6533b828fe1ef96bd12882b8

RESEARCH PRODUCT

The kinetics of defect accumulation under irradiation: many-particle effects

V. N. KuzovkovEugene A. Kotomin

subject

Particle systemAnnihilationCritical distanceMaterials scienceCondensed matter physicsKröger–Vink notationMany-body theoryKineticsFrenkel defectIrradiationCondensed Matter PhysicsMathematical PhysicsAtomic and Molecular Physics and Optics

description

The kinetics of Frenkel defect accumulation under permanent particle source (irradiation) is discussed with special emphasis on many-particle effects. Defect accumulation is restricted by their diffusion and annihilation, A + B → 0, if the relative distance is less than the critical distance r0. A novel formalism of many-point particle densities based on Kirkwood's superposition approximation is developed to take into account aggregation of similar defects (A−A, B−B). The dependence of the saturation concentration after a prolonged irradiation upon spatial dimension ( = 1, 2, 3), defect mobility and the initial correlation within geminate pairs is analyzed. It is shown that the defect concentration really saturates only for = 3 whereas for low dimensions ( = 1, 2) it is not the case because of the macroscopic defect separation into alternating domains containing defects A or B only.

https://doi.org/10.1088/0031-8949/47/4/020