6533b821fe1ef96bd127b6b8

RESEARCH PRODUCT

Considering lithium-ion battery 3D-printing via thermoplastic material extrusion and polymer powder bed fusion

Arash JamaliLauri KivijärviEric MacdonaldMichel ArmandElmeri LahtinenAurélie CaylaAurélie CaylaMatti HaukkaAlexis MaurelAlexis MaurelLoic DupontLoic DupontHyeonseok KimHyeonseok KimSylvie GrugeonSylvie GrugeonStéphane Panier

subject

chemistry.chemical_classificationBattery (electricity)Polypropylene0209 industrial biotechnologyThermoplasticMaterials sciencebusiness.industryBiomedical Engineering3D printing02 engineering and technology021001 nanoscience & nanotechnologyIndustrial and Manufacturing EngineeringLithium-ion batterychemistry.chemical_compound020901 industrial engineering & automationchemistryElectrodeGeneral Materials ScienceExtrusionComposite material0210 nano-technologybusinessEngineering (miscellaneous)Electrical conductor

description

Abstract In this paper, the ability to 3D print lithium-ion batteries through Pmnbspace thermoplastic material extrusion and polymer powder bed fusion is considered. Focused on the formulation of positive electrodes composed of polypropylene, LiFePO4 as active material, and conductive additives, advantages and drawbacks of both additive manufacturing technologies, are thoroughly discussed from the electrochemical, electrical, morphological and mechanical perspectives. Based on these preliminary results, strategies to further optimize the electrochemical performances are proposed. Through a comprehensive modeling study, the enhanced electrochemical suitability at high current densities of various complex three-dimensional lithium-ion battery architectures, in comparison with classical two-dimensional planar design, is highlighted. Finally, the direct printing capability of the complete lithium-ion battery by means of multi-materials printing options processes is examined.

https://doi.org/10.1016/j.addma.2020.101651