0000000001072367
AUTHOR
A. Lightfoot
In-beam spectroscopic study of Cf244
The ground-state rotational band of the neutron-deficient californium (Z = 98) isotope 244Cf was identified for the first time and measured up to a tentative spin and parity of I I-pi = 20(+). The observation of the rotational band indicates that the nucleus is deformed. The kinematic and dynamic moments of inertia were deduced from the measured gamma-ray transition energies. The behavior of the dynamic moment of inertia revealed an up-bend due to a possible alignment of coupled nucleons in high-j orbitals starting at a rotational frequency of about (h) over bar (omega) = 0.20 MeV. The results were compared with the systematic behavior of the even-even N = 146 isotones as well as with avail…
Stability of the heaviest elements: K isomer in No250
Decay spectroscopy of No250 has been performed using digital electronics and pulse-shape analysis of the fast nuclear decays for the first time. Previous studies of No250 reported two distinct fission decay lifetimes, related to the direct fission of the ground state and to the decay of an isomeric state but without the possibility to determine if the isomeric state decayed directly via fission or via internal electromagnetic transitions to the ground state. The data obtained in the current experiment allowed the puzzle to finally be resolved, attributing the shorter half-life of t1/2=3.8±0.3μs to the ground state and the longer half-life t1/2=34.9−3.2+3.9μs to the decay of an isomeric stat…
First observation of high-K isomeric states in $$^{249}$$Md and $$^{251}$$Md
Decay spectroscopy of the odd-proton nuclei $^{249}$Md and $^{251}$Md has been performed. High-K isomeric states were identified for the first time in these two nuclei through the measurement of their electromagnetic decay. An isomeric state with a half-life of 2.8(5) ms and an excitation energy $\ge 910$ keV was found in $^{249}$Md. In $^{251}$Md, an isomeric state with a half-life of 1.4(3) s and an excitation energy $\ge 844$ keV was found. Similarly to the neighbouring $^{255}$Lr, these two isomeric states are interpreted as 3 quasi-particle high-K states and compared to new theoretical calculations. Excited nuclear configurations were calculated within two scenarios: via blocking nucle…
Prompt and delayed spectroscopy of 203At : Observation of a shears band and a 29/2+ isomeric state
Using fusion-evaporation reactions, a gas-filled recoil separator, recoil-gating technique and recoil-isomer decay tagging technique we have extended the level scheme of 203 At ( N = 118 ) significantly. We have observed an isomeric [ τ = 14.1 ( 3 ) μ s ] state with a spin and parity of 29 / 2 + . The isomeric state is suggested to originate from the π ( h 9 / 2 ) ⊗ ∣ ∣ 202 Po ; 11 − ⟩ coupling, and it is depopulated through 286 keV E 2 and 366 keV E 3 transitions. In addition, we have observed a cascade of magnetic-dipole transitions which is suggested to be generated by the shears mechanism. peerReviewed
Experimental study of isomeric intruder 12+ states in At197,203
A newly observed isomeric intruder ${\textonehalf{}}^{+}$ state $[{T}_{\textonehalf{}}=3.5(6)\phantom{\rule{0.16em}{0ex}}\mathrm{ms}]$ is identified in $^{203}\mathrm{At}$ using a gas-filled recoil separator and fusion-evaporation reactions. The isomer is depopulated through a cascade of $E3$ and mixed $M1/E2$ transitions to the ${9/2}^{\ensuremath{-}}$ ground state, and it is suggested to originate from the $\ensuremath{\pi}{({s}_{\textonehalf{}})}^{\ensuremath{-}1}$ configuration. In addition, the structures above the ${\textonehalf{}}^{+}$ state in $^{203}\mathrm{At}$ and $^{197}\mathrm{At}$ are studied using in-beam $\ensuremath{\gamma}$-ray spectroscopy, recoil-decay tagging, and recoi…
Stability of the heaviest elements : K isomer in 250No
Decay spectroscopy of 250No has been performed using digital electronics and pulse-shape analysis of the fast nuclear decays for the first time. Previous studies of 250No reported two distinct fission decay lifetimes, related to the direct fission of the ground state and to the decay of an isomeric state but without the possibility to determine if the isomeric state decayed directly via fission or via internal electromagnetic transitions to the ground state. The data obtained in the current experiment allowed the puzzle to finally be resolved, attributing the shorter half-life of t1/2 = 3.8 ± 0.3 μs to the ground state and the longer half-life t1/2 = 34.9+3.9 −3.2 μs to the decay of an isom…
A time-of-flight correction procedure for fast-timing data of recoils with varying implantation positions at a spectrometer focal plane
Abstract Fast-timing measurements at the focal plane of a separator can suffer from poor timing resolution. This is due to the variations in time-of-flight (ToF) for photons travelling to a given detector, which arise from the changes in the implantation positions of the recoil nuclei emitting the γ rays of interest. In order to minimise these effects on timing measurements, a procedure is presented that improves fast-timing data by performing ToF corrections on an event-by-event basis. This method was used to correct data collected with an array of eight LaBr 3 detectors, which detected γ rays from spatially distributed 138Gd recoil-implants at the focal plane of the Recoil-Ion-Transport-U…
Production cross section and decay study of $^{243}$Es and $^{249}$Md
In the study of the odd-$Z$, even-$N$ nuclei $^{243}$Es and $^{249}$Md, performed at the University of Jyv\"askyl\"a, the fusion-evaporation reactions $^{197}$Au($^{48}$Ca,2$n$)$^{243}$Es and $^{203}$Tl($^{48}$Ca,2$n$)$^{249}$Md have been used for the first time. Fusion-evaporation residues were selected and detected using the RITU gas-filled separator coupled with the focal-plane spectrometer GREAT. For $^{243}$Es, the recoil decay correlation analysis yielded a half-life of $24 \pm 3$s, and a maximum production cross section of $37 \pm 10$ nb. In the same way, a half-life of $26 \pm 1$ s, an $\alpha$ branching ratio of 75 $\pm$ 5%, and a maximum production cross section of 300 $\pm$ 80 nb…
Production cross section and decay study of Es243 and Md249
In the study of the odd-$Z$, even-$N$ nuclei $^{243}$Es and $^{249}$Md, performed at the University of Jyv\"askyl\"a, the fusion-evaporation reactions $^{197}$Au($^{48}$Ca,2$n$)$^{243}$Es and $^{203}$Tl($^{48}$Ca,2$n$)$^{249}$Md have been used for the first time. Fusion-evaporation residues were selected and detected using the RITU gas-filled separator coupled with the focal-plane spectrometer GREAT. For $^{243}$Es, the recoil decay correlation analysis yielded a half-life of $24 \pm 3$s, and a maximum production cross section of $37 \pm 10$ nb. In the same way, a half-life of $26 \pm 1$ s, an $\alpha$ branching ratio of 75 $\pm$ 5%, and a maximum production cross section of 300 $\pm$ 80 nb…
In-beam spectroscopic study of $^{244}$Cf
The ground-state rotational band of the neutron-deficient californium ( Z = 98 ) isotope 244 Cf was identified for the first time and measured up to a tentative spin and parity of I π = 20 + . The observation of the rotational band indicates that the nucleus is deformed. The kinematic and dynamic moments of inertia were deduced from the measured γ -ray transition energies. The behavior of the dynamic moment of inertia revealed an up-bend due to a possible alignment of coupled nucleons in high- j orbitals starting at a rotational frequency of about ℏ ω = 0.20 MeV . The results were compared with the systematic behavior of the even-even N = 146 isotones as well as with available theoretical c…