Thermal disorder driven magnetic phases in van der Waals magnet CrI3

Abstract Magnetic phase transitions often occur spontaneously at specific critical temperatures and are instrumental to understand the origin of long-range spin order in condensed matter systems. The presence of more than one critical temperature (Tc) has been observed in several compounds where the coexistence of competing magnetic orders highlights the importance of phase separation driven by different factors such as pressure, temperature and chemical composition. However, it is unknown whether recently discovered two-dimensional (2D) van der Walls (vdW) magnetic materials show such intriguing phenomena that can result in rich phase diagrams with novel magnetic features to be explored. H…