0000000001194867

AUTHOR

E A Woźnica

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A clickable NHC–Au(i)-complex for the preparation of stimulus-responsive metallopeptide amphiphiles

2018

We report the synthesis of an alkyne functionalised NHC-Au(i)-complex which is conjugated with amphiphilic oligopeptides using a copper(i) catalysed cycloaddition. The resulting Au(i)-metalloamphiphiles are shown to self-assemble into charge-regulated stimulus-responsive supramolecular polymers in water via a weakly cooperative polymerisation mechanism.

chemistry.chemical_classificationStimuli responsive010405 organic chemistryChemistryMetals and AlloysAlkyneGeneral ChemistryConjugated system010402 general chemistry01 natural sciencesCombinatorial chemistryCatalysisCycloaddition0104 chemical sciencesSurfaces Coatings and FilmsElectronic Optical and Magnetic MaterialsSupramolecular polymersPolymerizationAmphiphileMaterials ChemistryCeramics and CompositesClickableChemical Communications
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