6533b827fe1ef96bd1285dd5

RESEARCH PRODUCT

Efficient energy conversion for cubic third-harmonic generation that is phase matched in KTiOPO(4).

Benoît BoulangerY. GuillienJ.p. Feve

subject

Sum-frequency generationMaterials sciencebusiness.industryEnergy conversion efficiencyPhase (waves)Second-harmonic generationLaserAtomic and Molecular Physics and Opticslaw.inventionOpticslawPicosecondDispersion (optics)businessGaussian beam

description

We demonstrate, for the first time to our knowledge, that efficient third-harmonic generation can be achieved with a cubic contribution much larger than the quadratic processes. An energy-conversion efficiency of 2.4% is achieved for cubic third-harmonic generation that is phase matched along the x axis of a KTiOPO(4) crystal by use of a picosecond fundamental laser emitting at 1618 nm. The associated cascading processes are only 10% of the pure cubic interaction, which is very suitable for study of the specific quantum optical correlations. Calculations of the third-harmonic generation conversion efficiency with respect to group-velocity dispersion and to the longitudinal Gaussian beam profile account well for our experimental results.

10.1364/ol.25.001373https://pubmed.ncbi.nlm.nih.gov/18066221