [ 523 ] ground state and from the 1 / 2 + [ 411 ] isomer in deformed nucleus 141Ho was studied by means of fusion-evaporation reactions and digital signal processing. Proton transitions to the first excited 2+ state in 140Dy, with the branching ratio of I p g s ( 2 + ) = 0.9 ± 0.2 % and I p m ( 2 + ) = 1.7 ± 0.5 % , were observed. The data are analyzed within the non-adiabatic weak coupling model assuming a large quadrupole deformation of the daughter nucleus 140Dy as predicted by the self-consistent theory. Implications of this result on coexistence effects around N = 74 are discussed. Significant modifications of the proton shell…

The BRIKEN Project: Extensive Measurements of $\beta $-delayed Neutron Emitters for the Astrophysical r Process

An ambitious program to measure decay properties, primarily β-delayed neutron emission probabilities and half-lives, for a significant number of nuclei near or on the path of the rapid neutron capture process, has been launched at the RIKEN Nishina Center. We give here an overview of the status of the project.

β-decay study of150Er,152Yb, and156Yb: Candidates for a monoenergetic neutrino beam facility

The beta decays of ^{150}Er, ^{152}Yb, and ^{156}Yb nuclei are investigated using the total absorption spectroscopy technique. These nuclei can be considered possible candidates for forming the beam of a monoenergetic neutrino beam facility based on the electron capture (EC) decay of radioactive nuclei. Our measurements confirm that for the cases studied, the EC decay proceeds mainly to a single state in the daughter nucleus.

First β -decay spectroscopy of In 135 and new β -decay branches of In 134

Search for elements 119 and 120

A search for production of the superheavy elements with atomic numbers 119 and 120 was performed in the 50Ti+249Bk and 50Ti+249Cf fusion-evaporation reactions, respectively, at the gas-filled recoil separator TASCA at GSI Darmstadt, Germany. Over four months of irradiation, the 249Bk target partially decayed into 249Cf, which allowed for a simultaneous search for both elements. Neither was detected at cross-section sensitivity levels of 65 and 200 fb for the 50Ti+249Bk and 50Ti+249Cf reactions, respectively, at a midtarget beam energy of Elab=281.5 MeV. The nonobservation of elements 119 and 120 is discussed within the concept of fusion-evaporation reactions including various theoretical pr…

β-delayed neutron emission of r-process nuclei at the N = 82 shell closure

This experiment was performed at RI Beam Factory operated by RIKEN Nishina Center and CNS, University of Tokyo. O.H, T.D, P.J.W, C.G.B, C.J.G and D.K would like to thank STFC, UK for support. This research was sponsored in part by the Office of Nuclear Physics, U.S. Department of Energy under Award No. DE-FG02-96ER40983 (UTK) and DEAC05-00OR22725 (ORNL), and by the National Nuclear Security Administration under the Stewardship Science Academic Alliances program through DOE Award No. DENA0002132. This work was supported by National Science Foundation under Grants No. PHY-1430152 (JINA Center for the Evolution of the Elements), No. PHY-1565546 (NSCL), and No. PHY-1714153 (Central Michigan Uni…

Fusion reaction Ca48+Bk249 leading to formation of the element Ts ( Z=117 )

The heaviest currently known nuclei, which have up to 118 protons, have been produced in 48Ca induced reactions with actinide targets. Among them, the element tennessine (Ts), which has 117 protons, has been synthesized by fusing 48Ca with the radioactive target 249Bk, which has a half-life of 327 d. The experiment was performed at the gas-filled recoil separator TASCA. Two long and two short α decay chains were observed. The long chains were attributed to the decay of 294Ts. The possible origin of the short-decay chains is discussed in comparison with the known experimental data. They are found to fit with the decay chain patterns attributed to 293Ts. The present experimental results confi…

Production of very neutron-deficient isotopes near Sn via reactions involving light-particle and cluster emission

Abstract The production of very neutron-deficient isotopes near 100Sn has been investigated by using on-line mass separation of evaporation residues produced by heavy-ion induced complete-fusion reactions. We measured the cross sections for 99Cd, 100In, 101Sn and 102In via 58Ni+58Ni fusion reactions followed by cluster emission, and via 58Ni+50Cr fusion reactions accompanied by evaporation of protons, neutrons or α particles. Both types of reactions yield similar cross sections for the production of exotic nuclei near 100Sn. The data are discussed in comparison with results obtained from statistical-model calculations.

Intense beams of mass-separated, neutron-deficient indium, tin, thallium and lead isotopes

A discharge ion source of the FEBIAD-type that delivers intense beams of neutron-deficient isotopes of indium, tin, thallium and lead produced in heavy-ion-induced fusion reactions is described. After mass separation the isotopically pure beams with intensities of up to 3 × 107 ions/s were available for gamma and laser spectroscopy. This corresponds to an overall separation efficiency of about 30%.

Direct high-precision mass measurements onAm241,243,Pu244, andCf249

The absolute masses of four long-lived transuranium nuclides, $^{241,243}\mathrm{Am}$, $^{244}\mathrm{Pu}$, $^{244}\mathrm{Pu}$, and $^{249}\mathrm{Cf}$, in the vicinity of the deformed $N=152$ neutron shell closure have been measured directly with the Penning-trap mass spectrometer TRIGA-TRAP. Our measurements confirm the AME2012 mass values of $^{241,243}\mathrm{Am}$ and $^{244}\mathrm{Pu}$ within one standard deviation, which were indirectly determined, by decay spectroscopy studies. In the case of the $^{249}\mathrm{Cf}$ mass, a discrepancy of more than three standard deviations has been observed, affecting absolute masses even in the superheavy element region. The implementation of the…

A new reference database for beta-delayed neutrons

International audience; A new database containing all available experimental and evaluated β-delayed neutron data is presented in this paper. The database is the product of an international effort coordinated by the International Atomic Energy Agency. It comprises a microscopic section including all available experimental data on beta-decay half-lives, β-delayed neutron emission probabilities and spectra, as well as new systematics and global theoretical calculations for comparison. The beta-delayed neutron data for individual precursors have been benchmarked against available data on macroscopic properties such as total delayed-neutron yields and spectra, delayed-neutron decay curves and t…

117番元素Ts合成のための48Ca+249Bk融合反応

We have performed an experiment to synthesize the element 117 (Ts) with the $^{48}$Ca+$^{249}$Bk fusion reaction. Four $\alpha$-decay chains attributed to the element 117 were observed. Two of them were long decay chains which can be assigned to the one originating from the $\alpha$ decay of $^{294}$Ts. The other two were short decay chains which are consistent with the one originating from the $\alpha$ decay of $^{293}$Ts. We have compared the present results with the literature data, and found that our present results mostly confirmed the literature data, leading to the firm confirmation of the synthesis of the element 117.