0000000000936601
AUTHOR
U. Hager
Upgrade and yields of the IGISOL facility
The front end of the Jyvaskyla IGISOL facility was upgraded in 2003 by increasing its pumping capacity and by improving the radiation shielding. In late 2005, the skimmer electrode of the mass separator was replaced by a sextupole ion guide, which improved the mass separator efficiency up to an order of magnitude. The current design of the facility is described. The updated yield data, achieved with and without the additional JYFLTRAP purification, using both fusion evaporation reactions and particle induced fission is presented to give an overview of the capability of the facility. These data have been determined either by radioactivity measurements or by direct ion counting after the Penn…
Mass measurements beyond the major r-process waiting point $^{80}$Zn
High-precision mass measurements on neutron-rich zinc isotopes 71m,72-81Zn have been performed with the Penning trap mass spectrometer ISOLTRAP. For the first time the mass of 81Zn has been experimentally determined. This makes 80Zn the first of the few major waiting points along the path of the astrophysical rapid neutron capture process where neutron separation energy and neutron capture Q-value are determined experimentally. As a consequence, the astrophysical conditions required for this waiting point and its associated abundance signatures to occur in r-process models can now be mapped precisely. The measurements also confirm the robustness of the N = 50 shell closure for Z = 30 farthe…
Applications of the total absorption technique to improve reactor decay heat calculations: study of the beta decay of [sup 102,104,105]Tc
The decay heat of the fission products plays an important role in predicting the heat‐up of nuclear fuel after reactor shutdown. This form of energy release is calculated as the sum of the energy‐weighted activities of all fission products P(t) = ΣEiλiNi(t), where Ei is the decay energy of nuclide i (gamma and beta component), λi is the decay constant of nuclide i and Ni(t) is the number of nuclide i at cooling time t. Even though the reproduction of the measured decay heat has improved in recent years, there is still a long standing discrepancy at t∼1000 s cooling time for some fuels. A possible explanation for this disagreement can been found in the work of Yoshida et al. [1], who demonst…
Time-separated oscillatory fields for high-precision mass measurements on short-lived Al and Ca nuclides
High-precision Penning trap mass measurements on the stable nuclide 27Al as well as on the short-lived radionuclides 26Al and 38,39Ca have been performed by use of radiofrequency excitation with time-separated oscillatory fields, i.e. Ramsey's method, as recently introduced for the excitation of the ion motion in a Penning trap, was applied. A comparison with the conventional method of a single continuous excitation demonstrates its advantage of up to ten times shorter measurements. The new mass values of 26,27Al clarify conflicting data in this specific mass region. In addition, the resulting mass values of the superallowed beta-emitter 38Ca as well as of the groundstate of the beta-emitte…
Mass Measurements and Implications for the Energy of the High-Spin Isomer inAg94
Nuclides in the vicinity of {sup 94}Ag have been studied with the Penning trap mass spectrometer JYFLTRAP at the Ion-Guide Isotope Separator On-Line. The masses of the two-proton-decay daughter {sup 92}Rh and the beta-decay daughter {sup 94}Pd of the high-spin isomer in {sup 94}Ag have been measured, and the masses of {sup 93}Pd and {sup 94}Ag have been deduced. When combined with the data from the one-proton- or two-proton-decay experiments, the results lead to contradictory mass excess values for the high-spin isomer in {sup 94}Ag, -46 370(170) or -44 970(100) keV, corresponding to excitation energies of 6960(400) or 8360(370) keV, respectively.
Mass measurements and implications for the energy of the high-spin isomer in 94Ag.
Nuclides in the vicinity of 94Ag have been studied with the Penning trap mass spectrometer JYFLTRAP at the Ion-Guide Separator On-Line. The masses of the two-proton-decay daughter 92Rh and the beta-decay daughter 94Pd of the high-spin isomer in 94Ag have been measured, and the masses of 93Pd and 94Ag have been deduced. When combined with the data from the one-proton or two-proton-decay experiments, the results lead to contradictory mass excess values for the high-spin isomer in 94Ag, -46370(170) or -44970(100) keV, corresponding to excitation energies of 6960(400) or 8360(370) keV, respectively.
Restoration of theN=82Shell Gap from Direct Mass Measurements ofSn132,134
A high-precision direct Penning trap mass measurement has revealed a 0.5-MeV deviation of the binding energy of (134)Sn from the currently accepted value. The corrected mass assignment of this neutron-rich nuclide restores the neutron-shell gap at N=82, previously considered to be a case of "shell quenching." In fact, the new shell gap value for the short-lived (132)Sn is larger than that of the doubly magic (48)Ca which is stable. The N=82 shell gap has considerable impact on fission recycling during the r process. More generally, the new finding has important consequences for microscopic mean-field theories which systematically deviate from the measured binding energies of closed-shell nu…
Magnetic field stabilization for high-accuracy mass measurements on exotic nuclides
The magnetic-field stability of a mass spectrometer plays a crucial role in precision mass measurements. In the case of mass determination of short-lived nuclides with a Penning trap, major causes of instabilities are temperature fluctuations in the vicinity of the trap and pressure fluctuations in the liquid helium cryostat of the superconducting magnet. Thus systems for the temperature and pressure stabilization of the Penning trap mass spectrometer ISOLTRAP at the ISOLDE facility at CERN have been installed. A reduction of the fluctuations by at least one order of magnitude downto dT=+/-5mK and dp=+/-50mtorr has been achieved, which corresponds to a relative frequency change of 2.7x10^{-…
TAS measurements for reactor physics and nuclear structure
In this contribution we will present recent total absorption measurements of the beta decay of neutron‐rich nuclei performed at the IGISOL facility of the Univ. of Jyvaskyla. In the measurements the JYFL Penning Trap was used as a high resolution isobaric separator. The total absorption technique will be described and the impact of recent results in the fields of reactor physics (decay heat calculations) and nuclear structure will be discussed.
Total absorption study of theβdecay of102,104,105Tc
The $\ensuremath{\beta}$-feeding probabilities for three important contributors to the decay heat in nuclear reactors, namely ${}^{102,104,105}$Tc, have been measured using the total absorption spectroscopy technique. For the measurements, sources of very high isobaric purity have been obtained using a Penning trap (JYFLTRAP). A detailed description of the data analysis is given and the results are compared with high-resolution measurements and theoretical calculations.