Chemical studies of Fl (element 114): Heaviest chemically studied element

High brilliance uranium beams for the GSI FAIR

The 40 years old GSI-UNILAC (Universal Linear Accelerator) as well as the heavy ion synchrotron SIS18 will serve as a high current heavy ion injector for the new FAIR (Facility for Antiproton and Ion Research) synchrotron SIS100. In the context of an advanced machine investigation program in combination with the ongoing UNILAC upgrade program, a new uranium beam intensity record (11.5 emA, ${\mathrm{U}}^{29+}$) at very high beam brilliance was achieved recently in a machine experiment campaign. This is an important step paving the way to fulfill the FAIR heavy ion high intensity beam requirements. Results of high current uranium beam measurements applying a newly developed pulsed hydrogen g…

Measurements of charge state distributions of 0.74 and 1.4  MeV/u heavy ions passing through dilute gases

In many modern heavy-ion accelerator facilities, gas strippers are used to increase the projectile charge state for improving the acceleration efficiency of ion beams to higher energies. For this application, the knowledge on the behavior of charge state distributions of heavy-ions after passing through dilute gases is of special interest. Charge state distributions of uranium ($^{238}\mathrm{U}$), bismuth ($^{209}\mathrm{Bi}$), titanium ($^{50}\mathrm{Ti}$), and argon ($^{40}\mathrm{Ar}$) ion beams with energies of $0.74\text{ }\mathrm{MeV}/\mathrm{u}$ and $1.4\text{ }\mathrm{MeV}/\mathrm{u}$ after passing through hydrogen (${\mathrm{H}}_{2}$), helium (He), carbon dioxide (${\mathrm{CO}}_{…

Applications of the pulsed gas stripper technique at the GSI UNILAC

Abstract In the frame of an upgrade program for the GSI UNILAC, preparing it for the use as an injector system for FAIR, a pulsed gas stripper cell was developed. It utilizes the required low duty cycle by applying a pulsed gas injection instead of a continuous gas inlet. The resulting lower gas consumption rate enables the use of low-Z gas targets over a wide range of stripper target thicknesses. The setup enables an increased flexibility for the accelerator by allowing the gas stripper to be used in time-sharing beam operation matching the capabilities of the GSI UNILAC like the acceleration of different ion beams in quasi-parallel operation. Measured charge state distributions of 238 U, …

Charge-state dynamics of 1.4- and 11-MeV/u uranium ions penetrating H2 and He gas targets

Abstract Theoretical description and interpretation are presented of the recent experimental data on stripping of fast 238U ions, penetrating H2 and He gaseous targets: obtained in GSI, Darmstadt, Germany at 1.4 MeV/u with a H2 stripper, and in RIKEN, Saitama, Japan at 11 MeV/u with H2 and He strippers. Electron-loss and capture cross sections for uranium ions, interacting with H2 and He targets are calculated and used as input data in the BREIT code to obtain dynamic characteristics of uranium-ion beams: non-equilibrium and equilibrium charge-state fractions, mean and equilibrium charges, and equilibrium thicknesses. Special attention is paid for the calculation of the dynamic characterist…

Radiochemical study of the kinematics of multi-nucleon transfer reactions in 48Ca + 248Cm collisions 10% above the Coulomb barrier

Abstract The kinematics of multi-nucleon transfer reactions in 48Ca + 248Cm collisions at 262 MeV (center of target) was investigated by using a stacked-foil technique and radiochemical separations of trans-curium elements. Trans-curium isotopes were identified by α-particle spectroscopy. For Fm isotopes, by comparing the centroids of the measured post-neutron emission isotope distributions with the most probable primary mass number predicted by Volkov's generalized Q g g systematics, the missing mass (number of evaporated neutrons) is estimated. The latter is compared with that deduced from the measured centroid of the laboratory angular distribution peaked closely to the grazing angle and…

TASCAを用いたCn, Nh, Fl化学実験のためのHg, Tl, PbのSiO2及びAu表面に対するオンライン化学吸着研究

Online gas-solid adsorption studies with single atom quantities of Hg, Tl, and Pb on SiO$_{2}$ and Au surfaces were carried out using short-lived radioisotopes with half-lives in the range of 4-49 s. This is a model study to measure adsorption enthalpies of superheavy elements Cn, Nh, and Fl. The short-lived isotopes were produced and separated by the gas-filled recoil separator TASCA at GSI. The products were stopped in He gas, and flushed into gas chromatography columns made of Si detectors whose surfaces were covered by SiO$_{2}$ or Au. The short-lived Tl and Pb were successfully measured by the Si detectors with the SiO$_{2}$ surface at room temperature. On the other hand, the Hg did no…

Developments on the 1.4 MeV/u Pulsed Gas Stripper Cell

The GSI UNILAC in combination with SIS18 will serve as a high-current, heavy-ion injector for the FAIR facility. It must meet high demands in terms of beam brilliance at a low duty factor. As part of an UNILAC upgrade program dedicated to FAIR, a new pulsed gas stripper cell was developed, aiming for increased beam intensities inside the post-stripper. The pulsed gas injection is synchronized with the beam pulse timing, enabling a highly-demanded, increased gas density. First tests using uranium beams on a hydrogen target showed a 60%-increased stripping efficiency into the desired 28+ charge state. In 2015, the setup was improved to be able to deliver increased target thicknesses and enhan…